We study layered metal-dielectric structures, which can be considered as a simple example of nanostructured metamaterials. We analyze the dispersion properties of such structures and demonstrate that they show strong optical nonlocality due to excitation of surface plasmon polaritons. We derive a model of a nonlocal effective medium for describing the effects of strong spatial dispersion in the multilayered metal-dielectric metamaterials. We obtain analytical expressions for the components of the effective permittivity tensor which depend on the wave vector and reveal that spatial dispersion effects exist in both directions across and along the layers.
We consider multilayered metal-dielectric metamaterials composed of alternating nanolayers of two types and calculate the components of their effective dielectric permittivity tensors as functions of both frequency and wave vector. We demonstrate that such structures can be described as strongly nonlocal uniaxial effective media, and we analyze how the nonlocal permittivity tensor components are related to other manifestations of strong spatial dispersion in such structures, and how the resonance of permittivity depends on the propagation direction.
We theoretically demonstrate the strong Purcell effect in ε-near-zero ultra-anisotropic uniaxial metamaterials with elliptic isofrequency surface. Contrary to the hyperbolic metamaterials, the effect does not rely on the diverging density of states and evanescent waves. As a result, both the radiative decay rate and the far-field emission power are enhanced. The effect can be realized in the periodic layered metal-dielectric nanostructures with complex unit cell containing two different metallic layers.
Recently, hybrid halide perovskites have emerged as one of the most promising types of materials for thin-film photovoltaic and light-emitting devices because of their low-cost and potential for high efficiency. Further boosting their performance without detrimentally increasing the complexity of the architecture is critically important for commercialization. Despite a number of plasmonic nanoparticle based designs having been proposed for solar cell improvement, inherent optical losses of the nanoparticles reduce photoluminescence from perovskites. Here we use low-loss high-refractive-index dielectric (silicon) nanoparticles for improving the optical properties of organo-metallic perovskite (MAPbI 3 ) films and metasurfaces to achieve strong enhancement of photoluminescence as well as useful light absorption. As a result, we observed experimentally a 50% enhancement of photoluminescence intensity from a perovskite layer with silicon nanoparticles and 200% enhancement for a nanoimprinted metasurface with silicon nanoparticles on top. Strong increase in light absorption is also demonstrated and described by theoretical calculations. Since both silicon nanoparticle fabrication/deposition and metasurface nanoimprinting techniques are low-cost, we believe that the developed all-dielectric approach paves the way to novel scalable and highly effective designs of perovskite based metadevices.
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