The theory of superconductor-ferromagnet (S-F) heterostructures with two ferromagnetic layers predicts the generation of a long-range, odd-in-frequency triplet pairing at non-collinear alignment (NCA) of the magnetizations of the F-layers. This triplet pairing has been detected in a Nb/Cu 41 Ni 59 /nc-Nb/Co/CoO x spin-valve type proximity effect heterostructure, in which a very thin Nb film between the F-layers serves as a normal conducting (nc) spacer. The resistance of the sample as a function of an external magnetic field shows that for not too high fields the system is superconducting at a collinear alignment of the Cu 41 Ni 59 and Co layer magnetic moments, but switches to the normal conducting state at a NCA configuration. This indicates that the superconducting transition temperature T c for NCA is lower than the fixed measuring temperature. The existence of a minimum T c , at the NCA regime below that one for parallel or antiparallel alignments of the F-layer magnetic moments, is consistent with the theoretical prediction of a singlet superconductivity suppression by the long-range triplet pairing generation.An odd-in-frequency triplet pairing generation in singlet superconductor/ferromagnet thin-film heterostructures was predicted theoretically [1][2][3]. At least two ferromagnetic layers (F 1 ,F 2 ) with a non-collinear alignment of their magnetizations, are required to couple the conventional opposite-spin singlet s-wave pairing channel with the unconventional, odd-triplet s-wave pairing channel. The latter one is of extraordinary long range in F layers [1,2,4], because the magnetized conduction band of a ferromagnetic metal serves as an eigenmedia supporting the equal-spin pairing.Intense activities followed to formulate optimal conditions and realize experimental schemes for the generation and detection of this odd-triplet pairing utilizing the Josephson effect [5][6][7][8][9][10][11][12][13][14].

Abstract. The upper critical magnetic field H c2 in thin-film FSF trilayer spinvalve cores is studied experimentally and theoretically in geometries perpendicular and parallel to the heterostructure surface. The series of samples with variable thicknesses d F1 of the bottom and d F2 of the top Cu 41 Ni 59 F-layers are prepared in a single run, utilizing a wedge deposition technique. The critical field H c2 is measured in the temperature range 0.4 − 8 K and for magnetic fields up to 9 Tesla. A transition from oscillatory to reentrant behavior of the superconducting transition temperature versus F-layers thickness, induced by an external magnetic field, has been observed for the first time. In order to properly interpret the experimental data, we develop a quasiclassical theory, enabling one to evaluate the temperature dependence of the critical field and the superconducting transition temperature for an arbitrary set of the system parameters. A fairly good agreement between our experimental data and theoretical predictions is demonstrated for all samples, using a single set of fit parameters. This confirms adequacy of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) physics in determining the unusual superconducting properties of the studied Cu 41 Ni 59 /Nb/Cu 41 Ni 59 spin-valve core trilayers.Experimental and theoretical analysis of the upper critical field in FSF trilayers 2

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We fabricated a nanolayered hybrid superconductor-ferromagnet spin-valve structure, the resistive state of which depends on the preceding magnetic field polarity. The effect is based on a strong exchange bias (about -2 kOe) on a diluted ferromagnetic copper-nickel alloy and generation of a long range odd in frequency triplet pairing component. The difference of high and low resistance states at zero magnetic field is 90% of the normal state resistance for a transport current of 250 μA and still around 42% for 10 μA. Both logic states of the structure do not require biasing fields or currents in the idle mode.

The theoretical description of the Fulde-Ferrell-Larkin-Ovchinnikov like state establishing in nanostructered bilayers of ferromagnetic (F) and superconducting (S) material leads to critical temperature oscillations and reentrant superconductivity as the F-layer thickness gradually increases. The experimental realization of these phenomena is an important prerequisite for the fabrication of the Ferromagnet/Superconductor/Ferromagnet core structure of the superconducting spin-valve. A switching of the spin-valve is only expected if such nonmonotonic critical temperature behavior is observed in F/S bilayers as well as in the S/F bilayers, a combination of which the spin-valve core structure can be regarded to consist of. In our former investigations we could demonstrate the required non-monotonic behavior of the critical temperature in S/F bilayers. In this study we succeeded in the preparation of F/S bilayers, where the superconducting material is now grown on top of the ferromagnetic metal, which show deep critical temperature oscillations as a function of the ferromagnetic layer thickness as well as an extinction and recovery, i.e. a reentrant behavior, of superconductivity.Especially, the latter is necessary to obtain a spin-valve with a large critical temperature shift between the parallel and antiparallel configurations of magnetizations in the F layers.