However, their mode volumes and high-quality (Q) factors are restricted to the optical diffraction limit in their dielectric media. [6,7] Besides, the investigation and the optimization of light-pump threshold of these microlasers face great challenges, especially in reaching an ultralow pump fluence down to the level of tens of µJ cm −2 . [8,9] A lower threshold can provide more opportunities in choosing laser materials without considering the strong-light damage, and also could create a higher external quantum efficiency of the laser. [10][11][12] Surface plasmon is the collective oscillation of free electrons in noble metal nanostructures, which breaks the diffraction limit through harvesting far-field light energy into near-field electromagnetic (EM) field. [13,14] The plasmonic nanostructures hold natural features in exhibiting ultrasmall mode volume, which enables the modulation of strong light-matter interactions and the creation of ultralow threshold for the application of designing microlasers. [15][16][17] Plasmonic nano/ microlasers have been achieved in a series of compound semiconductors and low-dimensional semiconductors, such as GaN, ZnO, CdS, and WS 2 . [18][19][20][21][22] But the harsh fabrication condition and the unsatisfied threshold are still in urgent to be improved, which may place hope in exploiting a new material family.Recently, perovskites have emerged as promising optical gain materials for achieving ultralow-threshold microlasers, owing to their excellent optical properties, such as large absorption coefficient, high photoluminescence (PL) quantum yield, and low non-radiative recombination rate. [23][24][25] By interacting with plasmonic nanostructures, lasing behaviors in perovskites have been reported to show attenuated threshold and high mode quality owing to plasmonic effects. [26][27][28] Previous works reported the preparation of plasmonic perovskite lasers by fabricating perovskite flakes or nanowires on dielectric/metal films, but they always exhibit multi-wavelength lasing peaks due to the complex cavity-modes of perovskites. [29][30][31] The investigation of pure single-mode and tunable modes in plasmonic perovskite microlasers with ultralow thresholds has rarely been reported so far, which may have a great significance in realizing future on-chip integration of nano/microlasers. [32] Here, we develop a chemical vapor deposition (CVD) method to fabricate CsPbBr 3 /Ag (hybrid) heterostructures for plasmonic microlasers with low lasing threshold. Ag nanowires Low-dimensional perovskite structures are ideal materials for nano/microlasers owing to their excellent optical gain properties and high emission efficiency. But it is still a challenge to achieve single-mode and tunable lasing behaviors in micro-scale perovskite, especially showing ultralow thresholds in tens of µJ cm −2 . In this work, CsPbBr 3 /Ag hemispheroids have been synthesized in a designed chemical vapor deposition (CVD) process. Benefiting from the whispering gallery resonance mode and plasmon-enhanced light-m...