We propose a new application of inexpensive light‐emitting diode (LED)‐based Sun photometers, consisting of measuring the aerosol optical thickness (AOT) with high resolution within metropolitan scales. Previously, these instruments have been used at continental scales by the GLOBE program, but this extension is already covered by more expensive and higher‐precision instruments of the AERONET global network. For this we built an open source two‐channeled LED‐based Sun photometer based on previous developments, with improvements in the hardware, software, and modifications on the calibration procedure. Among these we highlight the use of MODTRAN to characterize the effect introduced by using LED sensors in the AOT retrieval, an open design available for the scientific community and a calibration procedure that takes advantage of a CIMEL Sun photometer located within the city, enables the intercomparison of several LED Sun photometers with a common reference. We estimated the root‐mean‐square error in the AOT retrieved by the prototypes as 0.006 at the 564 nm and 0.009 at the 408 nm. This error is way under the magnitude of the AOT daily cycle variability measured by us in our campaigns, even for distances closer than 15 km. In addition to inner city campaigns, we also show aerosol‐tracing applications by measuring AOT variations from the city of Santiago to the Andes glaciers. Measuring AOT at high spatial resolution in urban areas can improve our understanding of urban scale aerosol circulation, providing information for solar energy planning, health policies, and climatological studies, among others.

Abstract. Visibility reduction caused by fog can be hazardous for human activities, especially for the transport sector. Previous studies show that this problem could be mitigated by improving nowcasting of fog dissipation. To address this issue, we propose a new paradigm which could potentially improve our understanding of the life cycle of adiabatic continental fogs and of the conditions that must take place for fog dissipation. For this purpose, adiabatic fog is defined as a layer filled with suspended liquid water droplets, extending from an upper boundary all the way down to the surface, with a saturated adiabatic temperature profile. In this layer, the liquid water path (LWP) must exceed a critical value: the critical liquid water path (CLWP). When the LWP is less than the CLWP, the amount of fog liquid water is not sufficient to extend all the way down to the surface, leading to a surface horizontal visibility greater than 1 km. Conversely, when the LWP exceeds the CLWP, the amount of cloud water is enough to reach the surface, inducing a horizontal visibility of less than 1 km. The excess water with respect to the critical value is defined as the reservoir liquid water path (RLWP). The new fog paradigm is formulated as a conceptual model that relates the liquid water path of adiabatic fog with its thickness and surface liquid water content and allows the critical and reservoir liquid water paths to be computed. Both variables can be tracked in real time using vertical profiling measurements, enabling a real-time diagnostic of fog status. The conceptual model is tested using data from 7 years of measurements performed at the SIRTA observatory, combining cloud radar, microwave radiometer, ceilometer, scatterometer, and weather station measurements. In this time period we found 80 fog events with reliable measurements, with 56 of these lasting more than 3 h. The paper presents the conceptual model and its capability to derive the LWP from the fog top height and surface horizontal visibility with an uncertainty of 10.5 g m−2. The impact of fog liquid water path and fog top height variations on fog life cycle (formation to dissipation) is presented based on four case studies and statistics derived from 56 fog events. Our results, based on measurements and an empirical parametrization for the adiabaticity, validate the applicability of the model. The calculated reservoir liquid water path is consistently positive during the mature phase of fog and starts to decrease quasi-monotonously about 1 h before dissipation, reaching a near-zero value at the time of dissipation. Hence, the reservoir liquid water path and its time derivative could be used as indicators of the life cycle stage, to support nowcasting of fog dissipation.

