A theoretical framework to study linear and nonlinear Richtmyer-Meshkov instability (RMI) is presented. This instability typically develops when an incident shock crosses a corrugated material interface separating two fluids with different thermodynamic properties. Because the contact surface is rippled, the transmitted and reflected wavefronts are also corrugated, and some circulation is generated at the material boundary. The velocity circulation is progressively modified by the sound wave field radiated by the wavefronts, and ripple growth at the contact surface reaches a constant asymptotic normal velocity when the shocks/rarefactions are distant enough. The instability growth is driven by two effects: an initial deposition of velocity circulation at the material interface by the corrugated shock fronts and its subsequent variation in time due to the sonic field of pressure perturbations radiated by the deformed shocks. First, an exact analytical model to determine the asymptotic linear growth rate is presented and its dependence on the governing parameters is briefly discussed. Instabilities referred to as RM-like, driven by localized non-uniform vorticity, also exist; they are either initially deposited or supplied by external sources. Ablative RMI and its stabilization mechanisms are discussed as an example. When the ripple amplitude increases and becomes comparable to the perturbation wavelength, the instability enters the nonlinear phase and the perturbation velocity starts to decrease. An analytical model to describe this second stage of instability evolution is presented within the limit of incompressible and irrotational fluids, based on the dynamics of the contact surface circulation. RMI in solids and liquids is also presented via molecular dynamics simulations for planar and cylindrical geometries, where we show the generation of vorticity even in viscid materials.

In order to understand the dynamics of antioxidant actions of vitamin E (α-, β-, γ-, and δ-tocopherols, TocH) in biological systems, kinetic study of the formation and decay reactions of vitamin E radicals (α-, β-, γ-, and δ-tocopheroxyls, Toc•) has been performed in organic solvents, using stopped-flow spectrophotometry. By mixing α-, β-, γ-, and δ-TocH with aryloxyl radical (ArO•) in ethanol, the peaks of the UV–vis absorption due to α-, β-, γ-, and δ-Toc• radical appeared rapidly at ca. 430–340 nm, showed maxima, and then decayed gradually. The second-order rate constants (kf and 2kd) for the formation and decay (that is, bimolecular disproportionation) reactions of α-Toc• were determined by comparing the observed curves with the simulation ones obtained by the numerical calculation of differential equations related to the above reactions. From the results, the wavelengths of absorption maxima (λmaxi) and molar extinction coefficients (εi) (i = 1–4) of the optical spectra were determined for α-Toc• radical. Notable solvent effects have been observed for the reaction rates (kf and 2kd) and absorption spectra (λmaxi and εi) of α-Toc• radical. The scheme of the formation and decay reactions of α-, β-, γ-, and δ-Toc• radicals has been discussed based on the results obtained.

The amplification of a magnetic field due to the Richtmyer-Meshkov instability (RMI) is investigated by two-dimensional MHD simulations. Single-mode analysis is adopted to reveal definite relation between the nonlinear evolution of RMI and the field enhancement. It is found that an ambient magnetic field is stretched by fluid motions associated with the RMI, and the strength is amplified significantly by more than two orders of magnitude. The saturation level of the field is determined by a balance between the amplified magnetic pressure and the thermal pressure after shock passage. This effective amplification can be achieved in a wide range of the conditions for the RMI such as the Mach number of an incident shock and the density ratio at a contact discontinuity. The results suggest that the RMI could be a robust mechanism of the amplification of interstellar magnetic fields and cause the origin of localized strong fields observed at the shock of supernova remnants.

Motion of a fluid interface in Richtmyer-Meshkov instability is examined as a vortex sheet with the use of Birkhoff-Rott equation. This equation coupled with an evolution equation of the strength of the vortex sheet can describe all inviscid and incompressible fluid instabilities, i.e., Kelvin-Helmholtz, Rayleigh-Taylor, and Richtmyer-Meshkov instabilities, when Atwood numbers and initial distribution of vorticities are given. With these equations, detailed motion of a vortex core in the Richtmyer-Meshkov instability is investigated. For the Kelvin-Helmholtz and Rayleigh-Taylor instabilities, it is known that the curvature of a vortex sheet diverges at a finite time t=tc. This fact indicates that the solution loses its analyticity at tc. We show that the singularity formation also occurs in the Richtmyer-Meshkov instability and at the same time, accumulation of vorticity to some points where singularities are formed develops to the roll-up of a sheet when the sheet is regularized. We investigate motion of these accumulation points, i.e., vortex cores, and present that their trajectories and the strengths depend on the Atwood numbers.

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