The pressure-dependent optoelectronic properties of all-inorganic perovskite CsPbBr 3 nanocrystals (NCs) are investigated with steady-state and transient spectroscopy. The steady-state absorption and photoluminescence (PL) spectra under pressure show that CsPbBr 3 NCs pass through three electronic states (ES-I, ES-II, and ES-III) separated with two knee points located at 0.38 and 1.08 GPa, respectively, which are also confirmed by the PL dynamics. Analyzed with the two-carrier model of free carriers and trapped carriers, the PL dynamics show that the lifetime increases in ES-I, decreases in ES-II, and increases in ES-III for free carriers, while it is almost invariable for trapped carriers. The transformation from ES-I to ES-II is assigned to the contraction of the Pb−Br bond length while the transformation from ES-II to ES-III originated mostly from the distortion of the PbBr 6 octahedron. Apparently, the contraction of the Pb−Br bond and the distortion of octahedra benefit the tailoring of the generation and diffusion of carriers during the CsPbBr 3 NCs compression. These results in this work help us to design and optimize the perovskite-based optoelectronic devices of high performance.

We study a double-cavity optomechanical system in which a movable mirror with perfect reflection is inserted between two fixed mirrors with partial transmission. This optomechanical system is driven from both fixed end mirrors in a symmetric scheme by two strong coupling fields and two weak probe fields. We find that three interesting phenomena: coherent perfect absorption (CPA), coherent perfect transmission (CPT), and coherent perfect synthesis (CPS) can be attained within different parameter regimes. That is, we can make two input probe fields totally absorbed by the movable mirror without yielding any energy output from either end mirror (CPA); make an input probe field transmitted from one end mirror to the other end mirror without suffering any energy loss in the two cavities (CPT); make two input probe fields synthesized into one output probe field after undergoing either a perfect transmission or a perfect reflection (CPS). These interesting phenomena originate from the efficient hybrid coupling of optical and mechanical modes and may be all-optically controlled to realize novel photonic devices in quantum information networks.

No abstract

We study the optical response of cold rubidium atoms driven into the four-level Y configuration exhibiting two high Rydberg levels in the regime of electromagnetically induced transparency (EIT). Atoms excited to either Rydberg level interact with each other just via self-blockade potentials (I) or also via cross blockade potentials (II). Numerical results show a few interesting quantum phenomena on the transmitted properties of a weak probe field owing to controlled single and double Rydberg blockade. In case (I), it is viable to switch between single-photon outputs with vanishing (invariable) two-photon (three-photon) correlation and photon-pair outputs with vanishing (invariable) three-photon (two-photon) correlation. Such output switch can be easily done by modulating frequencies and intensities of two strong coupling fields to create a degenerate EIT window or two separated El 1 windows. In case (II), we find that two-photon and three-photon correlations decrease together at a degenerate EIT window center while increasing together between two separated EIT windows. Such consistent changes are observed because both correlations are modified by the identical polarizability degradation though depending on single and double Rydberg blockade, respectively.

No abstract