An Unnoticed Inorganic Solid Electrolyte: Dilithium Sodium Phosphate with the Nalipoite Structure. -Orthorhombic Li2NaPO4 is synthesized by stirring aqueous solutions of LiOH, NaOH, and H3PO4 followed by drying at 700°C in air overnight. The material exhibits conductivity values about two orders of magnitude higher than those of βand γ-Li3PO4 phases, making it a very appealing candidate as solid electrolyte for batteries. DFT calculations are used to evaluate the possibilities of preparing other crystal structures in the Li3-xNaxPO4 (0 ≤ x ≤ 3) system with potential applicability as lithium ion solid electrolyte. -(LOPEZ, M. C.; ORTIZ*, G. F.; ARROYO-DE DOMPABLO, E. M.; TIRADO, J. L.; Inorg. Chem. 53 (2014) 4, 2310-2316, http://dx.
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