Intense heating by wildfires can generate deep, smoke-infused thunderstorms, known as pyrocumulonimbus (pyroCb), which can release a large quantity of smoke particles above jet aircraft cruising altitudes. Injections of pyroCb smoke into the lower stratosphere have gained increasing attention over the past 15 years due to the rapid proliferation of satellite remote sensing tools. Impacts from volcanic eruptions and other troposphere-to-stratosphere exchange processes on stratospheric radiative and chemical equilibrium are well recognized and monitored. However, the role of pyroCb smoke in the climate system has yet to be acknowledged. Here, we show that the mass of smoke aerosol particles injected into the lower stratosphere from five near-simultaneous intense pyroCbs occurring in western North America on 12 August 2017 was comparable to that of a moderate volcanic eruption, and an order of magnitude larger than previous benchmarks for extreme pyroCb activity. The resulting stratospheric plume encircled the Northern Hemisphere over several months. By characterizing this event, we conclude that pyroCb activity, considered as either large singular events, or a full fire season inventory, significantly perturb the lower stratosphere in a manner comparable with infrequent volcanic intrusions.

In 2017, western Canadian wildfires injected smoke into the stratosphere that was detectable by satellites for more than 8 months. The smoke plume rose from 12 to 23 kilometers within 2 months owing to solar heating of black carbon, extending the lifetime and latitudinal spread. Comparisons of model simulations to the rate of observed lofting indicate that 2% of the smoke mass was black carbon. The observed smoke lifetime in the stratosphere was 40% shorter than calculated with a standard model that does not consider photochemical loss of organic carbon. Photochemistry is represented by using an empirical ozone-organics reaction probability that matches the observed smoke decay. The observed rapid plume rise, latitudinal spread, and photochemical reactions provide new insights into potential global climate impacts from nuclear war.

The Black Summer fire season of 2019–2020 in southeastern Australia contributed to an intense ‘super outbreak’ of fire-induced and smoke-infused thunderstorms, known as pyrocumulonimbus (pyroCb). More than half of the 38 observed pyroCbs injected smoke particles directly into the stratosphere, producing two of the three largest smoke plumes observed at such altitudes to date. Over the course of 3 months, these plumes encircled a large swath of the Southern Hemisphere while continuing to rise, in a manner consistent with existing nuclear winter theory. We connect cause and effect of this event by quantifying the fire characteristics, fuel consumption, and meteorology contributing to the pyroCb spatiotemporal evolution. Emphasis is placed on the unusually long duration of sustained pyroCb activity and anomalous persistence during nighttime hours. The ensuing stratospheric smoke plumes are compared with plumes injected by significant volcanic eruptions over the last decade. As the second record-setting stratospheric pyroCb event in the last 4 years, the Australian super outbreak offers new clues on the potential scale and intensity of this increasingly extreme fire-weather phenomenon in a warming climate.

One of the largest wildfires in California's history provides a unique opportunity to examine the meteorology driving extreme fire behavior and its impact on smoke plume altitude and downwind transport.

The first observationally based conceptual model for intense pyrocumulonimbus (pyroCb) development is described by applying reanalyzed meteorological model output to an inventory of 26 intense pyroCb events from June to August 2013 and a control inventory of intense fire activity without pyroCb. Results are based on 88 intense wildfires observed within the western United States and Canada. While surface-based fire weather indices are a useful indicator of intense fire activity, they are not a skillful predictor of intense pyroCb. Development occurs when a layer of increased moisture content and instability is advected over a dry, deep, and unstable mixed layer, typically along the leading edge of an approaching disturbance or under the influence of a monsoonal anticyclone. Upper-tropospheric dynamics are conducive to rising motion and vertical convective development. Mid- and upper-tropospheric conditions therefore resemble those that produce traditional dry thunderstorms. The specific quantity of midlevel moisture and instability required is shown to be strongly dependent on the surface elevation of the contributing fire. Increased thermal buoyancy from large and intense wildfires can serve as a potential trigger, implying that pyroCb occasionally develop in the absence of traditional meteorological triggering mechanisms. This conceptual model suggests that meteorological conditions favorable for pyroCb are observed regularly in western North America. PyroCb and ensuing stratospheric smoke injection are therefore likely to be significant and endemic features of summer climate. Results from this study provide a major step toward improved detection, monitoring, and prediction of pyroCb, which will ultimately enable improved understanding of the role of this phenomenon in the climate system.

