We demonstrate for the first time, to the best of our knowledge, the ability of extreme ultraviolet (XUV) Hartmann wavefront sensors to characterize high charge vortex beams produced by high-order harmonic generation up to the order of 25. We also show that phase matched absorption limited high harmonic generation is able to maintain the high charge vortex structure of the XUV beam even in a rather long (1 cm) generation medium.
The investigation of spatio-temporal couplings (STCs) of broadband light beams is becoming a key topic for the optimization as well as applications of ultrashort laser systems. This calls for accurate measurements of STCs. Yet, it is only recently that such complete spatio-temporal or spatio-spectral characterization has become possible, and it has so far mostly been implemented at the output of the laser systems, where experiments take place. In this survey, we present for the first time STC measurements at different stages of a collection of high-power ultrashort laser systems, all based on the chirped-pulse amplification (CPA) technique, but with very different output characteristics. This measurement campaign reveals spatio-temporal effects with various sources, and motivates the expanded use of STC characterization throughout CPA laser chains, as well as in a wider range of types of ultrafast laser systems. In this way knowledge will be gained not only about potential defects, but also about the fundamental dynamics and operating regimes of advanced ultrashort laser systems.
We investigate the coherence of plasma-based soft X-ray laser (XRL) for different conditions that can alter the electron density in the gain region. We first measure the source temporal coherence in amplified spontaneous emission (ASE) mode. We develop a data analysis procedure to extract both its spectral width and pulse duration. These findings are in agreement with the spectral line shape simulations and seeded operation experimental results. Utilizing the deduced spectral width and pulse duration in a one-dimensional Bloch-Maxwell code, we reproduce the experimental temporal coherence properties of the seeded-XRL. Finally, we demonstrate efficient lasing in ASE and seeded mode at an electron density two times higher than the routine conditions. In this regime, using Bloch-Maxwell modeling, we predict the pulse duration of the seeded XRL to be ∼500fs.
Optical beams carrying orbital angular momentum are a very active field of research for their prospective applications, especially at short wavelengths. We consider here such beams produced through high-harmonic generation (HHG) in a rare gas and analyze the characterization of their high-charge vortex structure by an extreme ultraviolet Hartmann wavefront sensor. We show that such HHG beams are generally composed of a set of numerous vortex modes. The sensitivity of the intensity and phase of the HHG beam to the infrared laser aberrations is investigated using a deformable mirror.
We present an experimental intensity and wavefront characterization of the infrared vortex driver as well as the extreme ultraviolet vortex obtained through high harmonic generation in an extended generation medium. In a loose focusing geometry, an intense vortex beam obtained through phase-matched absorption-limited high harmonic generation in a 15 mm long Argon filled gas-cell permits single-shot characterization of the vortex structure. Moreover, our study validates the multiplicative law of momentum conservation even for such an extended generation medium.
We demonstrate that high harmonic generation when driven by vortex driver contaminated with various orbital angular momentum (OAM) modes, the upconverted EUV harmonic deviates from perturbative conversion law to exhibit a spectrum of OAM orders.
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