[1] Detailed acoustic investigation of bubble streams rising from the seafloor were conducted during R/V Meteor cruise M72/3a at a deep submarine hydrocarbon seep environment. The area is located offshore Georgia (eastern part of the Black Sea) at a water depth between 840 m and 870 m. The sediment echosounder Parasound DS-3/P70 was used for detecting bubbles in the water column that causes strong backscatter in the echographs (''flares''). Employing the swath echsounder Kongsberg EM710 flares in the water column were mapped along the entire swath width of approximately 1000 m at high spatial resolution. The exact location of the flares could be extracted manually. Subsequently, the horizontally looking sonar Kongsberg digital telemetry MS1000 mounted on a remotely operated vehicle (ROV) was utilized to quantify the flux of bubbles. A model was developed that is based on the principle of finding the ''acoustic mass'' in order to quantify the bubble flux at various seeps. The acoustic approach from the backscatter data of the ROV sonar resulted in bubble fluxes in the range of 0.01 to 5.5 L/min (corresponding to 0.037 to 20.5 mol CH 4 /min) at in situ conditions ($850 m water depth, $9°C). Independent flux estimations using a funnel-shaped device showed that the acoustic model consistently produced lower values but the offset is less than 12%. Furthermore, the deviation decreased with increasing flux rates. A field of bubble streams was scanned three times from different directions in order to reveal the reproducibility of the method. Flux estimations yielded consistent fluxes of about 2 l/min (7.4 mol CH 4 /min) with variations of less than 10%. Although gas emissions have been found at many sites at the seafloor in a range of geological settings, the amount of escaping gas is still largely unknown. With this study presenting a novel method of quantifying bubble fluxes employing a horizontally looking sonar system, it is intended to contribute to the global effort of better constraining bubble fluxes at deep-sea settings.

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A chain of vertically rising discrete air bubbles represents a transition phenomenon from individual to continuum behavior in a bubbly liquid. Previous studies have reported that there is a preference for acoustic energy to propagate along the bubble chain and that this behavior could be explained by a coupled-oscillator model. However, it has recently been demonstrated that quantitative results from the coupled-oscillator model do not match experimental data. In this paper, it is shown how adding time delays to the coupled-oscillator model can produce results that are in better agreement with experimental data. In addition, the effects of time delays on the natural frequencies and damping of individual eigenmodes of the vertical bubble chain are also investigated. It was found that adding time delays can dramatically change the damping of the different modes of the system while having less dramatic impact on the natural frequencies of the individual eigenmodes. Counterintuitively, it is found that the effects of time delays appear to be more important when the bubbles are closer together than when they are farther apart.

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