In the tunneling regime for strong laser field ionization of atoms, experimental studies have shown that a substantial fraction of atoms survive the laser pulse in many Rydberg states. To explain the origin of such trapping of population into Rydberg states, two mechanisms have been proposed : the first involves AC-Stark-shifted multiphoton resonances and the second, called frustrated tunneling ionization, leads to the recombination of tunneled electrons into Rydberg states. We use a very accurate spectral method based on complex sturmian functions to solve the time dependent Schrödinger equation for hydrogen in a linearly polarized infrared pulse and to calculate the tunneling probability in terms of the atomic ground state width. We examine the probability of excitation into Rydberg states as a function of the peak intensity for various pulse durations and two wavelengths, 800 nm and 1800 nm and try to explain the results in light of the two aforementioned mechanisms. For long pulses of 800 nm wavelength, the extreme sensitivity of the trapping of population into high-lying Rydberg states to the peak intensity, the well defined value and parity of the angular momentum of the populated Rydberg states and the presence of Freeman resonances can be explained using a multiphotonic excitation mechanism. For strong pulses of 1800 nm wavelength, in the so-called adiabatic or quasi-static tunneling regime, the oscillations of the excitation probability as a function of intensity are in phase opposition to the ionization probability and we observe a migration towards high values of the angular momentum with different distributions in the angular momentum at the maxima and minima of the oscillations. We also present a detailed study of how the excited state wave packet builds up in time during the interaction of the atom with the pulse.
We present kinematically complete theoretical calculations and experiments for transfer ionization in H + +He collisions at 630 keV/u. Experiment and theory are compared on the most detailed level of fully differential cross sections in the momentum space. This allows us to unambiguously identify contributions from the shake-off and binary encounter mechanisms of the reaction. It is shown that the simultaneous electron transfer and ionization is highly sensitive to the quality of a trial initial-state wave function.
We present calculations of the electron angular distributions in the single ionization of helium by 1-MeV proton impact at momentum transfer of 0.75 a.u. and ejected-electron energy of 6.5 eV. The results using the first and second Born approximations and the 3C model with different trial helium functions are compared to the experimental data. A good agreement between theory and experiment is found in the case of the 3C final state and a strongly correlated helium wave function. The electron-electron correlations in the He atom are found to influence the ratio of the binary and recoil peak intensities.
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