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The Linac Coherent Light Source (LCLS) is an x-ray Free-Electron Laser (FEL) project presently in a commissioning phase at SLAC. We report here on very low emittance measurements made at low bunch charge, and a few femtosecond bunch length produced by the LCLS bunch compressors. Start-to-end simulations associated with these beam parameters show the possibilities of generating hundreds of GW at 1.5Å x-ray wavelength and nearly a single longitudinally spike at 1.5 nm with 2-fs duration.

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The X-ray free-electron laser has opened a new era for photon science, improving the X-ray brightness by ten orders of magnitude over previously available sources. Similar to an optical laser, the spectral and temporal structure of the radiation pulses can be tailored to the specific needs of many experiments by accurately manipulating the lasing medium, that is, the electron beam. Here we report the generation of mJ-level two-colour hard X-ray pulses of few femtoseconds duration with an XFEL driven by twin electron bunches at the Linac Coherent Light Source. This performance represents an improvement of over an order of magnitude in peak power over state-of-the-art two-colour XFELs. The unprecedented intensity and temporal coherence of this new two-colour X-ray free-electron laser enable an entirely new set of scientific applications, ranging from X-ray pump/X-ray probe experiments to the imaging of complex biological samples with multiple wavelength anomalous dispersion.

The ultrafast evolution of microstructure is key to understanding high-pressure and strain-rate phenomena. However, the visualization of lattice dynamics at scales commensurate with those of atomistic simulations has been challenging. Here, we report femtosecond x-ray diffraction measurements unveiling the response of copper to laser shock-compression at peak normal elastic stresses of ~73 gigapascals (GPa) and strain rates of 10(9) per second. We capture the evolution of the lattice from a one-dimensional (1D) elastic to a 3D plastically relaxed state within a few tens of picoseconds, after reaching shear stresses of 18 GPa. Our in situ high-precision measurement of material strength at spatial (<1 micrometer) and temporal (<50 picoseconds) scales provides a direct comparison with multimillion-atom molecular dynamics simulations.

The very bright electron beam required for an x-ray free-electron laser (FEL), such as the linac coherent light source (LCLS), is susceptible to a microbunching instability in the magnetic bunch compressors, prior to the FEL undulator. The uncorrelated electron energy spread in the LCLS can be increased by an order of magnitude to provide strong Landau damping against the instability without degrading the FEL performance. To this end, a ''laser-heater'' system has been installed in the LCLS injector, which modulates the energy of a 135-MeV electron bunch with an IR-laser beam in a short undulator, enclosed within a four-dipole chicane. In this paper, we report detailed measurements of laser-heater-induced energy spread, including the unexpected self-heating phenomenon when the laser energy is very low. We discuss the suppression of the microbunching instability with the laser heater and its impact on the x-ray FEL performance. We also present the analysis of these experimental results and develop a threedimensional longitudinal space charge model to explain the self-heating effect.