A novel optical arrangement for heterodyne detection of laser-induced gratings based on the use of a phase mask for both excitation and probe beams provides phase stability and control without the need for an active stabilization scheme. The arrangement greatly simplifies the laser-induced grating experiment. The performance of the technique in both transmission and reflection geometries is illustrated through measurements of bulk and surface acoustic waves generated by picosecond laser pulses.

▪ Abstract  The mechanical and acoustic properties of thin films and multilayer assemblies are important both for technological applications of these materials and for basic scientific studies of their physical behavior. Techniques that use optical methods to monitor acoustic waves stimulated in thin films with short pulsed lasers are useful for accurately and nondestructively characterizing the high frequency acoustic physics of these systems. This review briefly summarizes some of these techniques and focuses on a method known as impulsive stimulated thermal scattering or transient grating photoacoustics. It describes the most advanced experimental techniques for performing this measurement and outlines its application to the study of acoustic waveguide modes in a variety of thin films. These measurements, coupled with models for the physics of the modes, can be used to determine intrinsic mechanical properties of materials and structures that occur, for example, in microelectronics and high-frequency acoustic filters. This article summarizes a selected set of existing applications and concludes with an overview of future directions that include studies of the acoustics of complex microstructures such as microfluidic networks and synthetic phononic crystals.

The relaxation of a spatially sinusoidal temperature perturbation in a dielectric crystal at a temperature comparable to or higher than the Debye temperature is investigated theoretically. We assume that most phonons contributing to the specific heat have a mean free path (MFP) much shorter than the thermal transport distance and can be described by the thermal diffusion model. Low-frequency phonons that may have MFP comparable to or longer than the grating period are described by the Boltzmann transport equation. These low-frequency phonons are assumed to interact with the thermal reservoir of high-frequency phonons but not with each other. Within the single mode relaxation time approximation, an analytical expression for the thermal grating relaxation rate is obtained. We show that the contribution of "ballistic" phonons with long MFP to the effective thermal conductivity governing the grating decay is suppressed compared to their contribution to thermal transport at long distances. The reduction in the effective thermal conductivity in Si at room temperature is found to be significant at grating periods as large as 10 μm.

The newly popular topic of "phonon diodes" is discussed in the context of a broader issue of reciprocity in reflection/transmission (R-T) of waves. We first review a theorem well known in electromagnetism and optics but underappreciated in acoustics and phonon physics, stating that the matrix of R-T coefficients for properly normalized amplitudes is symmetric for linear systems that conform to power conservation and time reversibility for wave fields. It is shown that linear structures proposed for "acoustic diodes" in fact do obey R-T reciprocity, and thus should not strictly be called diodes or isolators. We also review examples of nonlinear designs violating reciprocity, and conclude that an efficient acoustic isolator has not yet been demonstrated. Finally, we consider the relationship between acoustic isolators and "thermal diodes", and show that ballistic phonon transport through a linear structure, whether an acoustic diode or not, is unlikely to form the basis for a thermal diode.

Scattering of normally incident longitudinal and transverse acoustic waves by a randomly rough surface of an elastically isotropic solid is analyzed within the small perturbation approach. In the limiting case of a large correlation length L compared with the acoustic wavelength, the The results indicate that thermal transport models using Ziman's formula are likely to overestimate the heat flux dissipation due to boundary scattering, whereas modeling interface roughness as atomic disorder is likely to underestimate scattering.