Although soil quality can be highly altered by mining activities, there are few reports on soil pollution in mining cities. We systematically characterized the heavy metals (HMs) pollution, risks, sources, and influencing factors in the surrounding soils of Shuozhou. Specifically, 146 samples were collected, and the potential ecological risk index (RI) and the single-factor index were jointly used to understand the environmental risk of HMs. Meanwhile, correlation analysis was applied to find the influencing factors of HMs. The results of the soil pollution risk assessment in the entire area of Shuozhou were compared with those in the open-pit mine area. (1) The mean concentrations of Cr, As, Cd, Pb, and Hg in our study were found to be higher than the background value. The RI results indicated that most soil samples (82.88%) in Shuozhou had a low potential ecological risk. Compared with the Pingshuo open-pit mine (average RI value: 200.07), the potential ecological RI was lower. (2) The HM correlation indicated that Cr and As were associated with the parent rock, whereas Cd, together with Hg and Pb, were associated with anthropic activities. (3) There was no significant correlation between HM concentrations and farmland slope. Located in the Datong Basin, the terrain of Shuozhou is relatively flat and open and has little impact on the distribution of HMs. (4) Only Hg and Pb have a negative correlation with pH. This suggests that soil with a lower pH value may be beneficial to the accumulation of Hg and Pb in soil. (5) Among the eight industry types examined, the pollution capacity level of the leather, fur, feather, and footwear industries is the strongest, indicating that HMs around LI industry sites represent the maximum level among the eight types.
Soil acidification, caused by intensified fertilizer application and acid deposition, has threatened the sustainability of agricultural ecosystems and soil quality in parts of China since the 1980s. However, little is known about the spatio-temporal change of soil pH in cropland at a large basin scale. Poyang Lake Basin of China was selected as the study area to identify the spatio-temporal change of cropland pH and detect potential soil acidification factors. A total of 507 and 503 topsoil samples were collected in 2012 and 2018, respectively, and methods including one-way analysis of variance (ANOVA), Pearson’s correlation analyses, and Inverse Distance Weighted (IDW) were applied. Results showed that soil pH ranged from 3.96 to 7.95 in 2012 and from 3.34 to 8.19 in 2018, with most samples being acidic (pH < 7) in both sets of data. The two soil datasets showed a significant decline (p < 0.05) of 0.1 pH units over the past six years and several soil samples that exhibited obvious uptrends in the groups of pH < 4.5 and 4.5–5.0 from 2012 to 2018. Overall, the distribution patterns of pH at the two sampling dates were similar, whereas local details of the pH spatial distribution patterns differed. While we found a significant correlation (p < 0.05) between soil pH and aspect, elevation and slope showed no significant correlation with pH. ANOVA showed that pH values in the water density (river or lake network density) range of 6.27–19.94 were significantly higher (p < 0.05) than the other water densities. Large amounts of precipitation with low pH values were found to significantly influence soil pH, whereas N-fertilizer inputs exerted limited effects on soil pH over the entire study area. These findings provided new insights on soil acidification assessment and potential factor detection at the basin scale.
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