The magnetic switching of ferromagnetic nanotubes is investigated as a function of their geometry. Two independent methods are used: Numerical simulations and analytical calculations. It is found that for long tubes the reversal of magnetization is achieved by two mechanism: The propagation of a transverse or a vortex domain wall depending on the internal and external radii of the tube.During the last decade, interesting properties of magnetic nanowires have attracted great attention. Besides the interest in their basic properties, there is evidence that they can be used in the production of new devices. More recently magnetic nanotubes have been grown 1,2,3,4 motivating a new research field. Magnetic measurements, 3 numerical simulations 4 and analytical calculations 5 on such tubes have identified two main states: an in-plane magnetic ordering, namely the fluxclosure vortex state, and a uniform state with all the magnetic moments pointing parallel to the axis of the tube. An important problem is to establish the way and conditions for reversing the orientation of the magnetization. Although the reversal process is well known for ferromagnetic nanowires, 6,7,8,9,10 the equivalent phenomenon in nanotubes has been poorly explored so far in spite of some potential advantages over solid cylinders. Nanotubes exhibit a core-free magnetic configuration leading to uniform switching fields, guaranteeing reproducibility, 4,5 and due to their low density they can float in solutions making them suitable for applications in biotechnology (see [1] and refs. therein).Let us consider a ferromagnetic nanotube in a state with the magnetization M along the tube axis. A constant and uniform magnetic field is then imposed antiparallel to M. After some delay time the magnetization reversal (MR) will start at any end. MR or magnetic switching can occur by means of different mechanisms, depending on the geometrical parameters of the tube. In this paper we will focus on the reversal process by means of two different but complementary approaches: numerical simulations and analytical calculations. Their mutual agreement sustains the results reported in this study.Numerical Simulations. Geometrically, tubes are characterized by their external and internal radii, R and a respectively, and height, H. It is convenient to define the ratio β ≡ a/R, so that β = 0 represents a solid cylinder and β → 1 correspond to a very narrow tube. The internal energy, E, of a nanotube with N magnetic moments can be written aswhere E ij is the dipolar energy given by E ij = µ i · µ j − 3(µ i ·n ij )(µ j ·n ij ) /r 3 ij , with r ij the distance between the magnetic moments µ i and µ j ,μ i the unit vector along the direction of µ i andn ij the unit vector along the direction that connects µ i and µ j . J ij = J is the exchange coupling constant between nearest neighbors and J ij = 0 otherwise. E a = − N i=1 µ i · H a is the contribution of the external magnetic field. In this paper we are interested in soft magnetic materials, in which case anisotropy can be s...
Using molecular dynamic simulations, we study a system of particles interacting through a continuous core-softened potentials consisting of a hard core, a shoulder at closest distances, and an attractive well at further distance. We obtain the pressure-temperature phase diagram of this system for various depths of the tunable attractive well. Since this is a two length scale potential, density, diffusion, and structural anomalies are expected. We show that the effect of increasing the attractive interaction between the molecules is to shrink the region in pressure in which the density and the diffusion anomalies are present. If the attractive forces are too strong, particle will be predominantly in one of the two length scales and no density of diffusion anomaly is observed. The structural anomalous region is present for all the cases.
Molecular dynamics simulations and instantaneous normal mode (INM) analysis of a fluid with core-softened pair interactions and waterlike liquid-state anomalies are performed to obtain an understanding of the relationship between thermodynamics, transport properties, and the potential energy landscape. Rosenfeld scaling of diffusivities with the thermodynamic excess and pair correlation entropy is demonstrated for this model. The INM spectra are shown to carry information about the dynamical consequences of the interplay between length scales characteristic of anomalous fluids, such as bimodality of the real and imaginary branches of the frequency distribution. The INM spectral information is used to partition the liquid entropy into two contributions associated with the real and imaginary frequency modes; only the entropy contribution from the imaginary branch captures the nonmonotonic behavior of the excess entropy and diffusivity in the anomalous regime of the fluid.
Using molecular dynamic simulations we study a family of continuous core-softened potentials consisting of a hard core, a shoulder at closest distances, and an attractive well at further distance. The repulsive shoulder and the well distances represent two length scales. We show that if the first scale, the shoulder, is repulsive or has a small well, the potential has a region in the pressure-temperature phase diagram with density, diffusion, and structural anomalies. However, if the closest scale becomes a deep well, the regions in the pressure-temperature phase diagram where the three anomalies are present shrink and disappear. This result helps in defining two length scales potentials that exhibit anomalies.
We use molecular dynamics simulations to study the diffusion of water inside deformed carbon nanotubes with different degrees of deformation at 300 K. It is found that the number of hydrogen bonds that water forms depends on nanotube topology, leading to an enhancement or suppression of water diffusion. The simulation results reveal that more realistic nanotubes should be considered to understand the confined water diffusion behavior, at least for the narrowest nanotubes, when the interaction between water molecules and carbon atoms are more relevant.
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