There are few studies that evaluate dietary intakes and predictors of diet quality in older adults. The objectives of this study were to describe nutrient intakes and examine associations between demographic, economic, behavioral, social environment, and health status factors and diet quality. Cross-sectional data was from Black, White, and Hispanic adults ages 60-99 years, living independently in New York City and participating in the Cardiovascular Health of Seniors and the Built Environment Study, 2009-2011 (n=1306). Multivariable log-linear regression estimated associations between selected factors and good diet quality, defined as a Healthy Eating Index score based on the 2005 Dietary Guidelines for Americans (HEI-2005)>80. Dietary intakes were similar for men and women; intakes of energy, fiber, and the majority of micronutrients were below recommendations, while intakes of fats, added sugar, and sodium were within the upper range or exceeded recommendations. Hispanic ethnicity (Relative Risk, RR=1.37; 95% Confidence Interval, CI, 1.07-1.75), caloric intake <~1500 calories/day (RR=1.93; 95%CI, 1.37-2.71), adherence to a special diet (RR=1.23; 95%CI: 1.02-1.50), purchasing food at supermarkets at least once/week (RR=1.34; 95%CI, 1.04-1.74), and being married/living with a partner (RR=1.37; 95%CI, 1.10-1.71) were positively associated with HEI-2005>80. Consuming at least restaurant one meal/day was negatively associated with HEI-2005>80 (RR=0.69; 95%CI, 0.50-0.94). These findings identify specific groups of older adults, such as Blacks or those who live alone, who may benefit from dietary interventions, as well as specific modifiable behaviors among older adults, such as eating restaurant meals or shopping at supermarkets, which may be targeted through interventions.