Two peat sequences were sampled in the vicinity of the main mining districts of the Vosges Mountains: Sainte-Marie-aux-Mines and Plancher-les-Mines. Lead isotopic compositions and excess lead fluxes were calculated for each of these radiocarbon-dated sequences. Geochemical records are in very good agreement with the mining history of the area, well known over the last millennium. Except for an anomaly corresponding to the Middle Bronze Age which has not yet been resolved, there is no clear geochemical evidence of local metal production in the Vosges before the 10th century as excess lead deposition archived between 500 BC and 500 AD is attributed to long-range transport of polluted particulate matter. The approach described here can be applied to other mining districts where archaeological evidence is scarce or even lacking, but where past exploitation is suspected
a b s t r a c tThe Discrete Cosine Transform (DCT) is a Fourier-related transform widely used in signal processing and well suited to the analysis of open outlines. This method was applied here to evaluate the discrimination power of the inner lateral rib for two palstave populations dating from the Middle Bronze Age, excavated in northwest France. A corpus of almost 400 palstaves (bronze axes) of the Breton and Norman types was processed, and compared to specimens found at Sermizelles in Burgundy. The procedure is robust and produces a discrimination in good agreement with the traditional typology. Besides the definition of a 'standard' shape for each population, the morphometrical approach allows shape disparity, which is generally inaccessible to the naked eye, to be visualised and quantified. Shape disparity indicates that, contrary to previous assumptions, the bronze axes from the Sermizelles hoards cannot be explained as an assortment of Breton and Norman palstaves alone. We believe that this approach is quick, reproducible, and generalisable enough to be applied to a wide variety of artefacts from different periods, in order to clarify their typology and even their origin.
Magnetic susceptibility, surface rock soiling, elemental composition and lead isotope ratios were measured in surface stone samples collected at different heights of a late 19th century building in Dijon, France. We targeted four limestone facades that differ in orientation and proximity to car traffic. It seems that zinc, copper, sulphur and cadmium are present as diffuse pollutants in urban atmosphere, at least at the scale of the building studied. In contrast, lead and arsenic exhibit point sources: automotive traffic and past coal-burning fly-ash emissions; both coherent with lead isotopic composition measurements. Parameter variations primarily result from exposition to rain washing or micro-scale runoff, and from the closeness, magnitude and origin of anthropogenic sources. Both anthropogenic particles and natural dust tend to be similarly affected by deposition/soiling and rain washing, which act dynamically as competitive processes. Examination of archival photographs suggests that soiling predominated in the past, when the air was rich in black dust, whereas equilibrium or even weathering may occur nowadays due to recent improvements or at least changes in air quality. Using the chemical composition of building facades to provide insights into the magnitude and dispersion of urban atmospheric pollutants may not always be straightforward because of uncertainties related to the period of accumulation.
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