It has long been predicted that the scattering of ultracold atoms can be altered significantly through a so-called 'Feshbach resonance'. Two such resonances have now been observed in optically trapped Bose-Einstein condensates of sodium atoms by varying an external magnetic field. They gave rise to enhanced inelastic processes and a dispersive variation of the scattering length by a factor of over ten. These resonances open new possibilities for the study and manipulation of Bose-Einstein condensates.Bose-Einstein condensates of atomic gases offer new opportunities for studying quantum-degenerate fluids 1-5 . All the essential properties of Bose condensed systems-the formation and shape of the condensate, the nature of its collective excitations and statistical fluctuations, and the formation and dynamics of solitons and vortices-are determined by the strength of the atomic interactions. In contrast to the situation for superfluid helium, these interactions are weak, allowing the phenomena to be theoretically described from 'first principles'. Furthermore, in atomic gases the interactions can be altered, for instance by employing different species, changing the atomic density, or, as in the present work, merely by varying a magnetic field.At low temperatures, the interaction energy in a cloud of atoms is proportional to the density and a single atomic parameter, the scattering length a which depends on the quantum-mechanical phase shift in an elastic collision. It has been predicted that the scattering length can be modified by applying external magnetic 6-10 , optical 11,12 or radio-frequency 13 (r.f.) fields. Those modifications are only pronounced in a so-called ''Feshbach resonance'' 14 , when a quasibound molecular state has nearly zero energy and couples resonantly to the free state of the colliding atoms. In a timedependent picture, the two atoms are transferred to the quasibound state, 'stick' together and then return to an unbound state. Such a resonance strongly affects the scattering length (elastic channel), but also affects inelastic processes such as dipolar relaxation 6,7 and threebody recombination. Feshbach resonances have so far been studied at much higher energies 15 by varying the collision energy, but here we show that they can be 'tuned' to zero energy to be resonant for ultracold atoms. The different magnetic moments of the free and quasibound states allowed us to tune these resonances with magnetic fields, and as a result, minute changes in the magnetic field strongly affected the properties of a macroscopic system.Above and below a Feshbach resonance, the scattering length a covers the full continuum of positive and negative values. This should allow the realization of condensates over a wide range of interaction strengths. By setting a Ϸ 0, one can create a condensate with essentially non-interacting atoms, and by setting a Ͻ 0 one can make the system unstable and observe its collapse. Rapid tuning of an external magnetic field around a Feshbach resonance will lead to sudden changes of t...
Bose-Einstein condensates of dilute atomic gases, characterized by a macroscopic population of the quantum mechanical ground state, are a new, weakly interacting quantum fluid [1,2,3]. In most experiments condensates in a single weak field seeking state are magnetically trapped. These condensates can be described by a scalar order parameter similar to the spinless superfluid 4 He. Even though alkali atoms have angular momentum, the spin orientation is not a degree of freedom because spin flips lead to untrapped states and are therefore a loss process. In contrast, the recently realized optical trap for sodium condensates [4] confines atoms independently of their spin orientation. This opens the possibility to study spinor condensates which represent a system with a vector order parameter instead of a scalar. Here we report a study of the equilibrium state of spinor condensates in an optical trap. The freedom of spin orientation leads to the formation of spin domains in an external magnetic field. The structure of these domains are illustrated in spin domain diagrams. Combinations of both miscible and immiscible spin components were realized.A variety of new phenomena is predicted [5,6,7] for spinor condensates, such as spin textures, propagation of spin waves and coupling between superfluid flow and atomic spin. To date such effects could only be studied in superfluid 3 He, which can be described by Bose-Einstein condensation of Cooper pairs of quasi particles having both spin and orbital angular momentum [8]. Compared to the strongly interacting 3 He, the properties of weakly interacting BoseEinstein condensates of alkali gases can be calculated by mean field theories in a much more straightforward and simple way.Other systems which go beyond the description with a single scalar order parameter are condensates of two different hyperfine states of 87 Rb confined in magnetic traps. Recent experimental studies have explored the spatial separation of the two components [9,10] and their relative phase [11]. Several theoretical papers describe their structure [12,13,14,15,16,17,18] and their collective excitations [19,20,21,22].Compared to these two-component condensates, spinor condensates have several new features including the vector character of the order parameter and the changed role of spin relaxation collisions which allow for population exchange among hyperfine states without trap loss. In contrast, for 87 Rb experiments trap loss due to spin relaxation severely limits the lifetime.We consider an F = 1 spinor condensate subject to spin relaxation, in which two m F = 0 atoms can collide and produce an m F = +1 and an m F = −1 atom and vice versa. We investigate the distribution of hyperfine states and the spatial distribution in equilibrium assuming conservation of the total spin. The ground state spinor wave function is found by minimizing the free energy [5]where kinetic energy terms are neglected in the ThomasFermi approximation which is valid as long as the dimension of spin domains (typically 50 µm) is ...
