The crystal structure of a disordered form of Cr 1/3 NbS2 has been characterized using diffraction and inelastic scattering of synchrotron radiation. In contrast to the previously reported symmetry (P6322), the crystal can be described by a regular twinning of an average P63 structure with three disordered positions of the Cr ions. Short-range correlations of the occupational disorder result in a quite intense and structured diffuse scattering; a static nature of the disorder was unambiguously attributed by the inelastic x-ray scattering. The diffuse scattering has been modeled using a reverse Monte-Carlo algorithm assuming a disorder of the Cr sub-lattice only. The observed correlated disorder of the Cr sub-lattice reduces the temperature of the magnetic ordering from 130 K to 88 K and drastically modifies the field dependence of the magnetization as it is evidenced by the SQUID magnetometery. We conclude, that in contrast to the helicoidal spin structure assumed for P6322 form, the compound under study is ferromagnetically ordered with a pronounced in-plane anisotropy.
We have used time-resolved scanning Kerr microscopy (TRSKM) and micromagnetic simulations to demonstrate that, when driven by spatially uniform microwave field, the edges of patterned magnetic samples represent both efficient and highly tunable sources of propagating spin waves. The excitation is due to the local enhancement of the resonance frequency induced by the non-uniform dynamic demagnetizing field generated by precessing magnetization aligned with the edges. Our findings represent a crucial step forward in the design of nanoscale spin-wave sources for magnonic architectures, and are also highly relevant to the understanding and interpretation of magnetization dynamics driven by spatially-uniform magnetic fields in patterned magnetic samples.
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