[1] The Dutch-Finnish Ozone Monitoring Instrument (OMI) launched on the NASA Aura satellite in July 2004 offers unprecedented spatial resolution, coupled with contiguous daily global coverage, for space-based UV measurements of sulfur dioxide (SO 2 ). We present a first validation of the OMI SO 2 data with in situ aircraft measurements in NE China in April 2005. The study demonstrates that OMI can distinguish between background SO 2 conditions and heavy pollution on a daily basis. The noise (expressed as the standard deviation, s) is $1.5 DU (Dobson units; 1 DU = 2.69 Á 10 16 molecules/cm 2 ) for instantaneous field of view boundary layer (PBL) SO 2 data. Temporal and spatial averaging can reduce the noise to s $ 0.3 DU over a remote region of the South Pacific; the long-term average over this remote location was within 0.1 DU of zero. Under polluted conditions collection 2 OMI data are higher than aircraft measurements by a factor of two. Improved calibrations of the radiance and irradiance data (collection 3) result in better agreement with aircraft measurements on polluted days. The air mass-corrected collection 3 data still show positive bias and sensitivity to UV absorbing aerosols. The difference between the in situ data and the OMI SO 2 measurements within 30 km of the aircraft profiles was about 1 DU, equivalent to $5 ppb from 0 to 3000 m altitude. Quantifying the SO 2 and aerosol profiles and spectral dependence of aerosol absorption between 310 and 330 nm are critical for an accurate estimate of SO 2 from satellite UV measurements.
a b s t r a c tChina's urbanization has been a notable global event. The National New Urbanization Plan (2014)(2015)(2016)(2017)(2018)(2019)(2020) unveiled by the Chinese Central Government revealed a new path for urbanization that accommodated unique Chinese characteristics. The most notable aspect was the transfer from land-centered urbanization to people-oriented urbanization. Given that land urbanization was the key to the previous orbit, this manuscript aims to analyze the evolution and challenge for land-centered urbanization, and way forward for people-oriented urbanization in China. With increasing urban populations and expanding industrial activities, China has experienced vigorous land urbanization and an uneven population distribution pattern since 1978. Land-centered urbanization has created some economic and social benefits, but has also posed many adverse impacts. The issues of the loss of arable land, the phenomenon of "ghost cities," and the urban heat island effect have become critical challenges. Eight suggestions from two perspectives are recommended in this manuscript for achieving new-type urbanization in China. We should give priority to this issue of the citizenization of peasant migrants. Government, scientists, and the public can all combine to influence the development trajectories of China's new-type urbanization.
[1] Papers published in this special section report findings from the East Asian Study of Tropospheric Aerosols: An International Regional Experiment (EAST-AIRE). They are concerned with (1) the temporal and spatial distributions of aerosol loading and precursor gases, (2) aerosol single scattering albedo (SSA), (3) aerosol direct radiative effects, (4) validation of satellite products, (5) transport mechanisms, and (6) the effects of air pollution on ecosystems. Aerosol loading is heaviest in mideastern China with a mean aerosol optical depth (AOD) of 0.5 and increasing to 0.7 around major cities that reduced daily mean surface solar radiation by $30-40 W m À2 , but barely changed solar reflection at the top of the atmosphere. Aerosol loading, particle size and composition vary considerably with location and season. The MODIS AOD data from Collection 5 (C5) agree much better with ground data than earlier releases, but considerable discrepancies still exist because of treatments of aerosol SSA and surface albedo. Four methods are proposed/adopted to derive the SSA by means of remote sensing and in situ observation, which varies drastically with time and space. The nationwide means of AOD, Å ngström exponent, and SSA (0.5 mm) in China are 0.69 ± 0.17, 1.06 ± 0.26, and 0.89 ± 0.04, respectively. Measurements of trace gases reveal substantial uncertainties in emission inventories. An analysis of aircraft measurements revealed that dry convection is an important mechanism uplifting pollutants over northern China. Model simulations of nitrogen deposition and impact of ozone pollution on net primary productivity indicate an increasing threat of air pollution on the ecosystem.