In an environment with many local, remote, persistent, and episodic sources of pollution, meteorology is the primary factor that drives periods of unhealthy air quality and reduced visibility. The 2016 Korea-UnitedStatesAirQuality(KORUS-AQ)fieldstudyprovidesauniqueopportunitytoexaminethe impactofmeteorologyontherelativeinfluenceoflocalandtransboundarypollution.MuchoftheKORUS-AQ campaign can be grouped into four distinct research periods based on observed synoptic meteorology, includingaperiodofcomplexaerosolverticalprofilesdrivenbydynamicmeteorology,stagnationundera persistent anticyclone, low-level transport and haze development, and a blocking pattern. These episodes areexaminedusingadiversearchiveofground,airborne,andsatellitedata.Whilefrontalboundaries are recognized as the primary mechanism driving pollution transport in eastern Asia, results show that they are not always related to sustained periods of hazardous air quality and reduced visibility at the surface.Significantlong-rangetransportofpollutionanddustwasconstrainedtoafewshortevents, suggesting that the majority of pollutants sampled during KORUS-AQ originated from local sources. A severeregionalpollutionepisodeisexaminedindetail,featuringdensehazeandsignificantsecondary particle formation within a shallow moist boundary layer. Observations during KORUS-AQ also highlight a rapid,40ppbvincreaseinozonepollutionasastrongseabreezefronttraversedtheSeoulMetropolitan Area. Representativeness of meteorology and pollution conditions measured by KORUS-AQ is considered by comparison with climatology. This analysis is an essential step toward improved local and regional forecasting of air quality and visibility.

We couple airborne, ground‐based, and satellite observations; conduct regional simulations; and develop and apply an inversion technique to constrain hourly smoke emissions from the Rim Fire, the third largest observed in California, USA. Emissions constrained with multiplatform data show notable nocturnal enhancements (sometimes over a factor of 20), correlate better with daily burned area data, and are a factor of 2–4 higher than a priori estimates, highlighting the need for improved characterization of diurnal profiles and day‐to‐day variability when modeling extreme fires. Constraining only with satellite data results in smaller enhancements mainly due to missing retrievals near the emissions source, suggesting that top‐down emission estimates for these events could be underestimated and a multiplatform approach is required to resolve them. Predictions driven by emissions constrained with multiplatform data present significant variations in downwind air quality and in aerosol feedback on meteorology, emphasizing the need for improved emissions estimates during exceptional events.

Smoke particles can be injected by pyrocumulonimbus (pyroCb) in the upper troposphere and lower stratosphere, but their effects on the radiative budget of the planet remain elusive. Here, by focusing on the record‐setting Pacific Northwest pyroCb event of August 2017, we show with satellite‐based estimates of pyroCb emissions and injection heights in a chemical transport model (GEOS‐Chem) that pyroCb smoke particles can result in radiative forcing of ∼0.02 W/m2 at the top of the atmosphere averaged globally in the 2 months following the event and up to 0.9 K/day heating in the Arctic upper troposphere and lower stratosphere. The modeled aerosol distributions agree with observations from satellites (Earth Polychromatic Imaging Camera [EPIC], Cloud‐Aerosol Transport System [CATS], and Cloud‐Aerosol Lidar with Orthogonal Polarization [CALIOP]), showing the hemispheric transport of pyroCb smoke aerosols with a lifetime of 5 months. Hence, warming by pyroCb aerosols can have similar temporal duration but opposite sign to the well‐documented cooling of volcanic aerosols and be significant for climate prediction.