Vanadium dioxide
(VO2) is a compelling candidate for
next-generation electronics beyond conventional silicon-based devices
due to the exhibition of a sharp metal–insulator transition.
In this study, in order to realize functional VO2 film
for flexible electronics, the growth of VO2 film directly
on a transparent and flexible muscovite via van der Waals epitaxy
is established. The heteroepitaxy and structural transition of VO2 films on muscovite are examined by a combination of high-resolution
X-ray diffraction, transmission electron microscopy, and Raman spectroscopy.
The unique metal–insulator transition of VO2 is
further revealed with a change in electrical resistance over 103 and a more than 50% variation of optical transmittance. Furthermore,
due to the nature of muscovite, the VO2/muscovite heterostructure
possesses superior flexibility and optical transparence. The approach
developed in this study paves an intriguing way to fabricate functional
VO2 film for the applications in flexible electronics.
Magnetic and multiferroic nanocomposites with two distinct phases have been a topic of intense research for their profound potential applications in the field of spintronics. In addition to growing high-quality phase separated heteroepitaxial nanocomposites, the strain engineering that is conducive to enhance the tunability of material properties, in general, and the magnetic properties, in particular, is of utmost importance in exploring new possibilities. Here, we investigated the magneto-structural coupling between antiferromagnetic BiFeO3 (BFO) and ferrimagnetic CoFe2O4 (CFO) in self-assembled vertically aligned nanocomposites grown on LaAlO3 (LAO) and SrTiO3 (STO) substrates. We found that BFO exhibits tetragonal (T) and rhombohedral (R) structures as the stable phases and CFO has high magnetocrystalline anisotropy even in the form of nanocomposites. The temperature and magnetic field dependent magnetizations of T_BFO-CFO/LAO and R_BFO-CFO/STO nanocomposites primarily demonstrate the magnetoelastic coupling between these variants.
Hybrid nanoparticles (NPs) composed of multiple components offer new opportunities for next-generation materials. In this study, a paradigm for the noble metal/ternary complex oxide hybrid NPs is reported by adopting pulsed laser ablation in liquids. As model hybrids, gold-spinel heterodimer (Au-CoFe2O4) and gold-pervoskite heterodimer (Au-SrTiO3) NPs are investigated. This work has demonstrated the diverse playgroup of NP conjugation enlarged by complex oxides.
This study reports a self-assembled multiferroic nanostructure, composed of PbTiO 3 (PTO) pillars embedded in a CoFe 2 O 4 (CFO) matrix, deposited on MgO(001) by pulsed laser deposition. The epitaxial relationship in the PTO-CFO nanostructure is ð100Þ½101 PTO k ð001Þ½101 CFO k ð001Þ ½101 MgO , confirming the in-plane aligned polarization of PTO. The perpendicular magnetic anisotropy of this thin film results from the magnetoelastic anisotropy that exceeds the shape anisotropy. The increased frequency and the enhanced intensity of the tetrahedral (T-) site phonon modes by increasing the magnetic field indicate strong magnetoelastic coupling through magnetostriction in this multiferroic nanostructure. The anisotropic Raman strength enhancement of the T-site phonon along different directions suggests the magnetoelastic coupling is most efficient in the in-plane direction. V
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