A central goal in condensed matter and modern atomic physics is the exploration of manybody quantum phases and the universal characteristics of quantum phase transitions in so far as they differ from those established for thermal phase transitions. Compared with condensedmatter systems, atomic gases are more precisely constructed and also provide the unique opportunity to explore quantum dynamics far from equilibrium. Here we identify a second-order quantum phase transition in a gaseous spinor BoseEinstein condensate, a quantum fluid in which superfluidity and magnetism, both associated with symmetry breaking, are simultaneously realized. 87 Rb spinor condensates were rapidly quenched across this transition to a ferromagnetic state and probed using in-situ magnetization imaging to observe spontaneous symmetry breaking through the formation of spin textures, ferromagnetic domains and domain walls. The observation of topological defects produced by this symmetry breaking, identified as polar-core spin-vortices containing non-zero spin current but no net mass current, represents the first phase-sensitive in-situ detection of vortices in a gaseous superfluid.Most ultracold atomic gases consist of atoms with nonzero total angular momentum denoted by the quantum number F , which is the sum of the total electronic angular momentum and nuclear spin. In spinor atomic gases, such as F = 1 and F = 2 gases of 23 Na [1, 2] and 87 Rb [3,4], all magnetic sublevels representing all orientations of the atomic spin may be realized [5]. The phase coherent portion of a Bose-Einsein condensed spinor gas is described by a vector order parameter and therefore exhibits spontaneous magnetic ordering. Nevertheless, considerable freedom remains for the type of ordering that can occur. For 87 Rb F = 1 spinor gases, the spindependent energy per particle in the condensate is the sum of two terms, c 2 n F 2 + q F 2 z , where F denotes the dimensionless spin vector operator. The first term describes spin-dependent interatomic interactions, with n being the number density and c 2 = (4π 2 /3m)(a 2 − a 0 ) depending on the atomic mass m and the s-wave scattering lengths a f for collisions between pairs of particles with total spin f [6,7]. Given c 2 < 0 for our system [3,4,8,9], the interaction term alone favors a ferromagnetic phase with broken rotational symmetry. The second term describes a quadratic Zeeman shift in our experiment, with q = (h × 70 Hz/G 2 )B 2 at a magnetic field of magnitude B [10]. This term favors instead a scalar phase with no net magnetization, i.e. a condensate in the |m z = 0 magnetic sublevel. These phases are divided by a second-order quantum phase transition at q = 2|c 2 |n.This article describes our observation of spontaneous symmetry breaking in a 87 Rb spinor BEC that is rapidly quenched across this quantum phase transition. Nearlypure spinor Bose-Einstein condensates were prepared in the scalar |m z = 0 phase at a high quadratic Zeeman shift (q ≫ 2|c 2 |n). By rapidly reducing the magnitude of the applied magneti...
Spinor Bose gases form a family of quantum fluids manifesting both magnetic order and superfluidity. This article reviews experimental and theoretical progress in understanding the static and dynamic properties of these fluids. The connection between system properties and the rotational symmetry properties of the atomic states and their interactions are investigated. Following a review of the experimental techniques used for characterizing spinor gases, their mean-field and many-body ground states, both in isolation and under the application of symmetry-breaking external fields, are discussed. These states serve as the starting point for understanding low-energy dynamics, spin textures and topological defects, effects of magnetic dipole interactions, and various non-equilibrium collective spin-mixing phenomena. The paper aims to form connections and establish coherence among the vast range of works on spinor Bose gases, so as to point to open questions and future research opportunities. 42 B. Spin mixing instability 42 C. Quantum quench dynamics and the Kibble-Zurek mechanism 43 D. Parametric spin amplification 45 E. Quantum spin-nematicity squeezing 45
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