Abstract. Every year, from December to April, anthropogenic haze spreads over most of the North Indian Ocean, and South and Southeast Asia. The Indian Ocean Experiment (INDOEX) documented this Indo-Asian haze at scales ranging from individual particles to its contribution to the regional climate forcing. This study integrates the multiplatform observations (satellites, aircraft, ships, surface stations, and balloons) with one-and fourdimensional models to derive the regional aerosol forcing resulting from the direct, the semidirect and the two indirect effects. The haze particles consisted of several inorganic and carbonaceous species, including absorbing black carbon clusters, fly ash, and mineral dust. The most striking result was the large loading of aerosols over most of the South Asian region and the North Indian Ocean. The January to March 1999 visible optical depths were about 0.5 over most of the continent and reached values as large as 0.2 over the equatorial Indian ocean due to long-range transport. The aerosol layer extended as high as 3 km. Black carbon contributed about 14% to the fine particle mass and 11% to the visible optical depth. The single-scattering albedo estimated by several independent methods was consistently around 0.9 both inland and over the open ocean. Anthropogenic sources contributed as much as 80% (_+10%) to the aerosol loading and the optical depth. The in situ data, which clearly support the existence of the first indirect effect (increased aerosol concentration producing more cloud drops with smaller effective radii), are used to develop a composite indirect effect scheme. The Indo-Asian aerosols impact the radiative forcing through a complex set of heating (positive forcing) and cooling (negative forcing) processes. Clouds and black carbon emerge as the major players. The dominant factor, however, is the large negative forcing (-20 +_ 4 W m -t) at the surface and the comparably large atmospheric heating. Regionally, the absorbing haze decreased the surface solar radiation by an amount comparable to 50% of the total ocean heat flux and nearly doubled the lower tropospheric solar heating. We demonstrate with a general circulation model how this additional heating significantly perturbs the tropical rainfall patterns and the hydrological cycle with implications to global climate.

We report the detection of deuterium absorption at redshift 2.525659 toward Q1243+3047. We describe improved methods to estimate the deuterium to hydrogen abundance ratio (D/H) in absorption systems, including improved modeling of the continuum level, the Ly forest, and the velocity structure of the absorption. Together with improved relative flux calibration, these methods give D=H ¼ 2:42 À0:38 Â 10 À5 , from the log D/H-values toward five QSOs. The dispersion in the five values is larger than we expect from their individual measurement errors, and we suspect this is because some of these errors were underestimated. We observe a trend in D/H with log N H i that we also suspect is spurious. The best value for D/H is 0.6 smaller than we quoted in O'Meara et al. from three QSOs, and although we have more values, the error is similar because the dispersion is larger. In standard big bang nucleosynthesis (SBBN), the best D/H corresponds to a baryon-to-photon ratio ¼ 5:9 AE 0:5 Â 10 À10 and gives precise predictions for the primordial abundances of the other light nuclei. We predict more 4 He than is reported in most measurements, although not more than allowed by some estimates of the systematic errors. We predict a 3 He abundance very similar to that reported by Bania et al., and we predict 3-4 times more 7 Li than is seen in halo stars. It is unclear if those stars could have destroyed this much of their 7 Li. The -value from D/H corresponds to a cosmological baryon density b h 2 ¼ 0:0214 AE 0:0020 (AE9.3%), which agrees with the WMAP value of b h 2 ¼ 0:0224 AE 0:001.

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The warming of Arctic climate and decreases in sea ice thickness and extent observed over recent decades are believed to result from increased direct greenhouse gas forcing, changes in atmospheric dynamics having anthropogenic origin, and important positive reinforcements including ice-albedo and cloud-radiation feedbacks. The importance of cloud-radiation interactions is being investigated through advanced instrumentation deployed in the high Arctic since 1997 (refs 7, 8). These studies have established that clouds, via the dominance of longwave radiation, exert a net warming on the Arctic climate system throughout most of the year, except briefly during the summer. The Arctic region also experiences significant periodic influxes of anthropogenic aerosols, which originate from the industrial regions in lower latitudes. Here we use multisensor radiometric data to show that enhanced aerosol concentrations alter the microphysical properties of Arctic clouds, in a process known as the 'first indirect' effect. Under frequently occurring cloud types we find that this leads to an increase of an average 3.4 watts per square metre in the surface longwave fluxes. This is comparable to a warming effect from established greenhouse gases and implies that the observed longwave enhancement is climatologically significant.

