[1] Measurements obtained during the NASA Transport and Chemical Evolution over the Pacific (TRACE-P) experiment are used in conjunction with regional modeling analysis to evaluate emission estimates for Asia. A comparison between the modeled values and the observations is one method to evaluate emissions. Based on such analysis it is concluded that the inventory performs well for the light alkanes, CO, ethyne, SO 2 , and NO x . Furthermore, based on model skill in predicting important photochemical species such as O 3 , HCHO, OH, HO 2 , and HNO 3 , it is found that the emissions inventories are of sufficient quality to support preliminary studies of ozone production. These are important finding in light of the fact that emission estimates for many species (such as speciated NMHCs and BC) for this region have only recently been estimated and are highly uncertain. Using a classification of the measurements built upon trajectory analysis, we compare observed species distributions and ratios of species to those modeled and to ratios estimated from the emissions inventory. It is shown that this technique can reconstruct a spatial distribution of propane/benzene that looks remarkably similar to that calculated from the emissions inventory. A major discrepancy between modeled and observed behavior is found in the Yellow Sea, where modeled values are systematically underpredicted. The integrated analysis suggests that this may be related to an underestimation of emissions from the domestic sector. The emission is further tested by comparing observed and measured species ratios in identified megacity plumes. Many of the model derived ratios (e.g., BC/CO, SO x /C 2 H 2 ) fall within $25% of those observed and all fall outside of a factor of 2.5.
The first comprehensive set of in situ measurements of turbulence and dynamics in an experimental wildland grass fire should help improve fire models.-FJB
This paper is the second of two reviewing scientific literature from 100 years of research addressing interactions between the atmosphere and fire behaviour. These papers consider research on the interactions between the fuels burning at any instant and the atmosphere, and the interactions between the atmosphere and those fuels that will eventually burn in a given fire. The first paper reviews the progression from the surface atmospheric properties of temperature, humidity and wind to horizontal and vertical synoptic structures and ends with vertical atmospheric profiles. This second paper addresses plume dynamics and vortices. The review presents several questions and concludes with suggestions for areas of future research.
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