An upconversion pumping scheme was used to produce cw laser action at 0.55 μm in YAlO3:Er3+ at temperatures up to 77 K on the 4S3/2→4I15/2 transition. Two infrared dye lasers at 792.1 and 839.8 nm were used as the pump sources for stepwise two-photon excitation of the 4S3/2 upper laser level at 18 406 cm−1. The laser operates in the fundamental TEM00 mode, and a cw output power of ∼1 mW was achieved with ∼200 mW pump power from each infrared dye laser.

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We have observed cw laser action on a new transition (4D3/2→4I11/2) of the Nd3+ ion at 380 nm. This was demonstrated in Nd:LaF3 using an upconversion pumping scheme in which near infrared (788 nm) and visible (591 nm) pump photons from cw dye lasers produce stepwise excitation of the Nd3+ ion. In addition, lasing was observed with a single pump source at wavelengths around 578 nm using doubly resonant, sequential absorption of two yellow photons. Single-mode, cw operation with an output power of 12 mW was measured at 20 K with 1% output coupling and pump powers of several hundred mW. At 77 K the maximum power dropped to 4 mW.

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