We report the measurement of the primordial D/H abundance ratio towards QSO HS 0105+1619. The column density of the neutral hydrogen in the z ≃ 2.536 Lyman limit system is high, log N HI = 19.422 ± 0.009 cm −2 , allowing for the deuterium to be seen in 5 Lyman series transitions. The measured value of the D/H ratio towards QSO HS 0105+1619 is found to be D/H= 2.54 ± 0.23 × 10 −5 . The metallicity of the system showing D/H is found to be ≃ 0.01 solar, indicating that the measured D/H is the primordial D/H within the measurement errors. The gas which shows D/H is neutral, unlike previous D/H systems which were more highly ionized. Thus, the determination of the D/H ratio becomes more secure since we are measuring it in different astrophysical environments, but the error is larger because we now see more dispersion between measurements. Combined with prior measurements of D/H, the best D/H ratio is now D/H= 3.0 ± 0.4 × 10 −5 , which is 10% lower than the previous value. The new values for the baryon-to-photon ratio, and baryonic matter density derived from D/H are η = 5.6 ± 0.5 × 10 −10 and Ω b h 2 = 0.0205 ± 0.0018 respectively.

Over the past two decades the primary driver of mass loss from the West Antarctic Ice Sheet (WAIS) has been warm ocean water underneath coastal ice shelves, not a warmer atmosphere. Yet, surface melt occurs sporadically over low-lying areas of the WAIS and is not fully understood. Here we report on an episode of extensive and prolonged surface melting observed in the Ross Sea sector of the WAIS in January 2016. A comprehensive cloud and radiation experiment at the WAIS ice divide, downwind of the melt region, provided detailed insight into the physical processes at play during the event. The unusual extent and duration of the melting are linked to strong and sustained advection of warm marine air toward the area, likely favoured by the concurrent strong El Niño event. The increase in the number of extreme El Niño events projected for the twenty-first century could expose the WAIS to more frequent major melt events.

The Impact of Arctic Aerosols on Clouds During one flight leg over the water on 4 April, large chunks of ice were seen floating in the Arctic Ocean after breaking up from the ice sheet along the coastline near Barrow, Alaska. Photo by Alexei Korolev.

We use Keck/HIRES spectra of 37 optically bright quasars at z = 2-4 to study narrow absorption lines that are intrinsic to the quasars (intrinsic NALs, produced in gas that is physically associated with the quasar central engine). We identify 150 NAL systems, that contain 124 C IV, 12 N V, and 50 Si IV doublets, of which 18 are associated systems (within 5,000 km s −1 of the quasar redshift). We use partial coverage analysis to separate intrinsic NALs from NALs produced in cosmologically intervening structures. We find 39 candidate intrinsic systems, (28 reliable determinations and 11 that are possibly intrinsic). We estimate that 10-17% of C IV systems at blueshifts of 5,000-70,000 km s −1 relative to quasars are intrinsic. At least 32% of quasars contain one or more intrinsic C IV NALs. Considering N V and Si IV doublets showing partial coverage as well, at least 50% of quasars host intrinsic NALs. This result constrains the solid angle subtended by the absorbers to the background source(s). We identify two families of intrinsic NAL systems, those with strong N V absorption, and those with negligible absorption in N V, but with partial coverage in the C IV doublet. We discuss the idea that these two families represent different regions or conditions in accretion disk winds. Of the 26 intrinsic C IV NAL systems, 13 have detectable low-ionization absorption lines at similar velocities, suggesting that these are two-phase structures in the wind rather than absorbers in the host galaxy. We also compare possible models for quasar outflows, including radiatively accelerated disk-driven winds, magnetocentrifugally accelerated winds, and pressure-driven winds, and we discuss ways of distinguishing between these models observationally.