This work demonstrates that mid-infrared quantum cascade lasers operating under external optical feedback can output a chaotic dynamics through low-frequency fluctuations close to 77 K. Results also show that the birth of chaotic dynamics is not limited to near-threshold pumping levels. In addition, when the semiconductor material is cooled down from room temperature to 77 K, it is found that the laser destabilization takes place at a lower feedback ratio which proves that quantum cascade lasers are sensitive to temperatures, likely due to changes in the upper state lifetime. These examinations are meaningful for chaotic operation of quantum cascade lasers in secure atmospheric transmission lines and optical countermeasure systems.

Mid-infrared free-space optical communication has a large potential for high speed communication due to its immunity to electromagnetic interference. However, data security against eavesdroppers is among the obstacles for private free-space communication. Here, we show that two uni-directionally coupled quantum cascade lasers operating in the chaotic regime and the synchronization between them allow for the extraction of the information that has been camouflaged in the chaotic emission. This building block represents a key tool to implement a high degree of privacy directly on the physical layer. We realize a proof-of-concept communication at a wavelength of 5.7 μm with a message encryption at a bit rate of 0.5 Mbit/s. Our demonstration of private free-space communication between a transmitter and receiver opens strategies for physical encryption and decryption of a digital message.

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