Ceaselessly increasing demands for elaborate nanostructures prompt advanced structure fabrication with good practicability, especially, subwavelength ordered structures in simple lattices even in superlattices over a large area, namely, large-scale photonic lattices, in which lattice arrangement, geometry, and components of unit cells are key factors for their macroscopic optical properties. Moreover, exciting properties always occur at high symmetry points of the lattice; therefore, straightforward modulation of symmetry points over a large area is very important for the investigation and application of photonic lattices. Here, this work establishes a lithography-free approach of undervoltage oxidation (UVO) for regulating high symmetry points in the reciprocal space of a dielectric alumina superlattice. Embedding subunit cells at high symmetry points Γ (M) result in the degenerate energy changing from 1.34 eV (924.6 nm) to 1.87 eV (662.6 nm) under normal excitation at the Γ point, and the degeneracy lifting under off-normal excitation along the Γ–X high symmetry orientation. Furthermore, systematic characterizations of the alumina membrane are presented to learn its dynamic evolution of the morphology on a centimeter scale, and the pore array changes from a hierarchical period to a form of hexagonal close packing, especially at Γ and M points of the square lattice. Therefore, the reported lithography-free alumina-based nanofabrication offers an ability for varying the spatial structure at high symmetry points of photonic lattices, which is of great significance in the fields of nanomanufacturing and has great potential to bring about preferable performances in nanodevices.
Lanthanide-doped upconversion nanoparticles (UCNPs) are appealing for light emitting applications because their high internal conversion efficiency facilitates the amplified spontaneous emission (ASE) under low pumping. In addition, the integration of photonic crystals and microcavities with optical quantum emitters provides a unique opportunity to manipulate their light emissions and generate coherent light sources for quantum photonics. Here, this work describes a two-dimensional (2D) plasmonic lattice of Al nanocone array (Al NCA), which can confine the light at the tip. Light confinement by the enhancement effect supports narrow linewidth resonances as optical feedback for the ASE of UCNPs doped with sensitizer Yb 3+ ions/emitter Ho 3+ ions/relaxator Ce 3+ ions. An off-angle ASE with an enhancement of 19-fold from UCNPs is achieved by propagating lattice plasmons from the Al NCA. Moreover, this upconverting ASE can be switched on or off by adjusting the polarization state of the incident pump light, and photonic band engineering can be used to manipulate it intentionally. This composite plasmonic system opens prospective applications for the ASE as directional emission, real-time tunable wavelengths, controlled multimode lasing, and optical switches.
The light−matter interactions at nanoscale can be enhanced by Blochsurface plasmon polariton (Bloch-SPP) on the plasmonic lattice. An Ag nanohole array in hexagonal arrangement served as an optical cavity to realize the directional and polarized amplified spontaneous emission (ASE) of R6G. A 100-fold enhanced ASE was observed at 15°emission angle under TM polarization when the pump power density exceeded the threshold of 198 W/cm 2 based on the degenerated high state density modes. Moreover, a specific polarization dependence of ASE was modulated by the Bloch-SPP modes, and the degree of polarization was enhanced from 1.3 to 2.1 when the pump power density exceeded the threshold of ASE. This work clarifies the interaction between the gain media and plasmonic systems, which lays a foundation for the plasmonic device designing.
Structural color has been studied through various methods due to its distinguished features of stability, durability, high information storage density and high integration. However, the artificial structural color samples do not exhibit superior performance in color saturation and low angular dependence. Here, we present an approach to acquire additive reflective color based on a metal-dielectric-metal (MDM) stack. The upper layer composed of Ag particles is perforated in a hexagonal arrangement which profits from the dielectric anodic aluminum oxide (AAO) membrane, the size and shape of the Ag particles are getting inhomogeneous as the deposition thickness of the upper layer increasing, which expands the desired absorption range of surface plasmons. The residual non-anodized Al foil serves as a highly reflective substrate for efficient color presenting through the thin-film interference in this plasmonic MDM system. As a result, the color gamut area of this MDM stack is extended 8 times in CIE chromaticity coordinates. Finally, a wafer-scale (diameter of 83 mm) badge of Harbin Engineering University (HEU) with highly saturated colors and a pattern characterized with low angle-dependent property (up to 60°) are presented, which exhibit promising prospects in commercial coloring and imaging.
Strong light–matter coupling manifested by Rabi splitting has drawn considerable interest owing to its fundamental significance for impressive interaction enhancement in the fields of ultrafast active plasmonic devices and quantum information. In this paper, we investigate the coherent optical properties of a plasmonic system consisting of periodic metal nanoparticle arrays covered by a WS2 thin film of atomic layer thickness. The coupling factor, energy splitting, and temporal dynamics of this coherent coupling phenomenon are quantitatively revealed by finite-difference time-domain (FDTD) simulation and a full quantum mechanical model proves that the exciton behavior of the fermionic quantum emitter WS2 is carefully modulated by bosonic surface lattice resonances. This work may pave the way for coherent modulation of polariton and plasmon devices and can potentially open up diverse exciting possibilities like nanoscale light sources, single-photon emitters, and all-optical transistors.
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