The layers of a high-temperature novel GaAs:Fe diluted magnetic semiconductor (DMS) with an average Fe content up to 20 at. % were grown on (001) i-GaAs substrates using a pulsed laser deposition in a vacuum. The transmission electron microscopy (TEM) and energy-dispersive x-ray spectroscopy investigations revealed that the conductive layers obtained at 180 and 200 ºC are epitaxial, do not contain any second-phase inclusions, but contain the Fe-enriched columnar regions of overlapped microtwins. The TEM investigations of the non-conductive layer obtained at 250 ºC revealed the embedded coherent Fe-rich clusters of GaAs:Fe DMS. The x-ray photoelectron spectroscopy investigations showed that Fe atoms form chemical bonds with Ga and As atoms with almost equal probability and thus the comparable number of Fe atoms substitute on Ga and As sites. The n-type conductivity of the obtained conductive GaAs:Fe layers is apparently associated with electron transport in a Fe acceptor impurity band within the GaAs band gap. A hysteretic negative magnetoresistance (MR) was observed in the conductive layers up to room temperature (RT). MR measurements point to the out-of-plane magnetic anisotropy of the conductive GaAs:Fe layers related to the presence of the columnar regions. The studies of the magnetic circular dichroism confirm that the layers obtained at 180, 200 and 250 ºC are intrinsic ferromagnetic semiconductors and the Curie point can reach up to at least RT in case of the conductive layer obtained at 200 ºC. It was suggested that in heavily Fe-doped GaAs layers the ferromagnetism is related to the Zener double exchange between Fe atoms with different valence states via an intermediate As and Ga atom.
We investigate the nature of transport and ferromagnetic properties of the epitaxial GaAs structure with the Mn δdoped layer. To modify the properties of the structure electrically active radiation defects are created by irradiation with 50 keV helium ions and a fluence in the range of 1 × 10 11 -1 × 10 13 cm -2 . The investigations show that transport properties of the structure are determined by two parallel conduction channels (the channel associated with hole transport in a valence band and the channel associated with electron transport in the Mn-related impurity band) and that ferromagnetic properties are determined by electrons localized at allowed states within the Mn impurity band. The ferromagnetic properties of the Mn δ-layer region cannot be affected by the closely located InGaAs quantum well, since the presence of quantum well has negligible influence on the Mn impurity band filling by electrons.
The dynamics of Dirac-Weyl spin-polarized wavepackets driven by periodic electric field is considered for the electrons in a mesoscopic quantum dot formed at the edge of two-dimensional HgTe/CdTe topological insulator with Dirac-Weyl massless energy spectra, where the motion of carriers is less sensitive to disorder and impurity potentials. It was observed that the interplay of strongly coupled spin and charge degrees of freedom creates the regimes of irregular dynamics both in coordinate and spin channels. The border between the regular and irregular regimes determined by the strength and frequency of the driving field is found analytically within the quasiclassical approach by means of the Ince-Strutt diagram for Mathieu equation, and is supported by full quantum mechanical simulations of the driven dynamics.The investigation of quasienergy spectrum by Floquet approach reveals the presence of non-Poissonian level statistics which indicates the possibility of chaotic quantum dynamics and corresponds to the areas of parameters for irregular regimes within the quasiclassical approach. We found that the influence of weak disorder leads to partial suppression of the dynamical chaos. Our findings are of interest both for progress in a fundamental field of quantum chaotic dynamics and for further experimental and technological applications of spin-dependent phenomena in nanostructures based on topological insulators.
Semiconductor quantum dots have attracted tremendous attention owing to their novel electrical and optical properties as a result of their size dependent quantum confinement effects. This provides the advantage of tunable wavelength detection, which is essential to realize spectrally selective photodetectors. We report on the fabrication and characterization of a high performance narrow band ultraviolet photodetector (UV-B) based on Indium oxide (InO) nanocrystals embedded in aluminium oxide (AlO) matrices. The InO nanocrystals are synthesized in an AlO matrix by sequential implantation of In and [Formula: see text] ions and post-implantation annealing. The photodetector exhibits excellent optoelectronic performances with high spectral responsivity and external quantum efficiency. The spectral response shows a band-selective nature with a full width half maximum of ∼60 nm, and a responsivity reaching up to 70 A W under 290 nm at 5 V bias. The corresponding rejection ratio to visible region was as high as 8400. The high performance of this photodetector makes it highly suitable for practical applications such as narrow-band spectrum-selective photodetectors. The device design based on ion-synthesized nanocrystals could provide a new approach for realizing a visible-blind photodetector.
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