Abstract. One year of meteorological and atmospheric radon observations in a topographically complex subalpine basin are used to identify persistent temperature inversion (PTI) events. PTI events play a key role in public health due to the accumulation of urban pollutants that they cause. Two techniques are compared: a new radon-based method (RBM), based on single-height 222Rn measurements from a single centrally located station, and an existing pseudo-vertical temperature gradient method (TGM) based on observations from eight weather stations around the subalpine basin. The RBM identified six PTI events (four in winter, two in autumn), a subset of the 17 events identified by the TGM. The RBM was more consistent in its identification of PTI events for all seasons and more selective of persistent strongly stable conditions. The comparatively poor performance of the TGM was attributed to seasonal inconsistencies in the validity of the method's key assumptions (influenced by mesoscale processes, such as local drainage flows, nocturnal jets, and intermittent turbulence influence) and a lack of snow cover in the basin for the 2016–2017 winter period. Corresponding meteorological quantities for RBM PTI events (constituting 27 % of the autumn–winter cold season) were well characterized. PTI wind speeds in the basin were consistently low over the whole diurnal cycle (typically 0.2–0.6 m s−1). Suitability of the two techniques for air quality assessment was compared using hourly PM10 observations. Peak PM10 concentrations for winter (autumn) PTI events were underestimated by 13 µg m−3 (11 µg m−3) by the TGM compared with the RBM. Only the RBM indicated that nocturnal hourly mean PM10 values in winter PTI events can exceed 100 µg m−3, the upper threshold of low-level short-term PM10 exposure according to World Health Organization guidelines. The efficacy, simplicity, and cost effectiveness of the RBM for identifying PTI events has the potential to make it a powerful tool for urban air quality management in complex terrain regions, for which it adds an additional dimension to contemporary atmospheric stability classification tools. Furthermore, the long-term consistency of the radon source function will enable the RBM to be used in the same way in future studies, enabling the relative magnitude of PTI events to be gauged, which is expected to assist with the assessment of public health risks.

Radon gas is the largest source of public exposure to naturally occurring radioactivity. However, radon is also a useful tracer for understanding atmospheric processes, assessing the accuracy of chemical transport models, and enabling integrated emissions estimates of greenhouse gases. A sound metrological system for low level atmospheric radon observations is therefore needed for the benefit of the atmospheric, climate and radiation protection research communities. To this end, here we present a new calibration method for activity concentrations below 20 Bq m−3 and a prototype of the first portable radon monitor capable of achieving uncertainties of 5% (at k = 2) at these concentrations. Compliance checking of policy-driven regulations regarding greenhouse gas (GHG) emissions is an essential component of climate change mitigation efforts. Independent, reliable ‘top down’ methods that can be applied consistently for estimating local- to regional-scale GHG emissions (such as the radon tracer method (RTM)) are an essential part of this process. The RTM relies upon observed radon and GHG concentrations and measured or modeled radon fluxes. Reliable radon flux maps could also significantly aid EU member states comply with European COUNCIL DIRECTIVE 2013/59/EURATOM. This article also introduces the traceRadon project, key aims of which include outlining a standardized approach for application of the RTM, creating infrastructure with a traceability chain for radon concentration and radon flux measurements, and developing tools for the validation of radon flux models. Since radon progeny dominate the terrestrial gamma dose rate, the planned traceRadon activities are also expected to improve the sensitivity of radiation protection early warning networks because of the correlation known to exist between radon flux and ambient equivalent dose rates.

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Abstract. Radon (222Rn) gas is the largest source of public exposure to naturally occurring radioactivity and the identification of radon priority areas is required by the Council Directive 2013/59/Euratom. Radon is also used as a tracer to improve atmospheric transport models and to indirectly estimate greenhouse gas (GHG) fluxes using the Radon Tracer Method (RTM). This method is based on the correlation between atmospheric concentrations of radon and GHG, together with information on the radon flux data. For radiological data, all European countries have installed networks of automatic gamma dose rate monitoring stations and report the real-time information gathered to the European Radiological Data Exchange Platform (EURDEP). So far, atmospheric radon activity concentrations and radon fluxes are not yet reported in EURDEP, nor routinely measured within the European radiological networks although these observations could help to avoid false positives results. Due to above applications, there is a need of building a metrological chain to ensure high quality radon activity concentrations and radon flux measurements. Both climate and radiation protection research communities underline the need for improved traceability in low-level atmospheric radon measurements (Khanbabaee et al., 2021). The EMPIR project 19ENV01 traceRadon1 is aimed towards providing the necessary measurement infrastructure and transfer standards to fulfil this need. Results of this project are particularly important for improving independent GHG emission estimates that support national reporting under the Paris Agreement on climate change and for the Council Directive 2013/59/Euratom, thus benefitting two large scientific communities. In this paper, early results, such as new activity standard developments and an overview of commercial and research radon monitors are presented and discussed. These results will feed into the traceRadon project with respect to radionuclide metrology in air and its potential for the improvement of the RTM.

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