We study photoionization of argon atoms excited by attosecond pulses using an interferometric measurement technique. We measure the difference in time delays between electrons emitted from the 3s(2) and from the 3p(6) shell, at different excitation energies ranging from 32 to 42 eV. The determination of photoemission time delays requires taking into account the measurement process, involving the interaction with a probing infrared field. This contribution can be estimated using a universal formula and is found to account for a substantial fraction of the measured delay.

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition amplitudes and to make the connection with the time-delays that have been recently measured in experiments. We find that the overall phase contains two distinct types of contributions: one is expressed in terms of the phase-shifts of the photoelectron continuum wavefunction while the other is linked to continuum-continuum transitions induced by the infrared (IR) laser probe. Our formalism applies to both kinds of measurements reported so far, namely the ones using attosecond pulse trains of XUV harmonics and the others based on the use of isolated attosecond pulses (streaking). The connection between the phases and the time-delays is established with the help of finite difference approximations to the energy derivatives of the phases. The observed time-delay is a sum of two components: a one-photon Wigner-like delay and an universal delay that originates from the probing process itself.

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We present experimental measurements and theoretical calculations of photoionization time delays from the 3s and 3p shells in Ar in the photon energy range of 32-42 eV. The experimental measurements are performed by interferometry using attosecond pulse trains and the infrared laser used for their generation. The theoretical approach includes intershell correlation effects between the 3s and 3p shells within the framework of the random phase approximation with exchange (RPAE). The connection between single-photon ionization and the two-color two-photon ionization process used in the measurement is established using the recently developed asymptotic approximation for the complex transition amplitudes of laser-assisted photoionization. We compare and discuss the theoretical and experimental results especially in the region where strong intershell correlations in the 3s → kp channel lead to an induced "Cooper" minimum in the 3s ionization cross-section.

Laser-plasma acceleration [1,2] is an emerging technique for accelerating electrons to high energies over very short distances. The accelerated electron bunches have femtosecond duration [3,4], making them particularly relevant for applications such as ultrafast imaging [5] or femtosecond X-ray generation [6,7]. Current laser-plasma accelerators are typically driven by Joule-class laser systems that have two main drawbacks: their relatively large scale and their low repetition-rate, with a few shots per second at best. The accelerated electron beams have energies ranging from 100 MeV [8][9][10] to multi-GeV [11,12], however a MeV electron source would be more suited to many societal and scientific applications. Here, we demonstrate a compact and reliable laserplasma accelerator producing high-quality few-MeV electron beams at kilohertz repetition rate.This breakthrough was made possible by using near-single-cycle light pulses, which lowered the required laser energy for driving the accelerator by three orders of magnitude, thus enabling high repetition-rate operation and dramatic downsizing of the laser system. The measured electron bunches are collimated, with an energy distribution that peaks at 5 MeV and contains up to 1 pC of charge. Numerical simulations reproduce all experimental features and indicate that the electron bunches are only ∼ 1 fs long. We anticipate that the advent of these kHz femtosecond relativistic electron sources will pave the way to wide-impact applications, such as ultrafast electron diffraction in materials [13,14] In a laser-plasma accelerator, a laser pulse is focused to ultra-high intensity in an underdense plasma. The laser ponderomotive force sets up a charge separation in the plasma by displacing electrons, resulting in the excitation of a large-amplitude plasma wave, also called a wakefield. The wakefield carries enormous electric fields, in excess of 100 GV/m [16], that are well adapted for accelerating electrons to relativistic energies over short distances, typically less than a millimeter. The accelerated electron beams have femtosecond duration and are intrinsically synchronized to the laser pulse, which could lift the temporal resolution bottleneck in various experimental situations. For example, in ultrafast electron diffraction, the temporal resolution is currently limited to more than 100 fs, but it could be improved to sub-10 fs using laser driven electrons [15]. Thus, laser-plasma accelerators in the MeV range could find numerous applications with unprecedented time resolution, provided they operate reliably and at high repetition-rate. Indeed, in addition to temporal resolution, ultrafast imaging and diffraction also require statistics and a high signal-to-noise ratio [5,14] that can only be reached with a reliable and high repetition-rate electron source.In this letter, we demonstrate reliable operation of a laser-plasma accelerator delivering 5 MeV electrons at kHz repetition-rate. This breakthrough was made possible by the original use of a multi-mJ lase...

Electron dynamics induced by resonant absorption of light is of fundamental importance in nature and has been the subject of countless studies in many scientific areas. Above the ionization threshold of atomic or molecular systems, the presence of discrete states leads to autoionization, which is an interference between two quantum paths: direct ionization and excitation of the discrete state coupled to the continuum. Traditionally studied with synchrotron radiation, the probability for autoionization exhibits a universal Fano intensity profile as a function of excitation energy. However, without additional phase information, the full temporal dynamics cannot be recovered. Here we use tunable attosecond pulses combined with weak infrared radiation in an interferometric setup to measure not only the intensity but also the phase variation of the photoionization amplitude across an autoionization resonance in argon. The phase variation can be used as a fingerprint of the interactions between the discrete state and the ionization continua, indicating a new route towards monitoring electron correlations in time.

We determine relative photoemission time delays between valence electrons in different noble gas atoms (Ar, Ne and He) in an energy range between 31 and 37 eV. The atoms are ionized by an attosecond pulse train synchronized with an infrared laser field and the delays are measured using an interferometric technique. We compare our results with calculations using the random phase approximation with exchange and multi-configurational Hartree-Fock. We also investigate the influence of the different ionization angular channels.

We report on recent progress on laser-plasma acceleration using a low energy and high-repetition rate laser system. Using only few milliJoule laser energy, in conjunction with extremely short pulses composed of a single optical cycle, we demonstrate that the laser-plasma accelerator (LPA) can be operated close to the resonant blowout regime. This results in the production of high charge electron beams (>10 pC) with peaked energy distributions in the few MeV range and relatively narrow divergence angles. We highlight the importance of the plasma density profile and gas jet design for the performance of the LPA. In this extreme regime of relativistic laser-plasma interaction with near-single-cycle laser pulses, we find that the effect of group velocity dispersion and carrier envelope phase can no longer be neglected. These advances bring LPAs closer to real scientific applications in ultrafast probing.