A statistical formalism for describing the behavior of sprays is presented, which includes the effects of droplet growth, the formation of new droplets, collisions, and aerodynamic forces. Criteria for the efficiency of impinging jet atomization are developed. It is shown that if the incident jets have a size distribution of a generalized Rosin-Rammler type, then the resulting spray belongs to the same class of distributions. The size history of evaporating sprays is also obtained from the theory. A spray combustion analysis given by Probert is extended to include more general size distributions and the effects of droplet interactions and the relative motion of the droplets and the fluid. It is shown that the over-all spray evaporation rate is largest for uniform sprays.

To study effects of flow inhomogeneities on the dynamics of laminar flamelets in turbulent flames, with account taken of influences of the gas expansion produced by heat release, a previously developed theory of premixed flames in turbulent flows, that was based on a diffusive-thermal model in which thermal expansion was neglected, and that applied to turbulence having scales large compared with the laminar flame-thickness, is extended by eliminating the hypothesis of negligible expansion and by adding the postulate of weak-intensity turbulence. The consideration of thermal expansion motivates the formal introduction of multiple-scale methods, which should be useful in subsequent investigations. Although the hydrodynamic-instability mechanism of Landau is not considered, no restriction is imposed on the density change across the flame front, and the additional transverse convection correspondingly induced by the tilted front is described. By allowing the heat-to-reactant diffusivity ratio to differ slightly from unity, clarification is achieved of effects of phenomena such as flame stretch and the flame-relaxation mechanism traceable to transverse diffusive processes associated with flame-front curvature. By carrying the analysis to second order in the ratio of the laminar flame thickness to the turbulence scale, an equation for evolution of the flame front is derived, containing influences of transverse convection, flame relaxation and stretch. This equation explains anomalies recently observed at low frequencies in experimental data on power spectra of velocity fluctuations in turbulent flames. It also shows that, concerning the diffusive-stability properties of the laminar flame, the density change across the flame thickness produces a shift of the stability limits from those obtained in the purely diffusive-thermal model. At this second order, the turbulent correction to the flame speed involves only the mean area increase produced by wrinkling. The analysis is carried to the fourth order to demonstrate the mean-stretch and mean-curvature effects on the flame speed that occur if the diffusivity ratio differs from unity.

A statistical theory is developed for the structure and propagation velocity of premixed flames in turbulent flows with scales large compared with the laminar flame thickness. The analysis, free of usual closure assumptions, involves a regular perturbation for small values of the ratio of laminar flame thickness to turbulence scale, termed the scale ratio ε, and a singular perturbation for large values of the non-dimensional activation temperature β. Any effects of the flame on the flow are considered to be given. In this initial study, molecular coefficients for diffusion of heat and reactants are set equal. The results identify convective-diffusive and reactive-diffusive zones in the flame and predict thickening of the flame by turbulence through streamwise displacement of the reactive-diffusive zone. Profiles for intensities of temperature fluctuations and for streamwise turbulent transport are obtained. A fundamental quantity occurring in the analysis is the longitudinal displacement of the reactive-diffusive zone in an Eulerian frame by turbulent fluctuations, and to first order in the scale ratio this equals the longitudinal displacement of fluid elements in an Eulerian frame by turbulent fluctuations, herein termed simply the Eulerian displacement. To first order in the scale ratio it is found that, if the Eulerian displacement experiences the same type of statistical non-stationarity as the corresponding Lagrangian displacement, then the diffusion approximation is valid for streamwise turbulent transport but the turbulent flame thickens as time increases, while if the Eulerian displacement is statistically stationary then the diffusion approximation necessitates a negative coefficient of diffusion in part of the flame but the flame thickness remains constant. By carrying the analysis to second order in the scale ratio it is shown that the turbulent-flame speed exceeds the laminar-flame speed by an amount proportional to the mean square of the transverse gradient of the Eulerian displacement. This result can be understood from the mechanistic viewpoint of a wrinkled laminar flame in terms of the increase in flame area produced by turbulence. Thus the theory provides a precise statistical quantification of the model of the wrinkled laminar flame for describing structures of turbulent flames.

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A four-step reduced chemical-kinetic mechanism for syngas combustion is proposed for use under conditions of interest for gas-turbine operation. The mechanism builds upon our recently published three-step mechanism for H 2 -air combustion (Boivin et al., Proc. Comb. Inst. 33, 2010), which was cate that the reduced description can be applied with reasonable accuracy in numerical studies of gas-turbine syngas combustion.

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