Magnetic skyrmions are nanoscale windings of the spin configuration that hold great promise for technology due to their topology-related properties and extremely reduced sizes. After the recent observation at room temperature of sub-100 nm skyrmions stabilized by interfacial chiral interaction in magnetic multilayers, several pending questions remain to be solved, notably about the means to nucleate individual compact skyrmions or the exact nature of their motion. In this study, a method leading to the formation of magnetic skyrmions in a micrometer-sized track using homogeneous current injection is evidenced. Spin-transfer-induced motion of these small electrical-current-generated skyrmions is then demonstrated and the role of the out-of-plane magnetic field in the stabilization of the moving skyrmions is also analyzed. The results of these experimental observations of spin torque induced motion are compared to micromagnetic simulations reproducing a granular type, nonuniform magnetic multilayer in order to address the particularly important role of the magnetic inhomogeneities on the current-induced motion of sub-100 nm skyrmions for which the material grains size is comparable to the skyrmion diameter.
Competition between magnetic interactions in multilayers stabilizes complex, vertically twisted topological spin textures.
Room-temperature skyrmions in ferromagnetic films and multilayers show promise for encoding information bits in new computing technologies. Despite recent progress, ferromagnetic order generates dipolar fields that prevent ultrasmall skyrmion sizes, and allows a transverse deflection of moving skyrmions that hinders their efficient manipulation. Antiferromagnetic skyrmions shall lift these limitations. Here we demonstrate that room-temperature antiferromagnetic skyrmions can be stabilized in synthetic antiferromagnets (SAFs), in which perpendicular magnetic anisotropy (PMA), antiferromagnetic coupling and chiral order can be adjusted concurrently. Utilizing interlayer electronic coupling to an adjacent bias layer (BL), we demonstrate that spin-spiral states obtained in a SAF with vanishing PMA can be turned into isolated antiferromagnetic skyrmions. We also provide model-based estimates of skyrmion size and stability, showing that room-temperature antiferromagnetic skyrmions below 10 nm in radius can be anticipated in further optimized SAFs. Antiferromagnetic skyrmions in SAFs may thus solve major issues associated with ferromagnetic skyrmions for low-power spintronic devices.
Magnetic skyrmions are topologically protected whirling spin textures that can be stabilized in magnetic materials by an asymmetric exchange interaction between neighbouring spins that imposes a fixed chirality. Their small size, together with the robustness against external perturbations, make magnetic skyrmions potential storage bits in a novel generation of memory and logic devices. To this aim, their contribution to the electrical transport properties of a device must be characterized-however, the existing demonstrations are limited to low temperatures and mainly in magnetic materials with a B20 crystal structure. Here we combine concomitant magnetic force microscopy and Hall resistivity measurements to demonstrate the electrical detection of sub-100 nm skyrmions in a multilayered thin film at room temperature. Furthermore, we detect and analyse the Hall signal of a single skyrmion, which indicates that it arises from the anomalous Hall effect with a negligible contribution from the topological Hall effect.
Using state-of-the-art, aberration-corrected scanning transmission electron microscopy and electron energy loss spectroscopy with atomic-scale spatial resolution, experimental evidence for an intrinsic electronic reconstruction at the LAO/STO interface is shown. Simultaneous measurements of interfacial electron density and system polarization are crucial for establishing the highly debated origin of the 2D electron gas.
We show that the growth of the heterostructure LaGaO 3 / SrTiO 3 yields the formation of a highly conductive interface. Our samples were carefully analyzed by high resolution electron microscopy, in order to assess their crystal perfection and to evaluate the abruptness of the interface. Their carrier density and sheet resistance are compared to the case of LaAlO 3 / SrTiO 3 and a superconducting transition is found. The results open the route to widening the field of polar-nonpolar interfaces, pose some phenomenological constrains to their underlying physics and highlight the chance of tailoring their properties for future applications by adopting suitable polar materials.The quasi-two-dimensional electron gas ͑q2DEG͒ recently discovered at the LaAlO 3 ͑LAO͒ / SrTiO 3 ͑STO͒ interface 1 is presently envisaged as an ideal system for the realization of nanoscale oxide devices. 2 The electronic reconstruction model attributes the origin of the q2DEG to an electronic relaxation mechanism occurring at the interface between the ͑nominally͒ non-polar ͑001͒ STO substrate and the polar ͑001͒ LAO film. The wide band gap of LAO is considered as crucial in this approach, because it determines the capability of the polar film to transfer charges over the band gap of STO. Ideally, half an electron per areal unit cell ͑Ϸ3.3ϫ 10 14 cm −2 ͒ is expected to be transferred at the TiO 2 -LaO interface, partially filling the 3d Ti levels of the STO conduction band ͑CB͒. Alternatively, a possible active role of oxygen vacancies in STO near the interface was envisaged. 3 Actually, the transport properties of the heterostructure are affected both by oxygen pressure during growth 4,5 and by the application of an oxygen postanneal. 5 Finally, it was argued that a substantial La substitution for Sr during sample growth might drive the insulating surface of STO into a conductor. [6][7][8] Obviously, also LAO poses material issues. 9 In this context, we started the search of novel heterostructures based on a different overlayer. On this basis, we identified as a first test material LaGaO 3 ͑LGO͒, a polar, wide band gap, pseudocubic perovskite.Films of LAO and LGO were deposited on nominally TiO 2 terminated STO substrates, chemically treated in deionized water and buffered-HF. 10,11 The growth was performed by reflection high energy electron diffraction ͑RHEED͒ as-sisted pulsed laser deposition ͑KrF excimer laser, 248 nm͒ with a typical fluence of Ϸ1.5-2.5 J cm −2 at the target, a substrate temperature of 800°C and different oxygen pressures within the 10 −2 -10 −4 mbar range. 12 LAO films presented regular RHEED oscillations typical of layer-by-layer growth and a final pattern reminiscent of a single crystal surface, whereas LGO films showed damped and less regular oscillations, and a streaky 2D pattern at the end of the growth ͑Fig. 1͒.The atomic and electronic structures of LAO/STO and LGO/STO interfaces were investigated by high-resolution scanning transmission electron microscopy ͑STEM͒ and electron energy loss spectroscopy ͑EELS͒ measur...
The pulsed laser deposition of SrTiO3/LaGaO3 and SrTiO3/LaAlO3 interfaces is analyzed with a focus on the kinetic energy of the ablated species. LaGaO3 and LaAlO3 plasma plumes were studied by fast photography and space-resolved optical emission spectroscopy. Reflection high energy electron diffraction was performed proving a layer-by-layer growth up to 10−1 mbar oxygen pressure. The role of the energetic plasma plume on the two-dimensional growth and on the presence of interfacial defects at different oxygen growth pressures is discussed in connection with the conducting properties of the polar/nonpolar interfaces.
A site-dependent charge transfer to 7,7′,8,8′-tetracyanoquinodimethane (TCNQ) adsorbed on a single layer of periodically rippled graphene grown epitaxially on Ru(0001), identified by X-ray photoemission techniques, can be spatially resolved using Scanning Tunneling Microscopy, which can also detect the formation of magnetic moments. The molecules adsorbed on the lower part of the ripples are charged with electrons donated from the doped graphene overlayer and develop a magnetic moment, while those at the upper part of the ripples are neutral. On the other hand, TCNQ adsorbed on graphene on Ir(111) shows negligible charge transfer and no magnetic moment. These observations explain the spatially dependent longrange magnetic order observed recently for TCNQ on gr/Ru(0001).
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