2023
DOI: 10.1021/acs.cgd.2c01345
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Zn(II) and Cd(II) Metal–Organic Frameworks with Azine-Functionalized Pores: Crystal Structures, Photoluminescence, Solvent Exchange, and Molecular Simulations of Carbon Dioxide Binding Sites

Abstract: Four neutral metal–organic frameworks (MOFs) {[Zn(bpdc)(3-bpmhz)]·1.5(dmf)} n MRT-1 (1), {[Zn(bpdc)(3-bpmhz)]·(dmf)·0.5(Py)} n MRT-2 (2), {[Zn(bpdc)(4-bpmhz)](MeOH)·0.5(H2O)} n MRT-3 (3), and {[Cd(bpdc)(bda4bPy)]·2.5(dmf)} n MRT-4 (4) (where MRT stands for the Moldova Research Team), along with a one-dimensional coordination polymer {[Zn(Hbpdc)2(3-bphz)(MeOH)2]·2(dmf)} n (5), a binuclear complex [Cd2(bpdc)2(3-bpmhz)(H2O)6] (6), and a two-dimensional coordination polymer {[Cd(bpdc)(dmso)(H2O)]·0.25(H2bpdc)… Show more

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