In the pursuit of broadband photodetection materials from visible to mid-IR region, the fresh three-dimensional topological insulators (3D TIs) are theoretically predicted to be a promising candidate due to its Dirac-like stable surface state and high absorption rate. In this work, a self-powered inorganic/organic heterojunction photodetector based on n-type 3D TIs Bi 2 Te 3 combined with p-type pentacene thin film was designed and fabricated. Surprisingly, it was found that the Bi 2 Te 3 /pentacene heterojunction photodetector exhibited a fast and wideband response from 450 to 3500 nm. The optimized responsivity of photodetector reached 14.89 A/W, along with the fast response time of 1.89 ms and the ultrahigh external quantum efficiency of 2840%. Moreover, at the mid-IR 3500 nm, our devices demonstrated a responsivity of 1.55 AW −1 , which was several orders of magnitude higher than that of previous 3D TIs photodetector. These excellent properties indicate that the inorganic/organic heterojunction, that is, the combination of 3D TIs with organic materials, is an exciting structure for high performance photodetectors in the wideband detection region. On account of the fact that the device is constructed on mica substrate, this work also represents a potential scenario for flexible optoelectronic devices. KEYWORDS: inorganic/organic heterojunction, wideband photodetector, Bi 2 Te 3 thin films, self-powered, fast response, flexible
A new approach has been proposed to derive the expressions for three-dimensional radiation stress using solutions of the pressure and velocity distributions and the coordinate transformation function that are derived from a Lagrangian description wherein the pressure is zero (relative to the atmospheric pressure) at the sea surface. Using this approach, analytical expressions of horizontal and vertical depth-dependent radiation stress are derived at a uniform depth and for a sloping bottom, respectively. The results of the depth integration of the expressions agree well with the theory of Longuet-Higgins and Stewart. In the case involving a sloping bottom, the radiation stress expressions from this study provide a better balance of the net momentum compared to those from previous studies.
A new method, Fe/Mg co-doping, is proposed for the first time to optimize thermochromic VO2 and the promising performance of VO2-based smart windows for practical applications is successfully achieved.
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