Subwavelength optical resonators made of high-index dielectric materials provide efficient ways to manipulate light at the nanoscale through mode interferences and enhancement of both electric and magnetic fields. Such Mie-resonant dielectric structures have low absorption, and their functionalities are limited predominantly by radiative losses. We implement a new physical mechanism for suppressing radiative losses of individual nanoscale resonators to engineer special modes with high quality factors: optical bound states in the continuum (BICs). We demonstrate that an individual subwavelength dielectric resonator hosting a BIC mode can boost nonlinear effects increasing second-harmonic generation efficiency. Our work suggests a route to use subwavelength high-index dielectric resonators for a strong enhancement of light–matter interactions with applications to nonlinear optics, nanoscale lasers, quantum photonics, and sensors.
We observe enhanced third-harmonic generation from silicon nanodisks exhibiting both electric and magnetic dipolar resonances. Experimental characterization of the nonlinear optical response through third-harmonic microscopy and spectroscopy reveals that the third-harmonic generation is significantly enhanced in the vicinity of the magnetic dipole resonances. The field localization at the magnetic resonance results in two orders of magnitude enhancement of the harmonic intensity with respect to unstructured bulk silicon with the conversion efficiency limited only by the two-photon absorption in the substrate.
Strong Mie-type magnetic dipole resonances in all-dielectric nanostructures provide novel opportunities for enhancing nonlinear effects at the nanoscale due to the intense electric and magnetic fields trapped within the individual nanoparticles. Here we study third-harmonic generation from quadrumers of silicon nanodisks supporting high-quality collective modes associated with the magnetic Fano resonance. We observe nontrivial wavelength and angular dependencies of the generated harmonic signal featuring a multifold enhancement of the nonlinear response in oligomeric systems.
We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologicallyprotected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by multipolar Mie resonances of silicon nanoparticles. Variation of the pump-beam wavelength enables independent high-contrast imaging of either bulk modes or spin-momentum-locked edge states. We demonstrate topology-driven tunable localization of the generated harmonic fields and map the pseudospin-dependent unidirectional waveguiding of the edge states bypassing sharp corners. Our observations establish dielectric metasurfaces as a promising platform for the robust generation and transport of photons in topological photonic nanostructures.Topological photonics describes optical structures with the properties analogous to electronic topological insulators [1]. These systems are distinguished by bulk band gaps that host disorder-robust states localized at edges or interfaces and provide a novel approach for designing non-reciprocal or localized modes for optical isolators, photonic-crystal waveguides, and lasers. Since the original demonstration of backscattering-immune photonic topological edge states with the use of a gyrotropic microwave photonic crystal under a strong magnetic field [2], there has been a concerted effort towards realizing topological photonics at the nanoscale. Recently suggested optical designs compatible with non-magnetic alldielectric structures [3][4][5][6][7][8] are now emerging as a promising platform for quantum and nonlinear topological photonics [9][10][11][12].Stimulated by the progress in nanofabrication techniques, a new favourable ground for topological photonics based on dielectric nanoparticles with high refractive index has recently emerged [13,14]. Strong optical resonances and low Ohmic losses make it feasible for practical implementation of topological order for light at subwavelength scales. The underlying conceptual framework is to use arrays of meta-atoms with judiciously engineered shape and lattice structure, with topologically nontrivial features arising from pseudospin degrees of freedom. It bridges fundamental physics of topological phases with resonant nanophotonics and multipolar electrodynamics [15,16]. Topological metasurfaces could form a ground for a new class of ultra-thin devices with functionalities based on novel physical principles through engineering light-matter interactions in synthetic photonic potentials [17]. Their pseudospindependent physics may be useful for manipulation of internal degrees of freedom of light such as polarization and angular momentum.However, the experimental characterization of topological photonic structures becomes much more challenging at the nanoscale. Most implementations so far have been limited to indirect probing of topological states such as transmission spectra [11,[18][19][20], which cannot provide spatially-resolved information about the edge modes and suffer from input/output coupling losses. ...
It is known that the nonlinear optical properties of photonic nanostructures can be modified substantially due to strong field confinement and optical resonances. In this contribution, we study third-harmonic generation from lowloss subwavelength silicon nanodisks arranged in the form of trimer oligomers with varying distance between the nanoparticles. Each of the nanodisks exhibits both electric and magnetic Mie-type resonances that are shown to affect significantly the nonlinear response. We observe the thirdharmonic radiation intensity that is comparable to that of a bulk silicon slab and demonstrate a pronounced reshaping of the third-harmonic spectra due to interference of the nonlinearly generated waves augmented by an interplay between the electric and the magnetic dipolar resonances.
The original Kerker effect was introduced for a hypothetical magnetic sphere, and initially it did not attract much attention due to a lack of magnetic materials required. Rejuvenated by the recent explosive development of the field of metamaterials and especially its core concept of optically-induced artificial magnetism, the Kerker effect has gained an unprecedented impetus and rapidly pervaded different branches of nanophotonics. At the same time, the concept behind the effect itself has also been significantly expanded and generalized. Here we review the physics and various manifestations of the generalized Kerker effects, including the progress in the emerging field of meta-optics that focuses on interferences of electromagnetic multipoles of different orders and origins. We discuss not only the scattering by individual particles and particle clusters, but also the manipulation of reflection, transmission, diffraction, and absorption for metalattices and metasurfaces, revealing how various optical phenomena observed recently are all ubiquitously related to the Kerker's concept.
Sharp optical resonances in high-index dielectric nanostructures have recently attracted significant attention for their promising applications in nanophotonics. Fano resonances, as well as resonances associated with bound states in the continuum (BIC), have independently shown a great potential for applications in nanoscale lasers, sensors, and nonlinear optical devices. Here, we demonstrate experimentally a close connection between Fano and quasi-BIC resonances excited in individual dielectric nanoantennas.We analyze systematically the resonant response of AlGaAs nanoantennas pumped with a structured light in the near-infrared range. We trace a variation of the scattering spectrum that fully agrees with an analytical expression governed by a Fano parameter and observe directly a transition to a quasi-BIC resonance. Our results suggest a unified approach toward the analysis of sharp resonances in subwavelength nanostructures originating from strong coupling of optical modes that can provide high energy localization for enhanced light−matter interactions.
We studied the nonlinear response of a dimer composed of two identical Mie-resonant dielectric nanoparticles illuminated normally by a circularly polarized light. We developed a general theory describing hybridization of multipolar modes of the coupled nanoparticles and reveal nonvanishing nonlinear circular dichroism (CD) in the second-harmonic generation (SHG) signal enhanced by the multipolar resonances in the dimer, provided its axis is oriented under an angle to the crystalline lattice of the dielectric material. We supported our multipolar hybridization theory by experimental results obtained for the AlGaAs dimers placed on an engineered substrate.
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