Two recent analyses that have exhaustively explored potential anomalous couplings in the Wtb vertex using t-channel single-top-quark events selected from collision data at √ s = 8 TeV with the ATLAS detector are reviewed. The first one measures the top-quark polarisation and six W -boson spin opservables from angular asymmetries unfolded to parton level. The second one measures the normalised triple-differential angular decay rate of top quarks to simultaneously constrain all the anomalous couplings. The limits on the anomalous couplings improve the existing limits set by ATLAS at √ s = 7 TeV. In addition, searches for flavour-changing neutral current top-quark interactions based on data collected by ATLAS and CMS, are reviewed. Finally, a recent search for t → qH, with H → γγ, performed by ATLAS at √ s = 13 TeV is also presented, where previous LHC limits are improved.