The fabrication and characterization of a glass containing a regular parallel array of submicrometer channels or capillaries are described. The capillaries are arranged in a two-dimensional hexagonal close packing configuration with channel diameters as small as 33 nanometers and packing densities as high as 3 x 10(10) channels per square centimeter. The high-temperature stability of the nanochannel glass array is well suited as a host or template for the formation of quantum confined semiconductor structures or as a mask for massively parallel patterned lithographic applications.
We report lasing characteristics of 40-60-microm-diameter Rhodamine 590/water solution droplets pumped by a 20-nsec-duration Q-switched laser. The Rhodamine/water solution provides a useful model system for studying the properties of oscillators based on whispering-gallery-wave spherical cavities. The low threshold for lasing, 10(4) W/cm(2) for 10(-4) M solutions, is consistent with particle size and a cavity Q factor of 10(4). Portions of the droplet lase purely in transverse electric (TE) modes, while other portions contain both TE and lower-Q transverse magnetic modes. In the far field, the lasing droplet approximates a coherent point source emitting in all directions.
Quantum-confined nanocrystallites of GaAs are fabricated in porous Vycor glass and the bound electronic nonlinear refractive index, the two-photon absorption coefficient, and the refraction from carriers generated by two-photon absorption are simultaneously determined using the Z-scan method and compared to those of bulk GaAs. The measured nonlinear refractive index is an order of magnitude larger than that of bulk GaAs at 1060 nm.
The limiting behavior of nigrosin dye dissolved in carbon disulfide was investigated in an f/5 defocusing geometry using 6 ns duration 532 nm laser excitation. Nigrosin dye is a broadband visible light absorber that is used here in conjunction with the large thermal nonlinearity of carbon disulfide solvent to defocus intense incident visible light. A limiting threshold energy of 40 nJ, corresponding to a fluence of only 100 mJ/cm2 in the solution, was observed with device absorption adjusted to 53%.
Gated detection of the output of a fiber-optic-coupled radiation dosimeter effectively eliminated the direct contribution of Cerenkov radiation to the signal. The radiation source was an external beam radiotherapy machine that provided pulses of 6-MeV x rays. Gated detection was used to discriminate the signal collected during the radiation pulses, including Cerenkov interference, from the signal collected between the radiation pulses due only to phosphorescence from the Cu(1+)-doped glass detector. Gated detection of the long-lived phosphorescence of the Cu(1+)-doped glass provided real-time dose measurements that were linear with the absorbed dose and that were accurate for all field sizes studied.
A novel approach for the fabrication of high-quality preforms for use in the fabrication of photonic crystal fibers is described. The preforms are fabricated in a multistep process that involves stacking a bundle with rods and (or) tubes of two dissimilar glasses, fusing the bundle, and then etching the fused bundle in acid to remove one of the two glasses. The procedure for fabrication of the fused preforms is similar to that used in the fabrication of microchannel plate glass and yields periodically spaced, uniform, round channels that extend through the length of the preform.
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