Abstract. This article presents a new cloud radar calibration methodology using solid reference reflectors mounted on masts, developed during two field experiments held in 2018 and 2019 at the Site Instrumental de Recherche par Télédétection Atmosphérique (SIRTA) atmospheric observatory, located in Palaiseau, France, in the framework of the Aerosol Clouds Trace gases Research InfraStructure version 2 (ACTRIS-2) research and innovation program. The experimental setup includes 10 and 20 cm triangular trihedral targets installed at the top of 10 and 20 m masts, respectively. The 10 cm target is mounted on a pan-tilt motor at the top of the 10 m mast to precisely align its boresight with the radar beam. Sources of calibration bias and uncertainty are identified and quantified. Specifically, this work assesses the impact of receiver compression, temperature variations inside the radar, frequency-dependent losses in the receiver's intermediate frequency (IF), clutter and experimental setup misalignment. Setup misalignment is a source of bias, previously undocumented in the literature, that can have an impact of the order of tenths of a decibel in calibration retrievals of W-band radars. A detailed analysis enabled the quantification of the importance of each uncertainty source to the final cloud radar calibration uncertainty. The dominant uncertainty source comes from the uncharacterized reference target which reached 2 dB. Additionally, the analysis revealed that our 20 m mast setup with an approximate alignment approach is preferred to the 10 m mast setup with the motor-driven alignment system. The calibration uncertainty associated with signal-to-clutter ratio of the former is 10 times smaller than for the latter. Following the proposed methodology, it is possible to reduce the added contribution from all uncertainty terms, excluding the target characterization, down to 0.4 dB. Therefore, this procedure should enable the achievement of calibration uncertainties under 1 dB when characterized reflectors are available. Cloud radar calibration results are found to be repeatable when comparing results from a total of 18 independent tests. Once calibrated, the cloud radar provides valid reflectivity values when sampling midtropospheric clouds. Thus, we conclude that the method is repeatable and robust, and that the uncertainties are precisely characterized. The method can be implemented under different configurations as long as the proposed principles are respected. It could be extended to reference reflectors held by other lifting devices such as tethered balloons or unmanned aerial vehicles.

Abstract. We propose a new paradigm to describe the temporal evolution of continental fog layers. This paradigm defines fog as a layer saturated from the surface to a known upper boundary, and whose liquid water path (LWP) exceeds a critical value, the critical liquid water path (CLWP). When the LWP is less than the CLWP the fog water cannot extend all the way to the surface, leading to a surface horizontal visibility greater than 1 km. On the opposite, when the LWP is larger than the CLWP, the fog water extends all the way to the surface, inducing a horizontal visibility less than 1 km. The excess water with respect to the critical value is then defined as the reservoir liquid water path (RLWP). The new fog paradigm is formulated as a conceptual model that relates the liquid water path of adiabatic fog with its thickness and surface liquid water content, and allows the critical and reservoir liquid water paths to be computed. Both variables can be tracked in real time using vertical profiling measurements, enabling a real time diagnostic of fog status. The conceptual model is tested using data from seven years of measurements performed at the SIRTA observatory, combining cloud radar, microwave radiometer, ceilometer, scatterometer and weather station measurements. In this time period we found 80 fog events with reliable measurements, with 56 of these lasting more than three hours. The paper presents the conceptual model and its capability to derive the LWP from the fog CTH and surface horizontal visibility with an RMS uncertainty of 10.5 g m−2. The impact of fog liquid water path and fog top height variations on fog life cycle (formation to dissipation) is presented based on four case studies, and statistics derived from 56 fog events. Our results show in particular that the reservoir liquid water path is consistently positive during the mature phase of the fog and that it starts to decrease quasi monotonously about one hour before dissipation, reaching a near-zero value at the time of dissipation. The reservoir liquid water path and its time derivative could hence be used as an indicator for life cycle stage and support short range forecasting of fog dissipation.

Abstract. An improved version of the near-real-time decision tool PARAFOG (PFG2) is presented to retrieve pre-fog alert levels and to discriminate between radiation (RAD) and stratus lowering (STL) fog situations. PFG2 has two distinct modules to monitor the physical processes involved in RAD and STL fog formation and is evaluated at European sites. The modules are based on innovative fuzzy logic algorithms to retrieve fog alert levels (low, moderate, high) specific to RAD/STL conditions, minutes to hours prior to fog onset. The PFG2-RAD module assesses also the thickness of the fog. Both the PFG2-RAD and PFG2-STL modules rely on the combination of visibility observations and automatic lidar and ceilometer (ALC) measurements. The overall performance of the PFG2-RAD and PFG2-STL modules is evaluated based on 9 years of measurements at the SIRTA (Instrumented Site for Atmospheric Remote Sensing Research) observatory near Paris and up to two fog seasons at the Paris-Roissy, Vienna, Munich, and Zurich airports. At all sites, pre-fog alert levels retrieved by PFG2 are found to be consistent with the local weather analysis. The advanced PFG2 algorithm performs with a hit rate of about 100 % for both considered fog types and presents a false alarm ratio on the order of 10 % (30 %) for RAD (STL) fog situations. Finally, the first high alerts that result in a subsequent fog event are found to occur for periods of time ranging from −120 min to fog onset, with the first high alerts occurring earlier for RAD than STL cases.