In recent years, two-dimensional (2D) ternary materials have attracted wide attention due to their novel properties which can be achieved by regulating their chemical composition with a very great degree of freedom and adjustable space.However, as for the precise synthesis of 2D ternary materials, great challenges still lie ahead that hinder their further development. In this work, we demonstrated a simple and reliable approach to synthesize 2D ternary-layered BiOCl crystals through a microwave-assisted space-confined process in a short time (<3 minutes). Their ultraviolet (UV) detection performance was analyzed systematically. The photodetectors based on the as-obtained BiOCl platelets demonstrate high sensitivity to 266-nm laser illumination. The responsivity is calculated to be $8 A/W and the response time is up to be $18 ps. On the other hand, the device is quite stable after being exposed in the ambient air within 3 weeks and the response is almost unchanged during the measurement. The facile and fast synthesis of single crystalline BiOCl platelets and its high sensitivity to UV light irradiation indicate the potential optoelectronic applications of 2D BiOCl photodetectors. K E Y W O R D S2D materials, bismuth oxyhalide, microwave synthesis, UV photodetector Lixing Kang, Xuechao Yu, and Xiaoxu Zhao contributed equally to this work.
Magnetic skyrmion transport has been primarily based on the use of spin torques which require high current densities and face performance deterioration associated with Joule heating. In this work, we derive an analytical model for energy efficient skyrmion propagation in an antiferromagneticallycoupled bilayer structure using a magnetic anisotropy gradient. The interlayer skyrmion coupling provides a strong restoring force between the skyrmions, which not only prevents annihilation but also increases their forward velocity up to the order of km s -1 . For materials with low Gilbert damping parameter, the interlayer skyrmion coupling force can be amplified up to ten times, with a corresponding increase in velocity. Furthermore, the analytical model also provides insights into the dynamics of skyrmion pinning and relaxation of asymmetric skyrmion pairs in bilayer-coupled skyrmion systems.
High temperature studies of spin Hall effect have often been neglected despite its profound significance in real-world devices. In this work, high temperature spin torque ferromagnetic resonance measurement was performed to evaluate the effects of temperature on the Gilbert damping and spin Hall efficiency of Pt x cu 1−x. When the temperature was varied from 300 K to 407 K, the Gilbert damping was relatively stable with a change of 4% at composition x = 66%. Alloying Pt and Cu improved the spin Hall efficiency of Pt 75 cu 25 /Co/Ta by 29% to a value of 0.31 ± 0.03 at 407 K. However, the critical switching current density is dependent on the ratio between the Gilbert damping and spin Hall efficiency and the smallest value was observed when x = 47%. It was found that at this concentration, the spin transparency was at its highest at 0.85 ± 0.09 hence indicating the importance of interfacial transparency for energy efficient devices at elevated temperature.
A combination of the harmonic measurement and in situ Kerr imaging was used to experimentally determine the spin–orbit (SO) effective fields in a MgO/CoFeB/Ta structure. Here, we evaluate the SO effective fields through an analytical energy approach by transforming the anomalous Hall effect and planar Hall effect (PHE) voltage into a field dependency while imaging the magnetisation behaviour by differential Kerr microscopy. The analytical fitting to the measurement data indicates the significant coexistence of both a transverse field, , and longitudinal field, , in the longitudinal (HL = –12 Oe, HT = 8 Oe per 106 A cm−2) and transverse (HL = –12 Oe, HT = –17 Oe per 106 A cm−2) measurement schemes, respectively, due to the PHE. Additionally, dendritic-like domains, indicating the influence of the interfacial Dzyaloshinskii–Moriya interaction (DMI) at the CoFeB/Ta interface, were observed by in situ Kerr imaging. Micromagnetic simulations confirm the dendritic domain formation and edge tilting of the magnetisation, as being due to the DMI.
Magnetic skyrmions are novel topological spin textures on the nanoscale, and significant efforts have been taken to improve their zero-field density at room temperature (RT). In this work, we reported an approach of improving zero-field skyrmion density in [Pt/Co/Fe/Ir] 2 multilayers at RT by using the first-order reversal curve (FORC) technique to obtain information on the irreversible or reversible behaviors in the magnetization switching process. It was found from the FORC diagram that the magnetization reversal mechanism can be characterized into three stages: (1) reversible labyrinth stripe domains expanding or shrinking stage; (2) irreversible stripe domains fracturing stage; and (3) irreversible skyrmion annihilation stage. Furthermore, the zero-field skyrmion density can be highly improved by choosing reversal fields from the irreversible stripe domains fracturing stage. The highest skyrmion density was approached according to the maximum FORC distribution ρ. Our results have established the FORC measurement as a valuable tool for investigating magnetic multilayers of high skyrmion densities.
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