We review recent studies of the evolution of collective excitations in atomic nuclei far from the valley of β-stability. Collective degrees of freedom govern essential aspects of nuclear structure, and for several decades the study of collective modes such as rotations and vibrations has played a vital role in our understanding of complex properties of nuclei. The multipole response of unstable nuclei and the possible occurrence of new exotic modes of excitation in weakly-bound nuclear systems, present a rapidly growing field of research, but only few experimental studies of these phenomena have been reported so far. Valuable data on the evolution of the lowenergy dipole response in unstable neutron-rich nuclei have been gathered in recent experiments, but the available information is not sufficient to determine the nature of observed excitations. Even in stable nuclei various modes of giant collective oscillations had been predicted by theory years before they were observed, and for that reason it is very important to perform detailed theoretical studies of the evolution of collective modes of excitation in nuclei far from stability. We therefore discuss the modern theoretical tools that have been developed in recent years for the description of collective excitations in weakly-bound nuclei. The review focuses on the applications of these models to studies of the evolution of low-energy dipole modes from stable nuclei to systems near the particle emission threshold, to analyses of various isoscalar modes, those for which data are already available, as well as those that could be observed in future experiments, to a description of charge-exchange modes and their evolution in neutron-rich nuclei, and to studies of the role of exotic low-energy modes in astrophysical processes.

Large-scale QRPA calculations of the E1 strength are performed on top of HFB calculations in order to derive the radiative neutron capture cross sections for the whole nuclear chart. The spreading width of the GDR is taken into account by analogy with the second-RPA (SRPA) method. The accuracy of HFB+QRPA model based on various Skyrme forces with different pairing prescription and parameterization is analyzed. It is shown that the present model allows to constrain the effective nucleon-nucleon interaction with the GDR data and to provide quantitative predictions of dipole strengths.

Large-scale QRPA calculations of the E1-strength are performed as a first attempt to microscopically derive the radiative neutron capture cross sections for the whole nuclear chart. A folding procedure is applied to the QRPA strength distribution to take the damping of the collective motion into account. It is shown that the resulting E1-strength function based on the SLy4 Skyrme force is in close agreement with photoabsorption data as well as the available experimental E1 strength at low energies. The increase of the E1-strength at low energies for neutron-rich nuclei is qualitatively analyzed and shown to affect the corresponding radiative neutron capture cross section significantly. A complete set of E1-strength function is made available for practical applications in a table format for all 8 ≤ Z ≤ 110 nuclei lying between the proton and the neutron drip lines.

We consider the stochastic propagation of high-energy protons and nuclei in the cosmological microwave and infrared backgrounds, using revised photonuclear cross-sections and following primary and secondary nuclei in the full 2D nuclear chart. We confirm earlier results showing that the high-energy data can be fit with a pure proton extragalactic cosmic ray (EGCR) component if the source spectrum is ∝E −2.6 . In this case the ankle in the CR spectrum may be interpreted as a pair-production dip associated with the propagation. We show that when heavier nuclei are included in the source with a composition similar to that of Galactic cosmic-rays (GCRs), the pair-production dip is not present unless the proton fraction is higher than 85%. In the mixed composition case, the ankle recovers the past interpretation as the transition from GCRs to EGCRs and the highest energy data can be explained by a harder source spectrum ∝E −2.2 -E −2.3 , reminiscent of relativistic shock acceleration predictions, and in good agreement with the GCR data at low-energy and holistic scenarios.

Quadrupole excitations of neutron-rich nuclei are analyzed by using the linear response method in the Quasiparticle Random Phase Approximation (QRPA). The QRPA response is derived starting from the time-dependent Hartree-Fock-Bogoliubov (HFB) equations. The residual interaction between the quasiparticles is determined consistently from the two-body force used in the HFB equations, and the continuum coupling is treated exactly. Calculations are done for the neutron-rich oxygen isotopes. It is found that pairing correlations affect the low-lying states, and that a full treatment of the continuum can change the structure of the states in the giant resonance region.

Nucleonic matter displays a quantum liquid structure, but in some cases finite nuclei behave like molecules composed of clusters of protons and neutrons. Clustering is a recurrent feature in light nuclei, from beryllium to nickel. For instance, in 12 C the Hoyle state, crucial for stellar nucleosynthesis, can be described as a nuclear molecule consisting of three alpha-particles. The mechanism of cluster formation, however, has not yet been fully understood. We show that the origin of clustering can be traced back to the depth of the confining nuclear potential. By employing the theoretical framework of energy density functionals that encompasses both cluster and quantum liquid-drop aspects of nuclei, it is shown that the depth of the potential determines the energy spacings between single-nucleon orbitals, the localization of the corresponding wave functions and, therefore, the degree of nucleonic density clustering. Relativistic functionals, in particular, are characterized by deep single-nucleon potentials. When compared to non-relativistic functionals that yield similar ground-state properties (binding energy, deformation, radii), they predict the occurrence of much more pronounced cluster structures. More generally, clustering is considered as a transitional phenomenon between crystalline and quantum liquid phases of fermionic systems.The occurrence of molecular states in atomic nuclei and the formation of clusters of nucleons were already predicted in the 30's by von Weizsäcker and Wheeler [1,2]. Even though the description of nuclear dynamics became predominantly based on the concept of independent nucleons in a mean-field potential, a renewed interest in clustering phenomena in the 60's led to the development of dedicated theoretical methods [3]. Numerous experimental studies have revealed a wealth of data on clustering phenomena in light nuclei [4], and modern theoretical approaches use microscopic models that fully take into account single-nucleon degrees of freedom [5][6][7]. Clustering gives rise to nuclear molecules. For instance, in 12 C the second 0 + state the Hoyle state that plays a critical role in stellar nucleosynthesis, is predicted to display a three-α structure [8,9]. The binding energy of the α-particle, formed from two protons and two neutrons, is much larger than in other light nuclei. Cluster radioactivity [10], discovered in the 80's, is another manifestation of clustering in atomic nuclei. Experimental signatures of clustering are usually indirect. Quasi-molecular resonances are probed by scattering one cluster on another, such as in the 12 C+ 12 C system [4,11], and cluster structures are also discernible in the breakup of nuclei. Evidence has been reported for the formation of clusters in ground and excited states of a number of α-conjugate nuclei [4], that is nuclei with an equal even number of protons and neutrons, from 8 Be to 56 Ni.The mechanism of cluster formation in nuclei has not yet been fully understood. Deformation plays an important role because it removes the degenera...

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Only one-third of the nucleons in 208Pb occupy the saturation density area. Consequently, nuclear observables related to the average properties of nuclei, such as masses or radii, constrain the equation of state not at the saturation density but rather around the so-called crossing density, localized close to the mean value of the density of nuclei: ρ is approximately equal to 0.11 fm(-3). This provides an explanation for the empirical fact that several equation of state quantities calculated with various functionals cross at a density significantly lower than the saturation one. The third derivative M of the energy per unit of volume at the crossing density is constrained by the giant monopole resonance measurements in an isotopic chain rather than the incompressibility at saturation density. The giant monopole resonance measurements provide M=1100±70 MeV (6% uncertainty), whose extrapolation gives K(∞)=230±40 MeV (17% uncertainty).