One of the leading issues in high-T(c) superconductors is the origin of the pseudogap phase in underdoped cuprates. Using polarized elastic neutron diffraction, we identify a novel magnetic order in the YB(2)Cu(3)O(6+) system. The observed magnetic order preserves translational symmetry of the lattice as proposed for orbital moments in the circulating current theory of the pseudogap state. To date, it is the first direct evidence of a hidden order parameter characterizing the pseudogap phase in high-T(c) cuprates.
Electronic phases with symmetry properties matching those of conventional liquid crystals have recently been discovered in transport experiments on semiconductor heterostructures and metal oxides at milli-Kelvin temperatures. We report the spontaneous onset of a onedimensional, incommensurate modulation of the spin system in the high-temperature superconductor YBa 2 Cu 3 O 6.45 upon cooling below ~150 K, while static magnetic order is absent above 2 K. The evolution of this modulation with temperature and doping parallels that of the in-plane anisotropy of the resistivity, indicating an electronic nematic phase that is stable over a wide temperature range. The results suggest that soft spin fluctuations are a microscopic route towards electronic liquid crystals, and nematic order can coexist with high-temperature superconductivity in underdoped cuprates.The electronic states near the Fermi level of high-temperature superconductors derive from the hybridized d-and p-orbitals of copper and oxygen ions in a square-planar network. At a doping level of 1/8 hole per Cu ion, experimental work on a specific superconducting cuprate family, (La,Nd) 2-x (Sr,Ba) x CuO 4 (La214), has shown that the two-dimensional electron system in the CuO 2 layers can support a state with uniaxial spin (1-3) and charge (1,4,5) order ("stripes"). Static stripe order implies that both translational and rotational symmetries of the copper-oxide square lattice are spontaneously broken. More unusual "electronic liquid crystal" states (6) that break the rotational symmetry of the lattice while at least partially preserving its translational symmetry can arise from quantum fluctuations of stripes(6-8), or from Fermi surface instabilities (9-11). Electronic nematic states have recently been discovered in semiconductor heterostructures (12) and in the bulk transition metal oxide Sr 3 Ru 2 O 7 (13). In both cases, however, they are stable only at milli-Kelvin temperatures and in high magnetic fields, and have thus far only been probed by transport measurements. We use neutron scattering to address the role of magnetic degrees of freedom in driving the formation of electronic liquid crystals, and to explore the presence of liquid-crystalline order in the cuprates.In the prior experiments on semiconductor heterostructures and on Sr 3 Ru 2 O 7 , the nematic director was aligned by external magnetic fields, resulting in a strong macroscopic anisotropy of 2 the current flow (12,13), analogous to the alignment of nematic domains in conventional liquid crystals by electric fields or confining walls. In the cuprates, subtle crystallographic distortions can serve as aligning fields for symmetry-broken electronic phases. They reduce the fourfold rotational symmetry of the CuO 2 layer to a twofold rotational or mirror symmetry by introducing a slight (~1%) difference between the in-plane lattice parameters. In stripe-ordered La214, the stripe domains in every CuO 2 layer are aligned by such a twofold axis, but the layers are stacked in such a way that the glob...
The proximity of superconductivity and antiferromagnetism in the phase diagram of iron arsenides [1, 2], the apparently weak electron-phonon coupling [3] and the "resonance peak" in the superconducting spin excitation spectrum [4, 5, 6, 7] have fostered the hypothesis of magnetically mediated Cooper pairing. However, since most theories of superconductivity are based on a pairing boson of sufficient spectral weight in the normal state, detailed knowledge of the spin excitation spectrum above the superconducting transition temperature T c is required to assess the viability of this hypothesis [8,9]. Using inelastic neutron scattering we have studied the spin excitations in optimally doped BaFe 1.85 Co 0.15 As 2 (T c = 25 K) over a wide range of temperatures and energies. We present the results in absolute units and find that the normal state spectrum carries a weight comparable to underdoped cuprates [10,11]. In contrast to cuprates, however, the spectrum agrees well with predictions of the theory of nearly antiferromagnetic metals [12], without complications arising from a pseudogap [13, 14, 15] or competing incommensurate spin-modulated phases [16]. We also show that the temperature evolution of the resonance energy follows the superconducting energy gap ∆, as expected from conventional Fermi-liquid approaches [17, 18]. Our observations point to a surprisingly simple theoretical description of the spin dynamics in the iron arsenides and provide a solid foundation for models of magnetically mediated superconductivity.
Intense paramagnon excitations in a large family of high-temperature superconductor
No abstract
The pseudogap is one of the most pervasive phenomena of high temperature superconductors [1]. It is attributed either to incoherent Cooper pairing setting in above the superconducting transition temperature Tc, or to a hidden order parameter competing with superconductivity. Here we use inelastic neutron scattering from underdoped YBa2Cu3O6.6 to show that the dispersion relations of spin excitations in the superconducting and pseudogap states are qualitatively different. Specifically, the extensively studied "hour glass" shape of the magnetic dispersions in the superconducting state [2,3,4] is no longer discernible in the pseudogap state and we observe an unusual "vertical" dispersion with pronounced in-plane anisotropy. The differences between superconducting and pseudogap states are thus more profound than generally believed, suggesting a competition between these two states. Whereas the high-energy excitations are common to both states and obey the symmetry of the copper oxide square lattice, the low-energy excitations in the pseudogap state may be indicative of collective fluctuations towards a state with broken orientational symmetry predicted in theoretical work [5,6,7,8].
The fundamental building block of the copper oxide superconductors is a Cu4O4 square plaquette. The plaquettes in most of these materials are slightly distorted to form a rectangular lattice, for which an influential theory predicts that high-transition-temperature (high-T(c)) superconductivity is nucleated in 'stripes' aligned along one of the axes. This theory received strong support from experiments that indicated a one-dimensional character for the magnetic excitations in the high-T(c) material YBa2Cu3O6.6 (ref. 4). Here we report neutron scattering data on 'untwinned' YBa2Cu3O6+x crystals, in which the orientation of the rectangular lattice is maintained throughout the entire volume. Contrary to the earlier claim, we demonstrate that the geometry of the magnetic fluctuations is two-dimensional. Rigid stripe arrays therefore appear to be ruled out over a wide range of doping levels in YBa2Cu3O6+x, but the data may be consistent with liquid-crystalline stripe order. The debate about stripes has therefore been reopened.
Using angular resolved photoemission spectroscopy we studied the evolution of the surface electronic structure of the topological insulator Bi(2)Se(3) as a function of water vapor exposure. We find that a surface reaction with water induces a band bending, which shifts the Dirac point deep into the occupied states and creates quantum well states with a strong Rashba-type splitting. The surface is thus not chemically inert, but the topological state remains protected. The band bending is traced back to Se abstraction, leaving positively charged vacancies at the surface. Because of the presence of water vapor, a similar effect takes place when Bi(2)Se(3) crystals are left in vacuum or cleaved in air, which likely explains the aging effect observed in the Bi(2)Se(3) band structure.
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