International audienceSilicone elastomers are available in different formulations that are mainly discriminated by their crosslinking mechanisms. Different chemical networks lead to diverse mechanical behaviours. This work aims at comparing three types of conventional silicone elastomers, one Liquid Silicone Rubber (LSR), one High Consistency Rubber (HCR) and one, thermoplastic, hydrogen bonded cross-linked elastomer (TPE). Each one is studied and compared in terms of network microstructure versus mechanical behaviour
One major challenge of biomaterial engineering is to mimic the mechanical properties of anisotropic, multifunctional natural soft tissues. Existing solutions toward controlled anisotropy include the use of oriented reinforcing fillers, with complicated interface issues, or UV‐curing processing through patterned masks, that makes use of harmful photosensitive molecules. Here, a versatile process to manufacture biocompatible silicone elastomer membranes by light degradation of the platinum catalyst prior to thermal cross‐linking is presented. The spatial control of network density is demonstrated by experimental and theoretical characterizations of the mechanical responses of patterned cross‐linked membranes, with a view to mimic advanced implantable materials.
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