We investigate the Landau–Zener (LZ) like dynamics of decaying two- and three-level systems with decay rates and for levels with minimum and maximum spin projection. Non-adiabatic and adiabatic transition probabilities are calculated from diabatic and adiabatic bases for two- and three-level systems. We extend the familiar two-level model of atoms with decay from the excited state out of the system into the hierarchy of three-level models which can be solved analytically or computationally in a non-perturbative manner. Exact analytical solutions are obtained within the framework of an extended form of the proposed procedure which enables to take into account all possible initial moments rather than large negative time as in standard LZ problems. We elucidate the applications of our results from a unified theoretical basis that numerically analyzes the dynamics of a system as probed by experiments.
Quantum triangles can work as interferometers. Depending on their geometric size and interactions between paths, "beats" and/or "steps" patterns are observed. We show that when inter-level distances between level positions in quantum triangles periodically change with time, formation of beats and/or steps no longer depends only on the geometric size of the triangles but also on the characteristic frequency of the transverse signal. For large-size triangles, we observe the coexistence of beats and steps when the frequency of the signal matches that of non-adiabatic oscillations and for large frequencies, a maximum of four steps instead of two as in the case with constant interactions is observed. Small-size triangles also revealed counter-intuitive interesting dynamics for large frequencies of the field: unexpected two-step patterns are observed. When the frequency is large and tuned such that it matches the uniaxial anisotropy, three-step patterns are observed. We have equally observed that when the transverse signal possesses a static part, steps maximize to six. These effects are semi-classically explained in terms of Fresnel integrals and quantum mechanically in terms of quantized fields with a photon-induced tunneling process. Our expressions for populations are in excellent agreement with the gross temporal profiles of exact numerical solutions. We compare the semi-classical and quantum dynamics in the triangle and establish the conditions for their equivalence.
Exact analytical solutions to the dissipative time-dependent Schrödinger equation are obtained for a decaying two-state system with decay rates Γ 1 and Γ 2 for levels with extremal spin projections. The system is coherently driven with a pulse whose detuning is made up of two parts: a time-dependent part (chirp) of hyperbolictangent shape and a static part with real and imaginary terms. This gives us a wide range of possibilities to arbitrarily select the interaction terms. We considered two versions which led to decaying Demkov-Kunike (DK) models; the version in which the Rabi frequency (interaction) is a time-dependent hyperbolic-secant function (called decaying DK1 model) and the case when it is constant in time and never turns off (decaying DK2 model). Our analytical solutions account for all possible initial moments instead of only t 0 = 0 or t 0 = −∞ as for non-decaying models and may be useful for experiments on level crossings. Two complementary limits of the pulse detuning are considered and explored: the limit of fast (i) and slow rise (ii). In the case (i), the coupling between level positions in the first DK model collapses while the second DK model reduces to a Rabi model (constant Hamiltonian), in the case (ii), both DK models reduce to the LZ model. In both cases (i) and (ii), analytical approximated solutions which conveniently approach the exact solutions are derived.
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