Spin-orbit coupling (SOC) is a key interaction in spintronics, allowing an electrical control of spin or magnetization and, vice versa, a magnetic control of electrical current. However, recent advances have revealed much broader implications of SOC that is also central to the design of topological states, including topological insulators, skyrmions, and Majorana fermions, or to overcome the exclusion of two-dimensional ferro-magnetism expected from the Mermin-Wagner theorem. SOC and the resulting emergent interfacial spin-orbit fields are simply realized in junctions through structural inversion asymmetry, while the anisotropy in magnetoresistance (MR) allows for their experimental detection. Surprisingly, we demonstrate that an all-epitaxial ferromagnet/ MgO/metal junction with only a negligible MR anisotropy undergoes a remarkable transformation below the superconducting transition temperature of the metal. The superconducting junction has a three orders of magnitude higher MR anisotropy and supports the formation of spin-triplet superconductivity, crucial for superconducting spintronics, and topologically-protected quantum computing. Our findings call for revisiting the role of SOC in other systems which, even when it seems negligible in the normal state, could have a profound influence on the superconducting response.For over 150 years magnetoresistive effects have provided attractive platforms to study spin-dependent phenomena and enable key spintronic applications [1]. Primarily, spintronics relies on junctions with at least two ferromagnetic layers to provide sufficiently large magnetoresistance (MR). Record room-temperature MR and commercial applications employ junctions of common ferromagnets, such as Co and Fe with MgO tunnel barrier [2,3]. Alternatively, MR occurs in single ferromagnetic layers with an interplay of interfacial spin-orbit coupling (SOC). However, in metallic systems this phenomenon, known as the tunneling anisotropic MR (TAMR) [4], is typically < 1% and precludes practical applications. Here we show experimentally that a negligible MR in an all-epitaxial ferromagnet/MgO/metal junction is drastically enhanced below the superconducting transition temperature of the metal. We explain this peculiar behavior with the role of the interfacial SOC in the formation of spin-triplet superconductivity which can enable low-power superconducting spintronics [5-7] and topologically-protected quantum computing [8,9].
The interaction between superconductivity and ferromagnetism in thin film superconductor/ferromagnet heterostructures is usually reflected by a change in superconductivity of the S layer set by the magnetic state of the F layers. Here we report the converse effect: transformation of the magnetocrystalline anisotropy of a single Fe(001) layer, and thus its preferred magnetization orientation, driven by the superconductivity of an underlying V layer through a spin-orbit coupled MgO interface. We attribute this to an additional contribution to the free energy of the ferromagnet arising from the controlled generation of triplet Cooper pairs, which depends on the relative angle between the exchange field of the ferromagnet and the spin-orbit field. This is fundamentally different from the commonly observed magnetic domain modification by Meissner screening or domain wall-vortex interaction, and it offers the ability to fundamentally tune magnetic anisotropies using superconductivity-a key step in designing future cryogenic magnetic memories.
Almost any use of a superconductor implies a nonequilibrium state. Remarkably, the nonequilibrium states induced by a microwave stimulus and the dynamics of magnetic flux quanta (Abrikosov vortices) can give rise to strikingly contrary effects: A sufficiently high-power electromagnetic field of GHz frequency can stimulate superconductivity, whereas fast vortex motion can trigger an instability abruptly quenching the superconducting state. Here, we advance or delay such dynamical quenching of the vortex state in Nb thin films by tuning the power and frequency of the microwave ac stimulus added to a dc bias current. The experimental findings are supported by time-dependent Ginzburg-Landau simulations and they can be explained qualitatively based on a model of "breathing mobile hot spots", implying a competition of heating and cooling of quasiparticles along the trajectories of moving fluxons whose core sizes vary in time. In addition, we demonstrate universality of the stimulation effect on the thermodynamic and transport properties of type II superconductors.
Controlling the perpendicular magnetic anisotropy (PMA) in thin films has received considerable attention in recent years due to its technological importance. PMA based devices usually involve heavy-metal (oxide)/ferromagnetic-metal bilayers, where, thanks to interfacial spin-orbit coupling (SOC), the in-plane (IP) stability of the magnetisation is broken. Here we show that in V/MgO/Fe(001) epitaxial junctions with competing in-plane and out-of-plane (OOP) magnetic anisotropies, the SOC mediated interaction between a ferromagnet (FM) and a superconductor (SC) enhances the effective PMA below the superconducting transition. This produces a partial magnetisation reorientation without any applied field for all but the largest junctions, where the IP anisotropy is more robust; for the smallest junctions there is a reduction of the field required to induce a complete OOP transition ($$H_\text {OOP}$$ H OOP ) due to the stronger competition between the IP and OOP anisotropies. Our results suggest that the degree of effective PMA could be controlled by the junction lateral size in the presence of superconductivity and an applied electric field. We also discuss how the $$H_\text {OOP}$$ H OOP field could be affected by the interaction between magnetic stray fields and superconducting vortices. Our experimental findings, supported by numerical modelling of the ferromagnet-superconductor interaction, open pathways to active control of magnetic anisotropy in the emerging dissipation-free superconducting spin electronics.
Here we describe a development of computer algorithm to simulate the Time Dependent Ginzburg-Landau equation (TDGL) and its application to understand superconducting vortex dynamics in confined geometries. Our initial motivation to get involved in this task was trying to understand better our experimental measurements on dynamics of superconductors with vortices at high frequencies leading to microwave stimulated superconductivity due to presence of vortex (Lara, et al., Scientific Reports, 5 9187 (2015)). arXiv:2001.07971v3 [cond-mat.supr-con]
Giant thermoelectric effects are known to arise at the interface between superconductors and strongly polarized ferromagnets, enabling the construction of efficient thermoelectric generators. We predict that the thermopower of such a generator can be completely controlled by a magnetic input signal: Not only can the thermopower be toggled on and off by rotating a magnet, but it can even be entirely reversed. This in situ control diverges from conventional thermoelectrics, where the thermopower is usually fixed by the device design.
Spin‐resolved electron symmetry filtering is a key mechanism behind giant tunneling magnetoresistance (TMR) in Fe/MgO/Fe and similar magnetic tunnel junctions (MTJs), providing room temperature functionality in spin electronics. However, the electron symmetry filtering breaks down under applied bias, dramatically reducing the TMR above 0.5 V. This strongly hampers the application range of MTJs. To circumvent the problem, resonant tunneling through quantum well states in thin layers has been used so far. This mechanism, however, is mainly effective at low temperatures. Here, a fundamentally different approach is demonstrated, providing a strong TMR boost under applied bias in V/MgO/Fe/MgO/Fe/Co hybrids. This pathway uses spin orbit coupling (SOC) controlled interfacial states in vanadium, which contrary to the V(001) bulk states are allowed to tunnel to Fe(001) at low biases. The experimentally observed strong increase of TMR with bias is modeled using two nonlinear resistances in series, with the low bias conductance of the first (V/MgO/Fe) element being boosted by the SOC‐controlled interfacial states, while the conductance of the second (Fe/MgO/Fe) junctions are controlled by the relative alignment of the ferromagnetic layers. These results pave a way to unexplored and fundamentally different spintronic device schemes, with tunneling magnetoresistance uplifted under applied electric bias.
Giant thermoelectric effects are known to arise at the interface between superconductors and strongly polarized ferromagnets, enabling the construction of efficient thermoelectric generators. We predict that the thermopower of such a generator can be completely controlled by a magnetic input signal: Not only can the thermopower be toggled on and off by rotating a magnet, but it can even be entirely reversed. This in situ control diverges from conventional thermoelectrics, where the thermopower is usually fixed by the device design.
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