Mn, 74.20.Rp, 71.27.ϩa, 71.18.ϩy, 99.10.Cd Our recent paper 1 contains an error in the formula for the high-frequency Hall constant for the experimentally relevant case of electron doping. Equation ͑3͒ giving the highfrequency Hall constant for the case of electron filling, i.e., electron density nϾ1, should correctly readwhere ␦ϭ͉1Ϫn͉. This differs essentially from the quoted answer by a minus sign that was missed by us, in addition to a factor of 2. This equation is obtained from Eq. ͑2͒ in the paper, calculated for the case of hole doping nϽ1, by a particle-hole transformation. Performing a canonical transformation c i, ↔c i, † in the Kubo formulas for models of lattice fermions ͓see, e.g., Ref. 2, Eqs. ͑1͒ and ͑2͔͒ yieldsThe crucial overall minus sign arises from the fact that the Hall constant involves a three-current propagator, and each current picks up a minus sign under the transformation. Incidentally this identity results in a vanishing at half filling for bipartite lattices of the Hall function R H (1,t,,T) for any value of T, and the interaction strength.The changed sign in Eq. (3Ј) has a few implications which we would like to state explicitly. The recent experiment of Wang, Rogado, Cava, and Ong 3 on the transport Hall constant, actually sees the predicted linear T behavior over a wide temperature range 200 KрTр400 K with a positive slope. From Eq. (3Ј) above, we deduce that the appropriate t-J model description of the system has tϽ0, i.e., belongs to case B(ii) in our notation, at least at the composition x ϳ0.7.We note that with this correction, the sign of the hopping t suggested by our calculation is the same as the one favored by Refs. 4 and 5, at least for the nonsuperconducting range xϳ0.7. In this composition range, photoemission data 6,7 also suggest the same sign of t, with an unoccupied region around the center of Brillouin zone, namely the ⌫ point.
We report remarkable multiferroic effects in polycrystalline Bi 2 Fe 4 O 9 . High-resolution X-ray diffraction shows that this compound has orthorhombic structure. Magnetic measurements confirm an antiferromagnetic transition around 260 K. A pronounced inverse S-shape anomaly in the loss tangent of dielectric measurement is observed near the Néel temperature. This feature shifts with the application of magnetic field. These anomalies are indicative of substantial coupling between the electric and magnetic orders in this compound.
Our recent paper [1] contains an error in the formula for the high frequency Hall constant for the experimentally relevant case of electron doping. Eq(3) giving the high frequency Hall constant for the case of electron filling, i.e. electron density n > 1, should correctly readwhere δ = |1 − n|. This differs essentially from the quoted answer by a minus sign that was missed by us, and by a factor of 2. This equation is obtained from Eq(2) in the paper, calculated for the case of hole doping n < 1, by a particle hole transformation. Performing a canonical transformation c i,σ ↔ c † i,σ in the Kubo formulas for models of lattice fermions (see e.g. [2] Eqn(1,2) ) yields:The crucial overall minus sign arises from the fact that the Hall constant involves a three current propagator, and each current picks up a minus sign under the transformation. Incidentally this identity results in a vanishing at half filling for bipartite lattices of the Hall function R H (1, t, ω, T ) for any value of T, ω and the interaction strength.The changed sign in Eq(3') has a few implications which we would like to state explicitly. The recent experiment of Wang, Rogado, Cava and Ong [3] on the transport Hall constant, actually sees the predicted linear T behaviour over a wide temperature range 200 0 K ≤ T ≤ 400 0 K with a positive slope. From Eq(3') above, we deduce that the appropriate t − J model description of the system has t < 0, i.e. belongs to case B(ii) in our notation, at least at the composition x ∼ .7.We note that with this correction, the sign of the hopping t suggested by our calculation is the same as the one favoured by Refs [4,5], at least for the non superconducting range x ∼ .7. In this composition range, photoemission data [6,7] also suggest the same sign of t, with an unoccupied region around the center of Brillouin zone, namely the Γ point. Motivated by the recent discovery of superconductivity in two dimensional CoO2 layers, we present some possibly useful results of the RVB mean field theory applied to the triangular lattice. An interesting time reversal breaking superconducting state arises from strongly frustrated interactions. Away from half filling, the order parameter is found to be complex, and yields a fully gapped quasiparticle spectrum. The sign of the hopping plays a crucial role in the analysis, and we find that superconductivity is as fragile for one sign as it is robust for the other. NaxCoO2 · yH2O is argued to belong to the robust case, by comparing the LDA fermi surface with an effective tight binding model. The high frequency Hall constant in this system is potentially interesting, since it is pointed out to increase linearly with temperature without saturation for T > T degeneracy .
The adsorption of basic molecules is one method often used to characterize the Brpnsted and Lewis acidity of a surface. IR spectroscopy is used to characterize the complexes formed, and temperature-programmed desorption is used to determine the strength of binding.1 In general, solid state NMR has been employed to study either the surface site or the adsorbed molecule, but not to correlate the site of adsorption with the adsorbed molecule.1 2 A notable exception to this is found in the work of Slichter and co-workers.3 They used SEDOR (spin echo double resonance) NMR to determine a 195Pt-,3C distance, for CO adsorbed on a platinum surface.3 Since SEDOR is a static NMR experiment, it cannot always be applied to systems with a variety of species and, consequently, many overlapping resonances.
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