The Asian summer monsoon (ASM) anticyclone circulation system is recognized to be a significant transport pathway for water vapor and pollutants to enter the stratosphere. The observational evidence, however, is largely based on satellite retrievals. We report the first coincident in situ measurements of water vapor and ozone within the ASM anticyclone. The combined water vapor and ozonesondes were launched from Kunming, China in August 2009 and Lhasa, China in August 2010. In total, 11 and 12 sondes were launched in Kunming and Lhasa, respectively. We present the key characteristics of these measurements, and provide a comparison to similar measurements from an equatorial tropical location, during the Tropical Composition, Cloud and Climate Coupling (TC4) campaign in July and August of 2007. Results show that the ASM anticyclone region has higher water vapor and lower ozone concentrations in the upper troposphere and lower stratosphere than the TC4 observations. The results also show that the cold point tropopause in the ASM region has a higher average height and potential temperature. The in situ observations therefore support the satellite‐based conclusion that the ASM is an effective transport pathway for water vapor to enter stratosphere.
Diurnal and seasonal variation, intensity, and structure of deep convective systems (DCSs; with 20-dBZ echo tops exceeding 14 km) over the Tibetan Plateau–South Asian monsoon region from the Tibetan Plateau (TP) to the ocean are investigated using 14 yr of Tropical Rainfall Measuring Mission (TRMM) data. Four unique regions characterized by different orography are selected for comparison, including the TP, the southern Himalayan front (SHF), the South Asian subcontinent (SAS), and the ocean. DCSs and intense DCSs (IDCSs; with 40-dBZ echo tops exceeding 10 km) occur more frequently over the continent than over the ocean. About 23% of total DCSs develop into IDCSs in the SHF, followed by the TP (21%) and the SAS (15%), with the least over the ocean (2%). The average 20-dBZ echo-top height of IDCSs exceeds 16 km and 9% of them even exceed 18 km. DCSs and IDCSs are the most frequent over the SHF, especially in the westernmost SHF, where the intensity—in terms of strong radar echo-top (viz., 40 dBZ) height, ice-particle content, and lightning flash rate—is the strongest. DCSs over the TP are relatively weak in convective intensity and small in size but occur frequently. Oceanic DCSs possess the tallest cloud top (which mainly reflects small ice particles) and the largest size, but their convective intensity is markedly weaker. DCSs and IDCSs show a similar diurnal variation, mainly occurring in the afternoon with a peak at 1600 local time over land. Although most of both DCSs and IDCSs occur between April and October, DCSs have a peak in August, whereas IDCSs have a peak in May.
Abstract. Using a combination of ozonesonde data and numerical simulations of the Chemical Lagrangian Model of the Stratosphere (CLaMS), the trend of tropospheric ozone (O 3 ) during 2002-2010 over Beijing was investigated. Tropospheric ozone over Beijing shows a winter minimum and a broad summer maximum with a clear positive trend in the maximum summer ozone concentration over the last decade. The observed significant trend of tropospheric column ozone is mainly caused by photochemical production (3.1 % yr −1 for a mean level of 52 DU). This trend is close to the significant trend of partial column ozone in the lower troposphere (0-3 km) resulting from the enhanced photochemical production during summer (3.0 % yr −1 for a mean level of 23 DU). Analysis of the CLaMS simulation shows that transport rather than chemistry drives most of the seasonality of tropospheric ozone. However, dynamical processes alone cannot explain the trend of tropospheric ozone in the observational data. Clearly enhanced ozone values and a negative vertical ozone gradient in the lower troposphere in the observational data emphasize the importance of photochemistry within the troposphere during spring and summer, and suggest that the photochemistry within the troposphere significantly contributes to the tropospheric ozone trend over Beijing during the last decade.
Satellite precipitation products provide alternative precipitation data in mountain areas. This study aimed to assess the performance of the latest Global Precipitation Measurement (GPM) Integrated Multi-satellite Retrievals for GPM (IMERG) version 5 (IMERG V5) and Global Satellite Mapping of Precipitation version 7 (GSMaP V7) products and their hydrological utilities over the Tibetan Plateau (TP). Here, two IMERG Final Run products (uncalibrated IMERG (IMERG-UC) and gauge-calibrated IMERG (IMEEG-C)) and two GSMaP products (GSMaP Moving Vector with Kalman Filter (GSMaP-MVK) and gauge-adjusted GSMaP (GSMaP-Gauge)) were evaluated from April 2014 to March 2017. Results show that all four satellite precipitation products could generally capture the spatial patterns of precipitation over the TP. The two gauge-adjusted products were more consistent with the ground measurements than the satellite-only products in terms of statistical assessment. For hydrological simulation, IMERG-UC and GSMaP-MVK showed unsatisfactory performance for hydrological utility, while GSMaP-Gauge demonstrated comparable performance with gauge reference data, suggesting that GSMaP-Gauge can be selected for hydrological application in the TP. Our study also indicates that accurately measuring light rainfall and winter snow is still a challenging task for the current satellite precipitation retrievals.
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