Carbonaceous aerosols (CA) emitted by fossil and biomass fuels consist of black carbon (BC), a strong absorber of solar radiation, and organic matter (OM). OM scatters as well as absorbs solar radiation. The absorbing component of OM, which is ignored in most climate models, is referred to as brown carbon (BrC). Model estimates of the global CA radiative forcing range from 0 to 0.7 Wm −2 , to be compared with the Intergovernmental Panel on Climate Change's estimate for the pre-Industrial to the present net radiative forcing of about 1.6 Wm −2 . This study provides a model-independent, observationally based estimate of the CA direct radiative forcing. Ground-based aerosol network data is integrated with field data and satellite-based aerosol observations to provide a decadal (2001 through 2009) global view of the CA optical properties and direct radiative forcing. The estimated global CA direct radiative effect is about 0.75 Wm −2 (0.5 to 1.0). This study identifies the global importance of BrC, which is shown to contribute about 20% to 550-nm CA solar absorption globally. Because of the inclusion of BrC, the net effect of OM is close to zero and the CA forcing is nearly equal to that of BC. The CA direct radiative forcing is estimated to be about 0.65 (0.5 to about 0.8) Wm −2 , thus comparable to or exceeding that by methane. Caused in part by BrC absorption, CAs have a net warming effect even over open biomass-burning regions in Africa and the Amazon.organic aerosol | global warming | environment B lack carbon (BC) and organic matter (OM) are emitted together by open biomass burning, indoor biomass combustion for cooking and heating, and fossil fuel combustion (1-3). In addition, OM is emitted both as primary aerosols and as volatile organic gases that are subsequently converted to the secondary organic aerosols. Most climate models treat OM as a scattering particle (4, 5). Based on this treatment, models estimate BC to be a climate-warming agent and OM to be a cooling agent. The combined climatic effect of BC and OM depends on the ratio of BC to OM. Biomass burning is known to emit a few times more primary OM over BC than fossil fuel combustion (2), and, as a result, models estimate a net warming over fossil fuel-dominated regions and indoor biomass-combustion regions, and a cooling-to-neutral forcing over open biomass-burning regions (6-10). Recent field studies (11, 12) have painted a different picture, revealing a substantially absorbing OM component-i.e., brown carbon (BrC) (13). BrC was found to be abundant in East Asian outflow (11) and biomass-burning regions (12,14,15). Although BrC and BC are both absorbing, BrC's absorption increases significantly towards shorter wavelengths from the visible to UV, relative to BC (11,12).We refer to BC þ OM as carbonaceous aerosol (CA) (see Table 1 for a summary of the acronyms used in this paper). The first measure for quantifying the climatic impact of aerosols is the change in the radiative flux at the TOA (top of atmosphere) by aerosols, denoted as the aerosol di...

Abstract. In this paper we describe SEAS5, ECMWF's fifth generation seasonal forecast system, which became operational in November 2017. Compared to its predecessor, System 4, SEAS5 is a substantially changed forecast system. It includes upgraded versions of the atmosphere and ocean models at higher resolutions, and adds a prognostic sea-ice model. Here, we describe the configuration of SEAS5 and summarise the most noticeable results from a set of diagnostics including biases, variability, teleconnections and forecast skill. An important improvement in SEAS5 is the reduction of the equatorial Pacific cold tongue bias, which is accompanied by a more realistic El Niño amplitude and an improvement in El Niño prediction skill over the central-west Pacific. Improvements in 2 m temperature skill are also clear over the tropical Pacific. Sea-surface temperature (SST) biases in the northern extratropics change due to increased ocean resolution, especially in regions associated with western boundary currents. The increased ocean resolution exposes a new problem in the northwest Atlantic, where SEAS5 fails to capture decadal variability of the North Atlantic subpolar gyre, resulting in a degradation of DJF 2 m temperature prediction skill in this region. The prognostic sea-ice model improves seasonal predictions of sea-ice cover, although some regions and seasons suffer from biases introduced by employing a fully dynamical model rather than the simple, empirical scheme used in System 4. There are also improvements in 2 m temperature skill in the vicinity of the Arctic sea-ice edge. Cold temperature biases in the troposphere improve, but increase at the tropopause. Biases in the extratropical jets are larger than in System 4: extratropical jets are too strong, and displaced northwards in JJA. In summary, development and added complexity since System 4 has ensured that SEAS5 is a state-of-the-art seasonal forecast system which continues to display a particular strength in the El Niño Southern Oscillation (ENSO) prediction.

