A structure composed of a monolayer of luminescent silicon quantum dots (Si-QDs) and a silver (Ag) film over nanosphere (AgFON) plasmonic nanostructure is prepared by precisely controlling the distance. A AgFON structure modifies both the photoluminescence (PL) and the PL excitation (PLE) spectra of a Si-QD monolayer significantly. It is shown that the spectral shape is very sensitive to the spacer thickness and the wavelength dependence of the PL and PLE enhancement factors agrees well with the absorptance spectra. Due to multiple surface plasmon resonances of a AgFON structure, in proper spacer thicknesses, simultaneous enhancements of the excitation cross section and the emission rate are achieved. In the wavelength range where the absorption cross section of Si-QDs is small, the PL enhancement factor averaged in a relatively wide region (10 × 10 mm2) reaches 12.

A continuous-wave (CW) broadband high-level optical quadrature squeezer is essential for high-speed large-scale fault-tolerant quantum computing on a time-domain-multiplexed continuous-variable optical cluster state. CW THz-bandwidth squeezed light can be obtained with a waveguide optical parametric amplifier (OPA); however, the squeezing level has been insufficient for applications of fault-tolerant quantum computation because of degradation of the squeezing level due to their optical losses caused by the structural perturbation and pump-induced phenomena. Here, by using mechanical polishing processes, we fabricated a low-loss quasi-single-mode periodically poled LiNbO3 (PPLN) waveguide, which shows 7% optical propagation loss with a waveguide length of 45 mm. Using the waveguide, we assembled a low-loss fiber-pigtailed OPA module with a total insertion loss of 21%. Thanks to its directly bonded core on a LiTaO3 substrate, the waveguide does not show pump-induced optical loss even under a condition of hundreds of milliwatts pumping. Furthermore, the quasi-single-mode structure prohibits excitation of higher-order spatial modes and enables us to obtain larger squeezing level. Even with including optical coupling loss of the modularization, we observe 6.3-dB squeezed light from the DC component up to a 6.0-THz sideband in a fully fiber-closed optical system. By excluding the losses due to imperfections of the modularization and detection, the squeezing level at the output of the PPLN waveguide is estimated to be over 10 dB. Our waveguide squeezer is a promising quantum light source for high-speed large-scale fault-tolerant quantum computing.

Figure S1. (a), (b) TEM images of Au-NPs/Si-QDs. Si-QDs are grown at 1200 o C.

Phase-sensitive detection is the essential projective measurement for measurement-based continuous-variable quantum information processing. The bandwidth of conventional electrical phase-sensitive detectors is up to several gigahertz, which would limit the speed of quantum computation. It is theoretically proposed to realize terahertz-order detection bandwidth by using all-optical phase-sensitive detection with an optical parametric amplifier (OPA). However, there have been experimental obstacles to achieve large parametric gain for continuous waves, which is required for use in quantum computation. Here, we adopt a fiber-coupled χ(2) OPA made of a periodically poled LiNbO3 waveguide with high durability for intense continuous-wave pump light. Thanks to that, we manage to detect quadrature amplitudes of broadband continuous-wave squeezed light. 3 dB of squeezing is measured up to 3 THz of sideband frequency with an optical spectrum analyzer. Furthermore, we demonstrate the phase-locking and dispersion compensation of the broadband continuous-wave squeezed light, so that the phase of the squeezed light is maintained over 1 THz. The ultra-broadband continuous-wave detection method and dispersion compensation would help to realize all-optical quantum computation with over-THz clock frequency.

Abstract