The advent of π-stacked layered metal-organic frameworks (MOFs) opened up new horizons for designing compact MOF-based devices as they offer unique electrical conductivity on top of permanent porosity and exceptionally high surface area. By taking advantage of the modular nature of these electrically conductive (EC) MOFs, an unlimited number of materials can be created for applications in electronic devices such as battery electrodes, supercapacitors, and spintronics. Permutation of structural building blocks including different metal nodes and organic linkers results in new systems with unprecedented and unexplored physical and chemical properties. With the ultimate goal of providing a platform for accelerated materials design and discovery, here, we lay the foundations towards creation of the first comprehensive database of EC-MOFs with an experimentally guided approach. The first phase of this database,