We have created polaritons in a harmonic potential trap analogous to atoms in optical traps. The trap can be loaded by creating polaritons 50 micrometers from its center that are allowed to drift into the trap. When the density of polaritons exceeds a critical threshold, we observe a number of signatures of Bose-Einstein condensation: spectral and spatial narrowing, a peak at zero momentum in the momentum distribution, first-order coherence, and spontaneous linear polarization of the light emission. The polaritons, which are eigenstates of the light-matter system in a microcavity, remain in the strong coupling regime while going through this dynamical phase transition.
In the past decade, there has been an increasing number of experiments on spontaneous Bose coherence of excitons and polaritons. Four major areas of research are reviewed here: three-dimensional excitons in the bulk semiconductor Cu2O, two-dimensional excitons in coupled quantum wells, Coulomb drag experiments in coupled two-dimensional electron gases, and polaritons in semiconductor microcavities. The unifying theory of all these experiments is the effect of spontaneous symmetry breaking in the Bose-Einstein condensation phase transition.
Bose-Einstein condensation of excitons is a unique effect in which the electronic states of a solid can self-organize to acquire quantum phase coherence. The phenomenon is closely linked to Bose-Einstein condensation in other systems such as liquid helium and laser-cooled atomic gases. This is the first book to provide a comprehensive survey of this field, covering theoretical aspects as well as recent experimental work. After setting out the relevant basic physics of excitons, the authors discuss exciton-phonon interactions as well as the behaviour of biexcitons. They cover exciton phase transitions and give particular attention to nonlinear optical effects including the optical Stark effect and chaos in excitonic systems. The thermodynamics of equilibrium, quasi-equilibrium, and nonequilibrium systems are examined in detail. The authors interweave theoretical and experimental results throughout the book, and it will be of great interest to graduate students and researchers in semiconductor and superconductor physics, quantum optics, and atomic physics.
Nearly one decade after the first observation of Bose-Einstein condensation in atom vapors and realization of matter-wave (atom) lasers, similar concepts have been demonstrated recently for polaritons: half-matter, half-light quasiparticles in semiconductor microcavities. The half-light nature of polaritons makes polariton lasers promising as a new source of coherent and nonclassical light with extremely low threshold energy. The half-matter nature makes polariton lasers a unique test bed for many-body theories and cavity quantum electrodynamics. In this article, we present a series of experimental studies of a polariton laser, exploring its properties as a relatively dense degenerate Bose gas and comparing it to a photon laser achieved in the same structure. The polaritons have an effective mass that is twice the cavity photon effective mass, yet seven orders of magnitude less than the hydrogen atom mass; hence, they can potentially condense at temperatures seven orders of magnitude higher than those required for atom Bose-Einstein condensations. Accompanying the phase transition, a polariton laser emits coherent light but at a threshold carrier density two orders of magnitude lower than that needed for a normal photon laser in a same structure. It also is shown that, beyond threshold, the polariton population splits to a thermal equilibrium Bose-Einstein distribution at in-plane wave number k ʈ > 0 and a nonequilibrium condensate at kʈ ϳ 0, with a chemical potential approaching to zero. The spatial distributions and polarization characteristics of polaritons also are discussed as unique signatures of a polariton laser. E xperimentally realized macroscopic degenerate boson systems, such as lasers, superfluid He 3 and He 4 , the Bardeen-CooperSchreiffer state in superconductors, and Bose-Einstein condensation (BEC) of atomic vapors, have deepened our fundamental understanding of macroscopic quantum orders and led to novel research tools as well as applications. A missing member from the family has been a macroscopically ordered state of weakly interacting bosons in condensed matter systems. Exciton and polariton BECs are the most promising candidates in this category. Since they were first proposed in the 1960s (1-3), tremendous efforts have been engaged in the search (4-13). Exciton and polariton BECs are attractive yet elusive because of the complications inherent to solid-state systems with strong Coulomb interactions. It is a formidable task to describe the excitations in solids in full detail. The common approach is to treat the stable ground state of an isolated system as a quasivacuum and to introduce quasiparticles as units of elementary excitation, which only weakly interact with each other. An exciton is a typical example of such a quasiparticle. As a result of optical excitation from the crystal ground state, an exciton consists of a bound pair of an electron and hole whose Coulomb interaction serves as the binding energy. Excitons have integral total spin, thus they behave like bosons, weakly interac...
During the past ten years, coupled quantum wells have emerged as a promising system for experiments on Bose condensation of excitons, with numerous theoretical and experimental studies aimed at the demonstration of this effect. One of the issues driving these studies is the possibility of long-range coherent transport of excitons. Excitons in quantum wells typically diffuse only a few micrometres from the spot where they are generated by a laser pulse; their diffusion is limited by their lifetime (typically a few nanoseconds) and by scattering due to disorder in the well structure. Here we report photoluminescence measurements of InGaAs quantum wells and the observation of an effect by which luminescence from excitons appears hundreds of micrometres away from the laser excitation spot. This luminescence appears as a ring around the laser spot; almost none appears in the region between the laser spot and the ring. This implies that the excitons must travel in a dark state until they reach some critical distance, at which they collectively revert to luminescing states. It is unclear whether this effect is related to macroscopic coherence caused by Bose condensation of excitons.
We report new results of Bose-Einstein condensation of polaritons in specially designed microcavities with a very high quality factor, on the order of 10 6 , giving polariton lifetimes of the order of 100 ps. When the polaritons are created with an incoherent pump, a dissipationless, coherent flow of the polaritons occurs over hundreds of microns, which increases as density increases. At high density, this flow is suddenly stopped, and the gas becomes trapped in a local potential minimum, with strong coherence.
In this Letter we report on lateral diffusion measurements of excitons at low temperature in double quantum wells of various widths. The structure is designed so that excitons live up to 30 micros and diffuse up to 500 microm. Particular attention is given to establishing that the transport occurs by exciton motion. The deduced exciton diffusion coefficients have a very strong well width dependence, and obey the same power law as the diffusion coefficient for electrons.
We report on new experiments and theory that unambiguously resolve the recent puzzling observation of large diameter exciton emission halos around a laser excitation spot in two dimensional systems. We find a novel separation of plasmas of opposite charge with emission from the sharp circular boundary between these two regions. This charge separation allows for cooling of initially hot optically generated carriers as they dwell in the charge reservoirs for very long times.
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