Abstract. In this paper we describe SEAS5, ECMWF’s fifth generation seasonal forecast system, which became operational in November 2017. Compared to its predecessor, System 4, SEAS5 is a substantially changed forecast system. It includes upgraded versions of the atmosphere and ocean models at higher resolutions, and adds a prognostic sea ice model. Here, we describe the configuration of SEAS5 and summarise the most noticeable results from a set of diagnostics including biases, variability, teleconnections and forecast skill. An important improvement in SEAS5 is the reduction of the Equatorial Pacific cold tongue bias, which is accompanied by a more realistic ENSO amplitude and an improvement in ENSO prediction skill over the central-west Pacific. Improvements in two-metre temperature skill are also clear over the tropical Pacific. SST biases in the northern extratropics change due to increased ocean resolution, especially in regions associated with western boundary currents. The increased ocean resolution exposes a new problem in the northwest Atlantic, where SEAS5 fails to capture decadal variability of the North Atlantic subpolar gyre, resulting in a degradation of DJF two-metre temperature prediction skill in this region. The prognostic sea ice model improves seasonal predictions of sea ice cover, although some regions and seasons suffer from biases introduced by employing a fully dynamical model rather than the simple, empirical scheme used in System 4. There are also improvements in two-metre temperature skill in the vicinity of the Arctic sea-ice edge. Cold temperature biases in the troposphere improve, but increase at the tropopause. Biases in the extratropical jets are larger than in System 4: extratropical jets are too strong, and displaced northwards in summer. In summary, development and added complexity since System 4 has ensured SEAS5 is a state-of-the-art seasonal forecast system which continues to display a particular strength in ENSO prediction.

Atmospheric seasonal predictability in winter over the Euro-Atlantic region is studied with an emphasis on the signal-to-noise paradox of the North Atlantic Oscillation. Seasonal hindcasts of the ECMWF model for the recent period show, in agreement with other studies, that correlation skill over Greenland and parts of the Arctic is higher than the signal-to-noise ratio implies. This leads to the paradoxical situation where the real world appears more predictable than the models suggest, with the forecast ensembles being overly dispersive (or underconfident). However, it is demonstrated that these conclusions are not supported by the diagnosed relationship between ensemble mean root-mean-square error (RMSE) and ensemble spread which indicates a slight under-dispersion (overconfidence). Furthermore, long atmospheric seasonal hindcasts suggest that over the 110-year period from 1900 to 2009 the ensemble system is well calibrated (neither overnor under-dispersive). The observed skill changed drastically in the middle of the twentieth century and paradoxical regions during more recent hindcast periods were strongly under-dispersive during mid-century decades. Due to non-stationarities of the climate system in the form of decadal variability, relatively short hindcasts are not sufficiently representative of longer-term behaviour. In addition, small hindcast sample size can lead to skill estimates, in particular of correlation measures, that are not robust. It is shown that the relative uncertainty due to small hindcast sample size is often larger for correlation-based than for RMSE-based diagnostics. Correlation-based measures like the RPC are shown to be highly sensitive to the strength of the predictable signal, implying that disentangling of physical deficiencies in the models on the one hand, and the effects of sampling uncertainty on the other hand, is difficult. Given the current lack of a causal physical mechanism to unravel the puzzle, our hypotheses of non-stationarity and sampling uncertainty provide simple yet plausible explanations for the paradox.

Land surface initial conditions have been recognized as a potential source of predictability in sub-seasonal to seasonal forecast systems, at least for near-surface air temperature prediction over the mid-latitude continents. Yet, few studies have systematically explored such an influence over a sufficient hindcast period and in a multi-model framework to produce a robust quantitative assessment. Here, a dedicated set of twin experiments has been carried out with boreal summer retrospective forecasts over the 1992–2010 period performed by five different global coupled ocean–atmosphere models. The impact of a realistic versus climatological soil moisture initialization is assessed in two regions with high potential previously identified as hotspots of land–atmosphere coupling, namely the North American Great Plains and South-Eastern Europe. Over the latter region, temperature predictions show a significant improvement, especially over the Balkans. Forecast systems better simulate the warmest summers if they follow pronounced dry initial anomalies. It is hypothesized that models manage to capture a positive feedback between high temperature and low soil moisture content prone to dominate over other processes during the warmest summers in this region. Over the Great Plains, however, improving the soil moisture initialization does not lead to any robust gain of forecast quality for near-surface temperature. It is suggested that models biases prevent the forecast systems from making the most of the improved initial conditions. © 2017 Springer-Verlag Berlin Heidelber