Strong-field laser excitation of solids can produce extremely nonlinear electronic and optical behaviour. As recently demonstrated, this includes the generation of high harmonics extending into the vacuum-ultraviolet and extreme-ultraviolet regions of the electromagnetic spectrum. High harmonic generation is shown to occur fundamentally differently in solids and in dilute atomic gases. How the microscopic mechanisms in the solid and the gas differ remains a topic of intense debate. Here we report a direct comparison of high harmonic generation in the solid and gas phases of argon and krypton. Owing to the weak van der Waals interaction, rare (noble)-gas solids are a near-ideal medium in which to study the role of high density and periodicity in the generation process. We find that the high harmonic generation spectra from the rare-gas solids exhibit multiple plateaus extending well beyond the atomic limit of the corresponding gas-phase harmonics measured under similar conditions. The appearance of multiple plateaus indicates strong interband couplings involving multiple single-particle bands. We also compare the dependence of the solid and gas harmonic yield on laser ellipticity and find that they are similar, suggesting the importance of electron-hole recollision in these solids. This implies that gas-phase methods such as polarization gating for attosecond pulse generation and orbital tomography could be realized in solids.
The mechanism of growth of fibrils of the β-amyloid peptide (Aβ) was studied by means of a physics-based coarse-grained united-residue (UNRES) model and molecular dynamics (MD) simulations. To identify the mechanism of monomer addition to an Aβ1–40 fibril, an unstructured monomer was placed at a 20 Å distance from a fibril template, and allowed to interact freely with it. The monomer was not biased towards the fibril conformation, by either the force field or the MD algorithm. By using a coarse-grained model with replica exchange MD, a longer time scale was accessible making it possible to observe how the monomers probe different binding modes during their search towards the fibril conformation. Although different assembly pathways were seen, they all follow a dock-lock mechanism, with two distinct locking stages, which is consistent with data from experiments on fibril elongation. Whereas these experiments have not been able to characterize the conformations populating the different stages, we have been able to describe these different stages explicitly by following free monomers as they dock onto a fibril template and adopt the fibril conformation; i.e., we describe fibril elongation step by step, at the molecular level. During the first stage of the assembly, “docking”, the monomer tries different conformations. After docking, the monomer is locked into the fibril through two different locking stages. In the first stage the monomer forms hydrogen bonds with the fibril template along one of the strands in a two-stranded β hairpin; in the second stage, hydrogen bonds are formed along the second strand, locking the monomer into the fibril structure. The data reveal a free-energy barrier separating the two locking stages. The importance of hydrophobic interactions and hydrogen bonds in the stability of the Aβ fibril structure was examined by carrying out additional canonical MD simulations of oligomers with different numbers of chains (4 to 16 chains) with the fibril structure as the initial conformation. The data confirm that the structures are stabilized largely by hydrophobic interactions and show that the intermolecular hydrogen bonds are highly stable and contribute to the stability of the oligomers as well.
We have synthesized polycrystalline samples of the noncentrosymmetric superconductor Mo 3 Al 2 C by arc and RF melting, measured its transport, magnetic and thermodynamic properties, and computed its band structure.Experimental results indicate a bulk superconducting transition at T c ~ 9.2 K, while the density of states at the Fermi surface is found to be dominated by Mo d-orbitals. Using the measured values for the lower critical field H c1 , upper critical field H c2 , and the specific heat C, we estimated the thermodynamic critical field H c (0), coherence length ξ(0), penetration depth λ(0), and the Ginzburg-Landau parameter κ(0). The specific heat jump at T c , ΔC/γT c = 2.14, suggests that Mo 3 Al 2 C is moderately-to-strongly coupled, consistent with the fast opening of the gap, as evidenced by the rapid release of entropy below T c from our electronic specific heat measurements. Above 2K the electronic specific heat exhibits the power law behavior, suggesting that synthesis of single crystals and measurements at lower temperature are needed to establish whether the gap is anisotropic. The estimated value of the upper critical field H c2 (0) is close to the calculated Pauli limit, therefore further studies are needed to determine whether the absence of an inversion center results in a significant admixture of the triplet component of the order parameter.
We explore the analogy between quark confinement and the Meissner effect in superconductors. We measure the response of color-magnetic "supercurrents" from Dirac magnetic monopoles to the presence of a static quark-antiquark pair in fourdimensional U(1) lattice gauge theory. Our results indicate that in the confined phase these currents screen the color-electric flux due to the quarks in an electric analogy of the Meissner effect. We show that U(1) lattice gauge theory obeys both a dual London equation and an electric fluxoid quantization condition.12.38. Aw, 11.15.Ha, 74.30.ci, 74.60.Ec Typeset Using REVTEX 1
We investigate high-order harmonic generation in a solid, modeled as a multi-level system dressed by a strong infrared laser field. We show that the cutoff energies and the relative strengths of the multiple plateaus that emerge in the harmonic spectrum can be understood both qualitatively and quantitatively by considering a combination of adiabatic and diabatic processes driven by the strong field. Such a model was recently used to interpret the multiple plateaus exhibited in harmonic spectra generated by solid argon and krypton [Ndabashimiye et al., Nature 534, 520 (2016)]. We also show that when the multi-level system originates from the Bloch state at the Γ point of the band structure, the laser-dressed states are equivalent to the Houston states [Krieger el al. Phys. Rev. B 33, 5494 (1986)] and will therefore map out the band structure away from the Γ point as the laser field increases. This leads to a semi-classical three-step picture in momentum space that describes the high-order harmonic generation process in a solid. arXiv:1609.09852v1 [quant-ph] 30 Sep 2016
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