Anisotropy of perpendicular field penetration into high- General rightsIt is not permitted to download or to forward/distribute the text or part of it without the consent of the author(s) and/or copyright holder(s), other than for strictly personal, individual use, unless the work is under an open content license (like Creative Commons). Disclaimer/Complaints regulationsIf you believe that digital publication of certain material infringes any of your rights or (privacy) interests, please let the Library know, stating your reasons. In case of a legitimate complaint, the Library will make the material inaccessible and/or remove it from the website. Please Ask the Library: http://uba.uva.nl/en/contact, or a letter to: Library of the University of Amsterdam, Secretariat, Singel 425, 1012 WP Amsterdam, The Netherlands. You will be contacted as soon as possible. AbstractThe geometry of penetration of a magnetic field oriented perpendicular to the surface of a superconductor is changed by the presence of a longitudinal field. This is studied directly by means of the magneto-optical technique in different high-Tc materials. In YBa2Cu307 single crystals Brandt's mode of magnetization is observed, namely, penetration of an AC field only along the longitudinal field even if the corresponding dimension of the sample is much longer than the other two. This anisotropy is the evidence that the force-free configuration of current and vortices cannot be destroyed by cutting and reconnection of the vortices in this 3D superconductor. On the contrary, the absence of the induced anisotropy in Bi2Sr2CaCu2Os single crystals reveals the independence of pancake vortices in CuO layers from longitudinal field which makes a realization of the force-free configuration impossible in the layered 2D superconductor. An intermediate effect in thin films indicates that vortices are almost normal to the film surface even if the applied field is nearly parallel to it. The described experiment can be used as a new tool to study the internal vortex structure in superconductors.
The role of orbital magnetism in the laser-induced demagnetization of Fe/Gd multilayers was investigated using time-resolved X-ray magnetic circular dichroism at 2-ps time resolution given by an xray streak camera. An ultrafast transfer of angular momentum from the spin via the orbital momentum to the lattice was observed which was characterized by rapidly thermalizing spin and orbital momenta. Strong interlayer exchange coupling between Fe and Gd led to a simultaneous demagnetization of both layers.1 Author to whom correspondence should be addressed; electronic mail: afbartelt@lbl.gov. 2 Author to whom correspondence should be addressed; electronic mail: a_scholl@lbl.gov. 2Ultrafast magnetic storage and processing is founded on our ability to control magnetism on picosecond and femtosecond time scales. Magnetic phase transitions conserve the total angular momentum and usually involve the crystal lattice as a quasi-infinite reservoir of angular momentum. A prototypical ultrafast magnetic phenomenon is the demagnetization after excitation by an intense laser pulse [1][2][3][4][5]. Here, the orbital momentum is crucial as it links the electron spin, which carries most of the magnetic moment, to the lattice via the spinorbit interaction. In this letter, we investigate the orbital momentum dynamics during an ultrafast demagnetization in the model system Fe/Gd using X-ray magnetic circular dichroism (XMCD) [6].The Fe/Gd multilayer consists of two metals of very different electronic structure. Fe has exchange-split 3d spin bands which intersect the Fermi surface, allowing both low-energy spin-flip (Stoner) and spin wave excitations (magnons). The spin momentum dominates the total angular momentum while the orbital momentum is quenched by the strong ligand field and only partially restored by the spin-orbit interaction. The coupling of the orbital momentum to the anisotropic ligand field enables the flow of angular momentum from the spin system to the lattice during the demagnetization. A direct photon-driven exchange of spin and orbital momentum as proposed by Hübner [7] would, for example, appear as a temporary accumulation of orbital and concomitant reduction of spin momentum. In contrast, a bottleneck caused by the spin-orbit interaction would be visible as a reduced orbital to spin momentum ratio. The second component of the multilayer, Gd, is best described as a Heisenberg ferromagnet with localized 4f electrons. Gd does not exhibit an orbital momentum in the 4f shell, which is half full. A large exchange energy of about 11 eV separates the majority and minority 4f states, inhibiting low-energy spin-flip excitations. Magnetic long range order in Gd is established via 4f-5d exchange with the Gd 5d valence states and their exchange interaction with Gd 5d orbitals of nearest neighbors [8]. Therefore, the Gd 4f demagnetization occurs indirectly via 4f-5d exchange and subsequent 5d electronphonon scattering while the Fe demagnetization occurs directly via 3d electron-phonon scattering. The Gd orbital momentum should t...
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