Metasurfaces, as the ultrathin version of metamaterials, have caught growing attention due to their superior capability in controlling the phase, amplitude and polarization states of light. Among various types of metasurfaces, geometric metasurface that encodes a geometric or Pancharatnam–Berry phase into the orientation angle of the constituent meta-atoms has shown great potential in controlling light in both linear and nonlinear optical regimes. The robust and dispersionless nature of the geometric phase simplifies the wave manipulation tremendously. Benefitting from the continuous phase control, metasurface holography has exhibited advantages over conventional depth controlled holography with discretized phase levels. Here we report on spin and wavelength multiplexed nonlinear metasurface holography, which allows construction of multiple target holographic images carried independently by the fundamental and harmonic generation waves of different spins. The nonlinear holograms provide independent, nondispersive and crosstalk-free post-selective channels for holographic multiplexing and multidimensional optical data storages, anti-counterfeiting, and optical encryption.

Nonlinear processes are often governed by selection rules imposed by the symmetries of the molecular configurations. The most well-known examples include the role of centrosymmetry breaking for the generation of even harmonics, and the selection rule related to the rotational symmetry in harmonic generation for fundamental beams with circular polarizations. While the role of centrosymmetry breaking in second harmonic generation has been extensively studied in plasmonic systems, the investigation of selection rules pertaining to circular polarization states of harmonic generation is limited to crystals, i.e., symmetries at the atomic level. In this Letter we demonstrate the rotational symmetry dependent third harmonic generation from nonlinear plasmonic metacrystals. We show that the selection rule can be imposed by the rotational symmetry of metacrystals embedded into an isotropic organic nonlinear thin film. The results presented here may open new avenues for designing symmetry-dependent nonlinear optical responses with tailored plasmonic nanostructures.

3D chirality is shown to be unnecessary for introducing strong circular dichroism for harmonic generations. Specifically, near-unity circular dichroism for both second-harmonic generation and third-harmonic generations is demonstrated on suitably designed ultrathin plasmonic metasurfaces with only 2D planar chirality. The study opens up new routes for designing chip-type biosensing platform, which may allow for highly sensitive detection of bio- and chemical molecules with weak chirality.

Magnetic fields in turbulent, convective high-β plasma naturally develop highly tangled and complex topologies-the solar photosphere being the paradigmatic example. These fields are mostly undetectable by standard diagnostic techniques with finite spatio-temporal resolution due to cancellations of Zeeman polarization signals. Observations of resonance scattering polarization have been considered to overcome these problems. But up to now, observations of scattering polarization lack the necessary combination of high sensitivity and high spatial resolution in order to directly infer the turbulent magnetic structure at the resolution limit of solar telescopes. Here, we report the detection of clear spatial structuring of scattering polarization in a magnetically quiet solar region at disk center in the Sr i 4607Å spectral line on granular scales, confirming theoretical expectations. We find that the linear polarization presents a strong spatial correlation with the local quadrupole of the radiation field. The result indicates that polarization survives the dynamic and turbulent magnetic environment of the middle photosphere and is thereby usable for spatially resolved Hanle observations. This is an important step toward the long-sought goal of directly observing turbulent solar magnetic fields at the resolution limit and investigating their spatial structure.